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In this paper, we investigate the non-Markovian dynamics of a model to mimic the excitation energy transfer (EET) between chromophores in photosynthesis systems. The numerical path integral method is used. This method includes the…

Chemical Physics · Physics 2015-05-14 Xian-Ting Liang

Energy-changing electron-hydrogen atom collisions are crucial to regulating the energy balance in astrophysical and laboratory plasmas and relevant to the formation of stellar atmospheres, recombination in H-II clouds, primordial…

Instrumentation and Methods for Astrophysics · Physics 2015-06-17 Daniel Vrinceanu , Roberto Onofrio , Hossein R. Sadeghpour

Mean-field molecular dynamics based on path integrals is used to approximate canonical quantum observables for particle systems consisting of nuclei and electrons. A computational bottleneck is the sampling from the Gibbs density of the…

Numerical Analysis · Mathematics 2023-11-30 Xin Huang , Petr Plechac , Mattias Sandberg , Anders Szepessy

Synchrotron emissivities, absorptivities, and Faraday rotation and conversion coefficients are needed in modeling a variety of astrophysical sources, including Event Horizon Telescope (EHT) sources. We develop a method for estimating…

High Energy Astrophysical Phenomena · Physics 2024-05-24 Monika Moscibrodzka , Charles F. Gammie

A self-consistent method for calculating electron transport through a molecular device is proposed. It is based on density functional theory electronic structure calculations under periodic boundary conditions and implemented in the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

In this review we consider those processes in condensed matter that involve the irreversible flow of energy between electrons and nuclei that follows from a system being taken out of equilibrium. We survey some of the more important…

Materials Science · Physics 2007-05-23 A. P. Horsfield , D. R. Bowler , H. Ness , C. G. Sanchez , T. N. Todorov , A. J. Fisher

A general approach to calculate the diabatic surfaces for electron-transfer reactions is presented, based on first-principles molecular dynamics of the active centers and their surrounding medium. The excitation energy corresponding to the…

Materials Science · Physics 2009-11-11 P. H. -L. Sit , Matteo Cococcioni , Nicola Marzari

We analyze the attosecond electron dynamics in hydrogen molecular ion driven by an external intense laser field using ab-initio numerical simulations of the corresponding time-dependent Schr{\"{o}}dinger equation and Bohmian trajectories.…

Chemical Physics · Physics 2015-05-20 Norio Takemoto , Andreas Becker

We extract electron transport properties from atomistic simulations of a two-component plasma, by mapping the long-wavelength behaviour to a two-fluid model. The mapping procedure is performed via Markov Chain Monte Carlo sampling over…

Plasma Physics · Physics 2024-10-14 Pontus Svensson , Patrick Hollebon , Daniel Plummer , Sam M. Vinko , Gianluca Gregori

The complex amplitudes of the electronic wavefunctions on different sites are used as Kramers variables for describing Electron Transfer. The strong coupling of the electronic charge to the many nuclei, ions, dipoles, etc, of the…

Condensed Matter · Physics 2009-11-07 S. Aubry , G. Kopidakis

We present an effective theory for describing electron dynamics driven by an optical external field in a Schr\"{o}dinger's cat state. We show that the electron density matrix evolves as an average over trajectories $\{\rho_\alpha\}$…

Quantum Physics · Physics 2025-01-29 Shohei Imai , Atsushi Ono , Naoto Tsuji

We apply field-particle correlations -- a technique that tracks the time-averaged velocity-space structure of the energy density transfer rate between electromagnetic fields and plasma particles -- to data drawn from a hybrid Vlasov-Maxwell…

Plasma Physics · Physics 2020-08-26 Kristopher G. Klein , Gregory G. Howes , Jason M. TenBarge , Francesco Valentini

We consider trasfer-ionization in collisions of fast (3.6 -- 11 MeV/u) protons, alpha-particles and lithium nuclei with helium atoms. There are just a few basic mechanisms contributing to this process which can be grouped into correlated…

Atomic Physics · Physics 2015-06-05 A. B. Voitkiv , X. Ma

Transport of fast electron in overdense plasmas is of key importance in high energy density physics. However, it is challenging to diagnose the fast electron transport in experiments. In this article, we study coherent transition radiation…

The computational study of energy storage and conversion processes calls for simulation techniques that can reproduce the electronic response of metal electrodes under electric fields. Despite recent advancements in machine-learning methods…

Materials Science · Physics 2024-05-14 Andrea Grisafi , Augustin Bussy , Mathieu Salanne , Rodolphe Vuilleumier

In this paper we present a simple model for computing single electron exchange between light nuclei. The electronic capture is pictured as a tunnelling process in a model potential. This allows to analytically compute the transmission…

Atomic Physics · Physics 2007-05-23 Fabio Sattin

We describe a method for numerically incorporating electron--electron scattering in quantum wells for small deviations of the distribution function from equilibrium, within the framework of the Boltzmann equation. For a given temperature…

Condensed Matter · Physics 2009-10-28 Ben Yu-Kuang Hu , Karsten Flensberg

Molecular systems containing donor-bridge-acceptor sites or molecular antennas constitute promising candidates for organic photovoltaic device implementation. Photo-induced electron transfer in multi-chromophore molecular systems is defined…

Chemical Physics · Physics 2021-06-09 Duvalier Madrid-Úsuga , John H. Reina

Data for inelastic processes due to hydrogen atom collisions with iron are needed for accurate modelling of the iron spectrum in late-type stars. Excitation and charge transfer in low-energy Fe+H collisions is studied theoretically using a…

Solar and Stellar Astrophysics · Physics 2018-05-09 P. S. Barklem

We compare numerical methods for solving the radiative transfer equation in the context of the photoionization of intergalactic gaseous hydrogen and helium by a central radiating source. Direct integration of the radiative transfer equation…

Instrumentation and Methods for Astrophysics · Physics 2023-01-18 Ka-Hou Leong , Avery Meiksin , Althea Lai , K. H. To
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