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LixTMO2 (TM=Ni, Co, Mn) forms an important family of cathode materials for Li-ion batteries, whose performance is strongly governed by Li composition-dependent crystal structure and phase stability. Here, we use LixCoO2 (LCO) as a model…

Computational Engineering, Finance, and Science · Computer Science 2023-02-20 G. H. Teichert , S. Das , M. Faghih Shojaei , J. Holber , T. Mueller , L. Hung , V. Gavini , K. Garikipati

Prediction of crystal system from X-ray diffraction (XRD) spectra is a critical task in materials science, particularly for perovskite materials which are known for their diverse applications in photovoltaics, optoelectronics, and…

The important peaks related to the physical properties of a lithium ion rechargeable battery were extracted from the measured X ray diffraction spectrum by a convolutional neural network based on the Attention mechanism. Among the deep…

Machine Learning · Statistics 2020-06-03 Koichi Kano , Takashi Segi , Hiroshi Ozono

Newly designed Li-ion battery cathode materials with high capacity and greater flexibility in chemical composition will be critical for the growing electric vehicles market. Cathode structures with cation disorder were once considered…

Machine learning (ML) techniques have rapidly found applications in many domains of materials chemistry and physics where large data sets are available. Aiming to accelerate the discovery of materials for battery applications, in this work,…

Materials Science · Physics 2019-05-24 Rajendra P. Joshi , Jesse Eickholt , Liling Li , Marco Fornari , Veronica Barone , Juan E. Peralta

The development of new battery materials, particularly novel cathode chemistries, is essential for enabling next generation energy storage technologies. In this work, we employ a multi-fidelity screening protocol combining the Energy-GNoME…

Materials Science · Physics 2026-02-11 Nada Alghamdi , Paolo de Angelis , Pietro Asinari , Eliodoro Chiavazzo

Solid state lithium- and sodium-ion batteries utilize solid ionicly conducting compounds as electrolytes. However, the ionic conductivity of such materials tends to be lower than their liquid counterparts, necessitating research efforts…

Materials Science · Physics 2020-03-12 Yijie Xu , Yun Zong , Kedar Hippalgaonkar

The performance of all-solid-state battery (ASSB) cathodes strongly depends on their microstructure. Optimizing the cathode morphology can therefore enhance effective macroscopic properties such as ionic and electronic conductivity. The…

Computational methods that automatically extract knowledge from data are critical for enabling data-driven materials science. A reliable identification of lattice symmetry is a crucial first step for materials characterization and…

Materials Science · Physics 2018-07-19 A. Ziletti , D. Kumar , M. Scheffler , L. M. Ghiringhelli

We propose a comprehensive set of indicators (including methods to obtain and analyse them) for computational screening of candidate cathode materials for rechargeable Zn-ion aqueous batteries relying on Zn$^{2+}$ intercalation processes.…

Materials Science · Physics 2023-04-18 Sriram Anand , Caio Miranda Miliante , Storm Gourley , Brian D. Adams , Drew Higgins , Oleg Rubel

Due to the subtle balance of intermolecular interactions that govern structure-property relations, predicting the stability of crystal structures formed from molecular building blocks is a highly non-trivial scientific problem. A…

Chemical Physics · Physics 2022-12-26 Rose K. Cersonsky , Maria Pakhnova , Edgar A. Engel , Michele Ceriotti

The identification of materials with exceptional properties is an essential objective to enable technological progress. We propose the application of \textit{Quality-Diversity} algorithms to the field of crystal structure prediction. The…

Materials Science · Physics 2024-03-07 Marta Wolinska , Aron Walsh , Antoine Cully

Challenges associated with in-service mechanical degradation of Li-ion battery cathodes has prompted a transition from polycrystalline to single crystal cathode materials. Whilst for single crystal materials, dislocation-assisted crack…

Materials Science · Physics 2023-08-15 Siyang Wang , Zonghao Shen , Aigerim Omirkhan , Oriol Gavalda-Diaz , Mary P. Ryan , Finn Giuliani

Atomic-level modeling performed at large scales enables the investigation of mesoscale materials properties with atom-by-atom resolution. The spatial complexity of such cross-scale simulations renders them unsuitable for simple human visual…

Materials Science · Physics 2022-04-05 Heejung Chung , Rodrigo Freitas , Gowoon Cheon , Evan J. Reed

Microstructure often dictates materials performance, yet it is rarely treated as an explicit design variable because microstructure is hard to quantify, predict, and optimize. Here, we introduce an image centric, closed-loop framework that…

Materials Science · Physics 2025-05-14 Geunho Choi , Changhwan Lee , Jieun Kim , Insoo Ye , Keeyoung Jung , Inchul Park

Machine learning models are susceptible to being misled by biases in training data that emphasize incidental correlations over the intended learning task. In this study, we demonstrate the impact of data bias on the performance of a machine…

Materials Science · Physics 2024-12-11 Ali Davariashtiyani , Busheng Wang , Samad Hajinazar , Eva Zurek , Sara Kadkhodaei

Machine learning has revolutionized many fields, including materials science. However, predicting properties of crystalline materials using machine learning faces challenges in input encoding, output versatility, and interpretability. We…

Materials Science · Physics 2025-05-22 Haosheng Xu , Dongheng Qian , Jing Wang

We report the development of a combined machine-learning and high-throughput density functional theory (DFT) framework to accelerate the search for new ferroelectric materials. The framework can predict potential ferroelectric compounds…

As the use of Lithium-ion batteries continues to grow, it becomes increasingly important to be able to predict their remaining useful life. This work aims to compare the relative performance of different machine learning algorithms, both…

Machine Learning · Computer Science 2023-12-12 Hudson Hilal , Pramit Saha

Li$_xTM$O$_2$ (TM={Ni, Co, Mn}) are promising cathodes for Li-ion batteries, whose electrochemical cycling performance is strongly governed by crystal structure and phase stability as a function of Li content at the atomistic scale. Here,…