Related papers: A Novel Chiroptical Spectroscopy Technique
The spin-orbit interaction in a focused-reflected beam of light results in spatially non-uniform polarization in the beam cross-section due to the superposition of orthogonal field components and polarization-dependent interface reflection…
Recently, we proposed a metasurface design for chiral sensing that (i) results in enhanced chiroptical signals by more than two orders of magnitude for ultrathin, subwavelength, chiral samples over a uniform and accessible area, (ii) allows…
Photoelectron circular dichroism (PECD) is a method whereby randomly oriented chiral molecules are irradiated by circularly-polarized light, photoionizing electrons, which are measured in a momentum-resolved manner. This scheme permits…
(Abridged) In the first part of this thesis, a general methodology for applying image deconvolution to wide-field CCD imagery. Results show that wavelet-based deconvolution can increase limiting magnitude up to 0.6 mag and improve limiting…
Chirality refers to the property that an object and its mirror image cannot overlap each other by spatial rotation and translation, and can be found in various research fields. We here propose chiral chaos and construct a chiral chaotic…
Chirality, a fundamental concept describing an object cannot superpose with its mirror image, is crucial in optics and photonics and leads to various exotic phenomena, such as circular dichroism, and optical activity. Recent findings reveal…
Spectro-polarimetric signatures of accretion disks in X-ray binaries and active galactic nuclei contain information about the masses and spins of their central black holes, as well as the geometry of matter close to the compact objects.…
Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…
Circular dichroism is the differential rate of absorption of right- and left-handed circularly polarized light by chiral particles. Optical vortices which convey orbital angular momentum (OAM) possess a chirality associated with the…
We calculate optical forces and torques exerted on a chiral dipole by chiral light fields and reveal genuinely chiral forces in combining the chiral contents of both light field and dipolar matter. Here, the optical chirality is…
We report on a universal topological dichroism of chiral three-dimensional systems in response to the chirality of light. We show that chiral topological invariants result in integer-quantized dichroic excitation rate differences. Moreover,…
Sensing molecular chirality at the nanoscale has been a long-standing challenge due to the inherently weak nature of chiroptical signals, and nanophotonic approaches have proven fruitful in accessing these signals. However, in most cases,…
We formulate a transparent measure that quantifies chirality in single electron ionization triggered in atoms, which are achiral systems. We do so in the context of Ar driven by a new type of optical fields that consists of two…
A fast and general Bayesian inference framework to infer the physical properties of dichroic polarization using mid-infrared imaging- and spectro-polarimetric observations is presented. The Bayesian approach is based on a hierarchical…
In this work a method of spectroscopy without monochromators for the undulator radiation (UR) source is proposed. This method is based of changing the magnetic field in the undulator. Different variations of field modulations and…
An approach for measuring linear X-ray polarization over a broad-band using conventional spectroscopic optics is described. A set of multilayer-coated flats reflect the dispersed X-rays to the instrument detectors. The intensity variation…
The recent discovery that linearly polarized light with a helical wavefront can exhibit vortex dichroism (also referred to as helical dichroism) has opened up new horizons in chiroptical spectroscopy with structured chiral light. Recent…
Spin-resolved photoelectron spectroscopy (PES) is a major experimental probe of chirality-induced spin selectivity (CISS), yet it remains unclear whether the measured spin polarization reflects molecular chirality itself or the broader…
Many chirality-sensitive light-matter interactions are governed by chiral electron dynamics. Therefore, the development of advanced technologies harnessing chiral phenomena would critically benefit from measuring and controlling chiral…
Chirality refers to the asymmetry of objects that cannot be superimposed on their mirror image. It is a concept that exists in various scientific fields and has profound consequences. Although these are perhaps most widely recognized within…