Related papers: A $^{3}$He-$^{21}$Ne Ramsey Comagnetometer with su…
We study the ability to implement unitary maps on states of the $I=9/2$ nuclear spin in \textsuperscript{87}Sr, a $d=10$ dimensional (qudecimal) Hilbert space, using quantum optimal control. Through a combination of nuclear spin-resonance…
The nuclear magnetic resonance (NMR) spectrum of spin-3/2 nuclei in a static magnetic field aligned with one of the electric field gradient (EFG) principal axes is developed analytically, based on fictitious spin-1/2 formalism. Compact…
Nuclear-spin qubits have long coherence time and are desirably applied into quantum information processing. However, the existing methods either fail to address single nucleus (such as nuclear magnetic resonance), or severely affect nuclear…
Electron spins in gate-defined quantum dots provide a promising platform for quantum computation. In particular, spin-based quantum computing in gallium arsenide takes advantage of the high quality of semiconducting materials, reliability…
Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…
Comagnetometers offer unique advantages in measuring exotic spin-dependent interactions by suppressing magnetic noise. Understanding the frequency response to exotic interactions is essential for evaluating and improving the sensitivity of…
We report on measurements of the spin lifetime of nuclear spins strongly coupled to a micromechanical cantilever as used in magnetic resonance force microscopy. We find that the rotating-frame correlation time of the statistical nuclear…
We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is…
NMR spin-spin relaxation in solids in strong magnetic fields is normally described only with the help of the secular part of the full spin-spin interaction Hamiltonian. This approximation is associated with the averaging of the spin-spin…
Local spectral functions and Nuclear Magnetic Relaxation (NMR) rates, 1/T1, for the spin-half Heisenberg antiferromagnet on the Kagome Lattice are calculated using Moriyas Gaussian approximation, as well as through an extrapolation of…
We report on the dynamics of the Rabi oscillation and the Larmor precession of $^{15}$N nuclear spin using nonselective short microwave pulses for initialization of $^{15}$N nuclear spins. We observe the Larmor precession of $^{15}$N…
The excellent sensitivities of quantum sensors are a double-edged sword: minuscule quantities can be observed, but any undesired signal acts as noise. This is challenging when detecting quantities that are obscured by such noise. Decoupling…
Low thermal polarization of nuclear spins is a primary sensitivity limitation for nuclear magnetic resonance. Here we demonstrate optically pumped (microwave-free) nuclear spin polarization of $^{13}\mathrm{C}$ and $^{15}\mathrm{N}$ in…
Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…
We report nuclear magnetic resonance (NMR) studies of the intercalated iron selenide superconductor (Tl, Rb)$_{y}$Fe$_{2-x}$Se$_2$ ($T_c = 32$ K). Single-crystal measurements up to 480 K on both $^{77}$Se and $^{87}$Rb nuclei show a…
The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultra-dense magnetic memory to the measurement of spins in complex structures with nanometer…
We propose a new method to detect short-range \textit{P-} and \textit{T-} violating interactions between nucleons, based on measuring the precession frequency shift of polarized $^3$He nuclei in the presence of an unpolarized mass. To…
Resistively detected nuclear magnetic resonance (NMR) is observed inside the ring-like structure, with a quantized Hall conductance of 6e^2/h, in the phase diagram of a two subband electron system. The NMR signal persists up to 400 mK and…
Nuclear magnetic resonance (NMR) experiments can reveal local properties in materials, but are often limited by the low signal-to-noise ratio. Spin squeezed states have an improved resolution below the Heisenberg limit in one of the spin…
Hybrid photoelectric detection of NV magnetic resonances (PDMR) is anticipated to lead to scalable quantum chip technology. To achieve this goal, it is crucial to prove that PDMR readout is compatible with the coherent spin control. Here we…