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We investigate the control of electronic energy transfer in molecular dimers through the preparation of specific vibrational coherences prior to electronic excitation, and its observation by nonlinear wave-packet interferometry.…

Quantum Physics · Physics 2015-05-14 Jason D. Biggs , Jeffrey A. Cina

Manipulation of quantum systems is the basis for many promising quantum technologies. However, how quantum mechanical principles can be used to manipulate the dynamics of quantum dissipative systems remains unanswered because of strong…

Mesoscale and Nanoscale Physics · Physics 2019-02-27 Nguyen Thanh Phuc , Akihito Ishizaki

We present a study of the prospects for coherence preservation in solid-state spin qubits using dynamical decoupling protocols. Recent experiments have provided the first demonstrations of multipulse dynamical decoupling sequences in this…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 M. J. Biercuk , H. Bluhm

The Van Allen radiation belts contain relativistic electrons trapped by Earth's magnetic field, posing serious risks to spacecraft. Chorus waves are known to accelerate these electrons via resonant interactions, but these interactions are…

Space Physics · Physics 2025-07-28 Xin Tao , Zeyu An , Fulvio Zonca , Liu Chen , Jacob Bortnik

We analyze the attosecond electron dynamics in hydrogen molecular ion driven by an external intense laser field using ab-initio numerical simulations of the corresponding time-dependent Schr{\"{o}}dinger equation and Bohmian trajectories.…

Chemical Physics · Physics 2015-05-20 Norio Takemoto , Andreas Becker

Recently it was demonstrated that long-lived quantum coherence exists during excitation energy transport in photosynthesis. It is a valid question up to which length, time and mass scales quantum coherence may extend, how to one may detect…

Quantum Physics · Physics 2015-05-19 A. Vaziri , M. B. Plenio

Exact calculations of collective excitations and charge/spin (pseudo)gaps in an ensemble of bipartite and nonbipartite clusters yield level crossing degeneracies, spin-charge separation, condensation and recombination of electron charge and…

Strongly Correlated Electrons · Physics 2009-11-13 A. N. Kocharian , G. W. Fernando , K. Palandage , J. W. Davenport

Coherent electrons coupled to the quantized electromagnetic field undergo decoherence which can be viewed as due either to fluctuations of the Aharonov-Bohm phase or to photon emission. When the electromagnetic field is in a squeezed vacuum…

Quantum Physics · Physics 2009-01-09 Jen-Tsung Hsiang , L. H. Ford

We discuss the various manifestations of quantum decoherence in the forms of dephasing, entanglement with the environment, and revelation of "which-path" information. As a specific example, we consider an electron interference experiment.…

Quantum Physics · Physics 2015-05-13 Jen-Tsung Hsiang , L. H. Ford

Molecular magnets are attractive as spin qubits due to their chemical tunability, addressability through electron-spin resonance techniques, and long coherence times. Clock transitions (CTs), for which the system is immune to the effect of…

Neutrino-nucleus scattering $\nu A\to \nu A$, in which the nucleus conserves its integrity, is considered. We show that elastic interactions keeping the nucleus in the same quantum state lead to a quadratic enhancement of the corresponding…

High Energy Physics - Phenomenology · Physics 2018-09-26 Vadim A. Bednyakov , Dmitry V. Naumov

We study the dynamics of an electron spin in a graphene quantum dot, which is interacting with a bath of less than ten nuclear spins via the anisotropic hyperfine interaction. Due to substantial progress in the fabrication of graphene…

Mesoscale and Nanoscale Physics · Physics 2014-01-09 Moritz Fuchs , John Schliemann , Björn Trauzettel

The photochemistry of a molecular ensemble coupled to a resonance cavity and triggered by a femtosecond laser pulse is investigated from a real-time, quantum dynamics perspective with the multi-configuration time-dependent Hartree method.…

Chemical Physics · Physics 2018-06-20 Oriol Vendrell

Ultrafast photoinduced dynamics of electronic excitation in molecular dimers is drastically affected by the dynamic reorganization of inter- and intra- molecular nuclear configuration modeled by a quantized nuclear degree of freedom [Cina…

Mathematical Physics · Physics 2009-11-10 Dmitri S. Kilin , Yuri V. Pereversev , Oleg V. Prezhdo

Nuclear orbiting resonances have been revealed at the sub-barrier energies as an atomic phenomenon by means of x-ray spectroscopy experiments. This interpretation is supported by several phenomenological models and theoretical estimates of…

We review theoretical foundations and some recent progress related to the quest of controlling the motion of charge carriers with intense laser pulses and optical waveforms. The tools and techniques of attosecond science enable detailed…

Mesoscale and Nanoscale Physics · Physics 2017-03-10 Vladislav S. Yakovlev , Stanislav Yu. Kruchinin , Tim Paasch-Colberg , Mark I. Stockman , Ferenc Krausz

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

We have theoretically analyzed coherent nuclear-spin dynamics induced by electron transport through a quantum-dot spin valve. The hyperfine interaction between electron and nuclear spins in a quantum dot allows for the transfer of angular…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Stefano Chesi , W. A. Coish

In quantum metrology and quantum simulation, a coherent non-classical state must be manipulated before unwanted interactions with the environment lead to decoherence. In atom interferometry, the non-classical state is a spatial…

Atomic Physics · Physics 2024-08-19 Cristian D. Panda , Matthew Tao , James Egelhoff , Miguel Ceja , Victoria Xu , Holger Müller

We develop a density matrix formalism to describe coupled electron-nuclear dynamics. To this end we introduce an effective Hamiltonian formalism that describes electronic transitions and small (quantum) nuclear fluctuations along a…

Chemical Physics · Physics 2020-09-07 Eugene Stolyarov , Alexander White , Dmitry Mozyrsky