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We perform a combined analytical and numerical investigation to explore how an analytically designed pulse can precisely control the rotational motions of a single-molecular polariton formed by the strong coupling of two low-lying…

Quantum Physics · Physics 2023-08-04 Li-Bao Fan , Chuan-Cun Shu

The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…

Atomic Physics · Physics 2015-05-27 Seth T. Rittenhouse , M. Mayle , P. Schmelcher , H. R. Sadeghpour

Spontaneous orientation polarization (SOP) of polar molecules is formed in vacuum-deposited films by tilting their permanent dipole moment against the substrate surface direction. In this study, we developed SOP molecules with high…

Materials Science · Physics 2026-02-18 Masaki Tanaka , Rena Sugimoto , Nobuhumi Nakamura

We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…

We theoretically explore the precise control of a molecular polariton by strongly coupling the lowest three rotational states of a single molecule with a single-mode cavity. We examine two distinct cavity resonance configurations: a…

Quantum Physics · Physics 2025-02-17 Li-Bao Fan , Hai-Ji Li , Qi Chen , Hang Zhou , Heng Liu , Chuan-Cun Shu

Significant molecular orientation can be achieved by time-symmetric single-cycle pulses of zero area, in the THz region. We show that in spite of the existence of a combined time-space symmetry operation, not only large peak instantaneous…

Chemical Physics · Physics 2012-10-22 Juan Ortigoso

Coherent, optically dressed media composed of two-level molecular systems without inversion symmetry are considered as all-optically tunable sources of coherent radiation in the microwave domain. A theoretical model and a numerical toolbox…

Quantum Physics · Physics 2020-12-08 Piotr Gładysz , Piotr Wcisło , Karolina Słowik

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

Optics · Physics 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

We introduce a new scheme for controlling the sense of molecular rotation. By varying the polarization and the delay between two ultrashort laser pulses, we induce unidirectional molecular rotation, thereby forcing the molecules to rotate…

Quantum Physics · Physics 2015-05-13 Sharly Fleischer , Yuri Khodorkovsky , Yehiam Prior , Ilya Sh. Averbukh

So-called polar liquid crystals possess spontaneous long-range mutual orientation of their electric dipole moments, conferring bulk polarity to fluid phases of matter. The combination of polarity and fluidity leads to complex phase…

Soft Condensed Matter · Physics 2025-08-22 Jordan Hobbs , Calum J. Gibb , Richard J. Mandle

Pair production due to the Schwinger mechanism is modeled in a self-consistent approach taking into account the backreaction of the created particles on the field. The model uses the Boltzmann kinetic equation for the electrons and…

Plasma Physics · Physics 2011-03-09 Alexander Tarasenko

Vacuum-stimulated Raman transitions are driven between two magnetic substates of a rubidium-87 atom strongly coupled to an optical cavity. A magnetic field lifts the degeneracy of these states, and the atom is alternately exposed to laser…

Quantum Physics · Physics 2007-05-23 T. Wilk , S. C. Webster , H. P. Specht , G. Rempe , A. Kuhn

Fully internal and motional state controlled and individually manipulable polar molecules are desirable for many quantum science applications leveraging the rich state space and intrinsic interactions of molecules. While prior efforts at…

The generation of pulsed polarization entangled photon pair has been realized using type-I phase matching in the spontaneous parametirc downconversion process in a space cascaded two-crystal geometry. The optical axes of the crystal are…

Quantum Physics · Physics 2009-11-07 Bao-Sen Shi , Akihisa Tomita

The lack of a direct map between control fields and desired control objectives poses a significant challenge in applying quantum control theory to quantum technologies. Here, we propose an analytical framework to precisely control a limited…

Quantum Physics · Physics 2025-03-05 Qian-Qian Hong , Daoyi Dong , Niels E. Henriksen , Franco Nori , Jun He , Chuan-Cun Shu

We present a technique for generating light in an arbitrary polarization state. The technique is based on interference of two orthogonally polarized light beams, whose amplitudes and phases are controlled with a Mach-Zehnder inteferometer…

Applied Physics · Physics 2018-10-22 P. Wlodarczyk , S. Pustelny , D. Budker

We explore the electronic structure and rovibrational properties of an ultralong-range triatomic Rydberg molecule formed by a Rydberg atom and a ground state heteronuclear diatomic molecule. We focus here on interaction of Rb($27s$) Rydberg…

Atomic Physics · Physics 2015-06-22 Rosario González-Férez , H. R. Sadeghpour , Peter Schmelcher

Magnetic fields play a role in the dynamics of many astrophysical processes, but they are hard to detect. In a partially ionized plasma, a magnetic field works directly on the ionized medium but not on the neutral medium, which gives rise…

Solar and Stellar Astrophysics · Physics 2020-06-24 Boy Lankhaar , Wouter Vlemmings

A mechanism is suggested for creating well-collimated beams of neutral spin-polarized particles by means of magnetic fields. This mechanism can be used in atom lasers for the formation of directed coherent beams of atoms. The directed…

Condensed Matter · Physics 2007-05-23 V. I. Yukalov , E. P. Yukalova

The spin polarization of photoelectrons induced by an intense linearly polarized laser field is investigated using numerical solutions of the time-dependent Schr\"odinger equation in companion with our analytic treatment via the…

Atomic Physics · Physics 2024-02-20 Pei-Lun He , Zhao-Han Zhang , Karen Z. Hatsagortsyan , Christoph H. Keitel