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Perturbative methods are attractive to describe the electronic structure of molecular systems because of their low-computational cost and systematically improvable character. In this work, a two-step perturbative approach is introduced…

Chemical Physics · Physics 2023-11-15 Loris Delafosse , Amr Hussein , Saad Yalouz , Vincent Robert

The numerical cost of variational methods suggests using perturbative approaches to determine the electronic structure of molecular systems. In this work, a sequential construction of effective Hamiltonians drives the definition of…

Chemical Physics · Physics 2024-08-30 Oussama Bindech , Bastien Valentin , Saad Yalouz , Vincent Robert

Brillouin-Wigner (BW) perturbation theory is developed for both ground and excited states of open-shell nuclei. We show that with optimal partitioning of the many-body Hamiltonian proposed earlier by the authors [Z. Li and N. Smirnova,…

Nuclear Theory · Physics 2024-01-24 Zhen Li , Nadezda A. Smirnova

A Brillouin-Wigner perturbation theory is developed for open electromagnetic systems which are characterised by discrete resonant states with complex eigenenergies. Since these states are exponentially growing at large distances, a modified…

Optics · Physics 2012-05-23 E. A. Muljarov , W. Langbein , R. Zimmermann

First principles calculations based on many-electron perturbation theory methods, such as the \textit{ab initio} GW and GW plus Bethe-Salpeter equation (GW-BSE) approach, are reliable ways to predict quasiparticle and optical properties of…

Materials Science · Physics 2017-01-11 Felipe H. da Jornada , Diana Y. Qiu , Steven G. Louie

Second-order M{\o}ller-Plesset perturbation theory (MP2) often breaks down catastrophically in small-gap systems, leaving much to be desired in its performance for myriad chemical applications such as noncovalent interactions,…

Chemical Physics · Physics 2023-07-05 Kevin Carter-Fenk , Martin Head-Gordon

We develop the high frequency expansion based on the Brillouin-Wigner (B-W) perturbation theory for driven systems with spin-orbit coupling which is applicable to the cases of silicene, germanene and stanene. We compute the effective…

Mesoscale and Nanoscale Physics · Physics 2016-12-19 Priyanka Mohan , Ruchi Saxena , Arijit Kundu , Sumathi Rao

Three well-known perturbative approaches to deriving low-energy effective theories, the degenerate Brillouin-Wigner perturbation theory (projection method), the canonical transformation, and the resolvent methods are compared. We use the…

Strongly Correlated Electrons · Physics 2009-11-10 A. L. Chernyshev , Dimitrios Galanakis , Philip Phillips , A. V. Rozhkov , A. -M. S. Tremblay

The behavior of electronic states of one dimensional correlated disordered systems which are modelled by a tight binding Hamiltonian is studied analytically using the invariant measure method. The approach of Bovier is generalized to…

Condensed Matter · Physics 2009-10-28 K. Kundu , D. Giri , K. Ray

We propose a refined scheme of deriving an effective low-energy Hamiltonian for materials with strong electronic Coulomb correlations beyond density functional theory (DFT). By tracing out the electronic states away from the target degrees…

Strongly Correlated Electrons · Physics 2017-08-09 Motoaki Hirayama , Takashi Miyake , Masatoshi Imada , Silke Biermann

We present an approximation scheme based on selective Hilbert space truncation for characterizing non-thermal states of magnetic systems beyond spin-wave theory. We study applications to states that are inaccessible through linear spin-wave…

Strongly Correlated Electrons · Physics 2026-01-13 Wesley Roberts , Michael Vogl , Roderich Moessner , Gregory A. Fiete

We explore the possibility of calculating electronic excited states by using perturbation theory along a range-separated adiabatic connection. Starting from the energies of a partially interacting Hamiltonian, a first-order correction is…

Chemical Physics · Physics 2014-12-15 Elisa Rebolini , Julien Toulouse , Andrew M. Teale , Trygve Helgaker , Andreas Savin

We develop a numerical Brillouin-zone integration scheme for real-time propagation of electronic systems with time-dependent density functional theory. This scheme is based on the decomposition of a large simulation into a set of small…

Materials Science · Physics 2021-12-03 Shunsuke A. Sato

For the one-dimensional, extended Peierls--Hubbard model we calculate analytically the ground-state energy and the single-particle gap to second order in the Coulomb interaction for a given lattice dimerization. The comparison with…

Strongly Correlated Electrons · Physics 2009-11-11 Anja Grage , Florian Gebhard , Joerg Rissler

We discuss a discrete approach to the multiscale reductive perturbative method and apply it to a biatomic chain with a nonlinear interaction between the atoms. This system is important to describe the time evolution of localized solitonic…

Pattern Formation and Solitons · Physics 2010-11-23 G. A. Cassatella Contra , D. Levi

We present an elementary pedagogical derivation of the Brillouin-Wigner and the Rayleigh-Schr\"odinger perturbation theories with Epstein-Nesbet partitioning. A variant of the Brillouin-Wigner perturbation theory is also introduced, which…

Quantum Physics · Physics 2013-07-17 Sangyoub Lee , Cheol Ho Choi , Eunji Kim , Young Kyun Choi

In the `Many Interacting Worlds' (MIW) discrete Hamiltonian system approximation of Schr\"odinger's wave equation, introduced in \cite{hall_2014}, convergence of ground states to the Normal ground state of the quantum harmonic oscillator,…

Mathematical Physics · Physics 2024-01-30 Alex Loomis , Sunder Sethuraman

We propose a new approach to the Rayleigh-Schr\"{o}dinger perturbation expansions of bound states in quantum mechanics. We are inspired by the enormous flexibility of solvable interactions with several (N) discontinuities. Their standard…

Quantum Physics · Physics 2014-11-18 Miloslav Znojil

This report discusses two new ideas for using perturbation methods to solve the time-independent Schr\"odinger equation. The first concept begins with rewriting the perturbation equations in a form that is closely related to matrix…

Quantum Physics · Physics 2013-10-25 Gerald I. Kerley

We present a scalable single-particle framework to treat electronic correlation in molecules and materials motivated by Green's function theory. We derive a size-extensive Brillouin-Wigner perturbation theory from the single-particle…

Chemical Physics · Physics 2023-09-12 Christopher J. N. Coveney , David P. Tew
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