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Here we employ the quasi-bound state in the continuum (quasi-BIC) resonance in all-dielectric metasurfaces for efficient nonlinear processes in consideration of the backward frequency conversion. We theoretically study the second-harmonic…

Optics · Physics 2024-06-28 Xu Tu , Siqi Feng , Jiajun Li , Yangguang Xing , Feng Wu , Tingting Liu , Shuyuan Xiao

We use the method of dynamical mean field thoery, to study the effect of Kondo resonance on optical third harmonic generation (THG) spectra of strongly correlated systems across the metal-insulator transition. We find that THG signals are…

Strongly Correlated Electrons · Physics 2015-06-25 S. A. Jafari , T. Tohyama , S. Maekawa

We demonstrate a novel scheme to dramatically enhance both the second- and third-harmonic generation in a graphene-insulator-graphene metasurface. The key underlying feature of our approach is the existence of a double-resonance phenomenon,…

Optics · Physics 2020-09-16 Jian Wei You , Nicolae C. Panoiu

We investigate the generation of ultraviolet (UV) second-harmonic radiation on the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By…

Optics · Physics 2016-12-19 Xiaohui Zhao , Yuanlin Zheng , Huaijin Ren , Ning An , Xuewei Deng , Xianfeng Chen

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…

Doubly enhanced third harmonic generation (THG) is realized by the electric dipole resonance (EDR) in silicon nanodisks placed onto a metallic film at near-infrared. By introducing the metal substrate, the perfect electric conductor (PEC)…

Optics · Physics 2019-12-30 Jin Yao , Na Liu , Guoxiong Cai , Qing Huo Liu

We show that the second harmonic generation (SHG) is enhanced in the chiral one-dimensional electron currents in a broad frequency range. The origin of the enhancement is two-fold: first, the linear dispersion of the current and the…

Mesoscale and Nanoscale Physics · Physics 2020-04-17 Ivan Iorsh , Gulnaz Rakhmanova

A comprehensive study of second harmonic generation on thermally oxidized MoS2 flakes with thickness ranging from monolayer up to seven layers is presented. Observing the fundamental nonlinear behavior for non-treated and oxidized MoS2…

Successful phase-matching methods for Third Harmonics Generation (THG) include phase-matching in birefringent crystal and quasi-phase-matching (QPM) in crystal with periodically poled domains. However, these methods are not feasible in some…

Optics · Physics 2013-07-25 Tan Yizhou , Yang Yisheng , Liao Jiali , Zhang Ming

Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…

Materials Science · Physics 2022-08-10 Wei Li , Yunpeng Ma , Tianyi Feng , Sergei V. Kalinin , Jing-Feng Li , Qian Li

Lithium niobate (LN) metasurfaces exhibit remarkable Pockels effect-driven electro-optic tunability, enabling dynamic control of optical responses through external electric fields. When combined with their high second-order nonlinear…

Optics · Physics 2025-08-19 Huifu Qiu , Xu Tu , Meibao Qin , Feng Wu , Tingting Liu , Shuyuan Xiao

The twist angle in transition metal dichalcogenide (TMD) heterobilayers is a compelling degree of freedom that determines electron correlations and the period of lateral confinement of moir\'e excitons. Here we perform polarization-resolved…

We report optical second-harmonic generation (SHG) in reflection from GaSe crystals of 1 to more than 100 layers using a fundamental picosecond pulsed pump at 1.58 eV and a supercontinuum white light pulsed laser with energies ranging from…

Mesoscale and Nanoscale Physics · Physics 2017-10-10 Yanhao Tang , Krishna C. Mandal , John A. McGuire , Chih Wei Lai

Here, we experimentally demonstrate an Indium Tin Oxide (ITO) Mach-Zehnder interferometer heterogeneously integrated in silicon photonics. The phase shifter section is realized in a novel lateral MOS configuration, which, due to favorable…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

Strongly Correlated Electrons · Physics 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

The non-linear propagation of the intense near-infrared (NIR) driving field in wide bandgap materials pose a challenge and an opportunity to control the spectral properties of high harmonic generation (HHG) in solids. Here, we have…

Optics · Physics 2023-07-06 Mukhtar Hussain , Gareth O Williams , Tayyab Imran , Marta Fajardo

We study third-harmonic generation (THG) in an excitonic insulator (EI) described in a two-band correlated electron model. Employing the perturbative expansion with respect to the external electric field, we derive the THG susceptibility…

Strongly Correlated Electrons · Physics 2021-12-28 Tetsuhiro Tanabe , Tatsuya Kaneko , Yukinori Ohta

Topological properties in quantum materials are often governed by symmetry and tuned by crystal structure and external fields, and hence symmetry-sensitive nonlinear optical measurements in a magnetic field are a valuable probe. Here we…

Mesoscale and Nanoscale Physics · Physics 2023-09-19 Shuang Wu , Zaiyao Fei , Zeyuan Sun , Yangfan Yi , Wei Xia , Dayu Yan , Yanfeng Guo , Youguo Shi , Jiaqiang Yan , David H. Cobden , Wei-Tao Liu , Xiaodong Xu , Shiwei Wu

Optical spectroscopy based on second-order nonlinearity is a critical technique for characterizing two-dimensional (2D) crystals as well as bioimaging and quantum optics. It is generally believed that second-harmonic generation (SHG) in…

Mesoscale and Nanoscale Physics · Physics 2026-01-14 Haoning Tang , Zhitong Ding , Tianyi Ruan , Zeyu Hao , Kenji Watanabe , Takashi Taniguchi , Haozhe Wang , Ali Javey , Feng Wang , Yuan Cao

Metal-organic molecular adsorbates on metallic surfaces offer the potential to both generate materials for future (spin-)electronics applications as well as a better fundamental understanding of molecule-substrate interaction, provided that…

Materials Science · Physics 2024-09-17 A. Eschenlohr , R. Shi , J. Chen , P. Zhou , U. Bovensiepen , W. Hübner , G. Lefkidis