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The recent discovery of superconductivity in oxygen-reduced monovalent nickelates has raised a new platform for the study of unconventional superconductivity, with similarities and differences with the cuprate high temperature…

Superconductivity · Physics 2021-03-16 Emily Been , Wei-Sheng Lee , Harold Y. Hwang , Yi Cui , Jan Zaanen , Thomas Devereaux , Brian Moritz , Chunjing Jia

We study by dynamical mean field theory the ground state of a quarter-filled Hubbard model of two bands with different bandwidths. At half-filling, this model is known to display an orbital selective Mott transition, with the narrower band…

Strongly Correlated Electrons · Physics 2018-07-11 Francesco Grandi , Adriano Amaricci , Massimo Capone , Michele Fabrizio

Hund's rule coupling ($\textit{J}$) has attracted much attention recently for its role in the description of the novel quantum phases of multi orbital materials. Depending on the orbital occupancy, $\textit{J}$ can lead to various…

We present a dynamical mean-field theory (DMFT) study of the charge and orbital correlations in finite-size La$_{0.5}$Ca$_{0.5}$MnO$_3$ (LCMO) nanoclusters. Upon nanostructuring LCMO to clusters of 3 nm diameter, the size reduction induces…

Strongly Correlated Electrons · Physics 2015-09-30 A. Valli , H. Das , G. Sangiovanni , T. Saha-Dasgupta , K. Held

The YNiO$_3$ nickelate is a paradigm d-electron oxide that manifests the intriguing temperature-mediated sequence of three phases transitions from (i) magnetically ordered insulator to (ii) paramagnetic (PM) insulator and then to (iii) PM…

Materials Science · Physics 2023-03-16 Oleksandr I. Malyi , Alex Zunger

We employ a density-functional theory plus dynamical mean-field theory framework to investigate the correlated electronic structure of the alternating single-layer trilayer (1313) polymorph of La$_3$Ni$_2$O$_7$ under pressure. At ambient…

Strongly Correlated Electrons · Physics 2024-10-30 Harrison LaBollita , Soumen Bag , Jesse Kapeghian , Antia S. Botana

We study the magnetic and spectral properties of a single-band Hubbard model for the infinite-layer nickelate compound LaNiO$_2$. As spatial correlations turn out to be the key ingredient for understanding its physics, we use two…

Strongly Correlated Electrons · Physics 2022-02-22 Marcel Klett , Philipp Hansmann , Thomas Schäfer

We conducted a comparative study of the rare-earth infinite-layer nickelates films, RNiO2 (R = La, Pr, and Nd) using resonant inelastic X-ray scattering (RIXS). We found that the gross features of the orbital configurations are essentially…

Using the local density approximation and its combination with dynamical mean-field theory, we show that electronic correlations induce a single-sheet, cuprate-like Fermi surface for hole-doped 1/1 LaNiO3 /LaAlO3 heterostructures, even…

Strongly Correlated Electrons · Physics 2009-12-15 P. Hansmann , Xiaoping Yang , A. Toschi , G. Khaliullin , O. K. Andersen , K. Held

Angle-resolved photoemission spectroscopy (ARPES) combined with band structure calculations have shown that the layered transition metal dichalcogenide(TMD) NiTe$_2$ is a type-II Dirac semimetal. However, conflicting conclusions were…

Strongly Correlated Electrons · Physics 2026-02-26 A. R. Shelke , C. -W. Chuang , S. Hamamoto , M. Oura , M. Yoshimura , N. Hiraoka , C. -N. Kuo , C. -S. Lue , A. Fujimori , A. Chainani

We investigate the crystal structure and the electronic properties of the trilayer nickelate La$_4$Ni$_3$O$_{10}$ by means of quantum mechanical calculations in the framework of the density functional theory. We find that, at low…

Strongly Correlated Electrons · Physics 2018-03-15 Danilo Puggioni , James M. Rondinelli

The recent discovery of superconductivity in hole-doped planar nickelates R1-xSrNiO2 (R=Pr,Nd) raises the foundational question of how the electronic structure and electronic correlations of these Ni1+ compounds compare to those of the Cu2+…

Motivated by recent photoemission measurements on the La$_{0.8}$Sr$_{0.2}$NiO$_2$, we carry out a systematic study of the infinite-layer nickelate using both dynamical mean-field theory and density matrix embedding theory. The renormalized…

Strongly Correlated Electrons · Physics 2024-11-07 Ziyan Chen , Yuxin Wang , Kun Jiang , Jiangping Hu

Optical conductivity spectra of single crystals of Ca_1-xSr_xVO_3 have been studied to elucidate how the electronic behavior depends on the strength of the electron correlation without changing the nominal number of electrons per vanadium…

Strongly Correlated Electrons · Physics 2009-10-31 H. Makino , I. H. Inoue , M. J. Rozenberg , Y. Aiura , I. Hase , S. Onari

Rare-earth nickelates exhibit a remarkable metal-insulator transition accompanied by a structural transition associated with a lattice `breathing' mode. Using model considerations and first-principles calculations, we present a theory of…

Strongly Correlated Electrons · Physics 2019-06-19 Oleg E. Peil , Alexander Hampel , Claude Ederer , Antoine Georges

Correlations between electrons and the effective dimensionality are crucial factors that shape the properties of an interacting electron system. For example, the onsite Coulomb repulsion, U, may inhibit, or completely block the intersite…

Strongly Correlated Electrons · Physics 2007-05-23 T. Valla , P. D. Johnson , Z. Yusof , B. Wells , Q. Li , S. M. Loureiro , R. J. Cava , M. Mikami , Y. Mori , M. Yoshimura , T. Sasaki

Due to the absence of interlayer coupling and inversion symmetry, transition metal dichalcogenide (MX$_2$) semiconductor monolayers exhibit novel properties that are distinctly different from their bulk crystals such as direct optical band…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Chung-Yu Wang , Guang-Yu Guo

The layered transition metal dichalcogenide vanadium disulfide (VS$_2$), which nominally has one electron in the $3d$ shell, is potent for strong correlation physics and is possibly another realization of an effective one-band model beyond…

Strongly Correlated Electrons · Physics 2016-07-12 Eric B. Isaacs , Chris A. Marianetti

The electronic and thermoelectric properties of one to four monolayers of MoS$_{2}$, MoSe$_{2}$, WS$_{2}$, and WSe$_{2}$ are calculated. For few layer thicknesses,the near degeneracies of the conduction band $K$ and $\Sigma$ valleys and the…

Materials Science · Physics 2014-04-03 Darshana Wickramaratne , Ferdows Zahid , Roger K. Lake

We report ab initio calculations of the dielectric function of six mono- and bilayer molybdenum dichalcogenides based in a Bethe Salpether equation+G$_0$W$_0$ ansatz, focussing on the excitonic transitions dominating the absorption spectrum…

Materials Science · Physics 2016-11-17 Roland Gillen , Janina Maultzsch