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Related papers: Ionization potential and electron affinity of supe…

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The successive ionization potentials (IPs) and electron affinities (EAs) for superheavy elements with $111 \leq Z \leq 114$, namely, Rg, Cn, Nh, and Fl are reexamined using the relativistic Fock-space coupled-cluster method with…

We present high accuracy relativistic coupled cluster calculations of the first and second ionisation potentials and the electron affinity of the heaviest element in the Periodic Table, Og. The results were extrapolated to the basis set…

Atomic Physics · Physics 2023-04-28 Yangyang Guo , Lukáš Félix Pašteka , Ephraim Eliav , Anastasia Borschevsky

The electron affinity (EA) of superheavy element Og is calculated by the use of the relativistic Fock-space coupled cluster (FSCC) and configuration interaction methods. The FSCC cluster operator expansion included single, double, and…

Theoretical calculations based on the Dirac--Coulomb--Breit relativistic coupled cluster method have been carried out for the electron affinities and ionization potentials of the superheavy element nihonium (Nh) and its lighter homologues…

Atomic Physics · Physics 2022-07-13 Yangyang Guo , Anastasia Borschevsky , Ephraim Eliav , Lukáš F. Pašteka

We use recently developed method of accurate atomic calculations which combines linearized single-double coupled cluster method with the configuration interaction technique to calculate ionisation potentials, excitation energies, static…

Atomic Physics · Physics 2017-02-01 V. A. Dzuba , V. V. Flambaum

Quantum electrodynamics coupled-cluster (QED-CC) theory is used to model vacuum-field-induced changes to ground-state properties of a series of sodium halide compounds (NaX, X = F, Cl, Br, I) strongly coupled to an optical cavity.…

Chemical Physics · Physics 2021-03-17 A. Eugene DePrince

We combine the electron attachment (EA) and ionization potential (IP) equation-of-motion (EOM) coupled-cluster (CC) approaches with the CC($P$;$Q$) formalism. The resulting methodologies are used to describe the electronic states of several…

Chemical Physics · Physics 2025-09-19 Karthik Gururangan , Stephen H. Yuwono , A. Eugene DePrince , Piotr Piecuch

The calculations of the first and the second ionization potentials of lawrencium and lutetium and the electron affinity of lawrencium are performed within the relativistic coupled cluster framework. These results are corrected by including…

In this paper, we have studied electron correlation and Gaunt interaction effects in ionization potentials (IPs) and hyperfine constants A of 2p$^2P_{1/2}$ and 2p$^2P_{3/2}$ states along with the fine structure splitting (FSS) between them…

Atomic Physics · Physics 2011-11-23 Narendra Nath Dutta , Sonjoy Majumder

We report the first results of ab initio relativistic correlation calculation of the effective electric field on the electron, E_eff, in the ground state of the HI$^+$ cation. This value is required for interpretation of the suggested…

Atomic Physics · Physics 2013-05-29 T. A. Isaev , N. S. Mosyagin , A. N. Petrov , A. V. Titov

Fully relativistic approach to evaluate the correlation effects in highly charged ions is presented. The interelectronic-interaction contributions of first and second orders in $1/Z$ are treated rigorously within the framework of…

Atomic Physics · Physics 2019-12-18 Y. S. Kozhedub , A. V. Malyshev , D. A. Glazov , V. M. Shabaev , I. I. Tupitsyn

We present relativistic many-body calculations of total electron binding energy of neutral atoms up to element $Z=120$. Binding energy for ions may be found by subtracting known ionization potentials. Accuracy of the results for $17<Z…

Atomic Physics · Physics 2025-03-25 V. A. Dzuba , V. V. Flambaum , A. V. Afanasjev

Within the Hubbard model, the ionization energy and electron affinity of the icosahedral C60 fullerene are calculated in the static fluctuation approximation. A graphical representation of the chemical potential equation is first obtained.…

Strongly Correlated Electrons · Physics 2026-01-22 Gennadiy Ivanovich Mironov

A systematic QED treatment of electron correlation is presented for ions along the lithium isoelectronic sequence. We start with the zeroth-order approximation that accounts for a part of the electron-electron interaction by a local model…

Atomic Physics · Physics 2009-11-13 V. A. Yerokhin , A. N. Artemyev , V. M. Shabaev

The article considers the successful implementation of relativistic equation-of-motion coupled cluster method for the electron attachment problem (EA-EOMCC) at the level of single- and double- excitation approximation. The implemented…

Atomic Physics · Physics 2016-01-06 Himadri Pathak , Sudip Sasmal , Malaya K. Nayak , Nayana Vaval , Sourav Pal

This study investigates the interplay between relativistic effects and electron correlation effects on the first ionization energies of heavy atoms (Au through Rn, Z = 79-86). We perform two complementary analyses: (1) comparing…

Atomic Physics · Physics 2026-02-06 Mohamed Kahil , Fatima Fakih , Nabil Joudieh , Nidal Chamoun

Core-polarization interactions are investigated in low-energy electron elastic scattering from the atoms In,Sn,Eu,Au and At through the calculation of their electron affinities. The complex angular momentum method wherein is embedded the…

Atomic Physics · Physics 2015-10-07 Z. Felfli , A. Z. Msezane

The ionization potential (IP) is an important parameter providing essential insights into the reactivity of chemical systems. IPs are also crucial for designing, optimizing, and understanding the functionality of modern technological…

Chemical Physics · Physics 2024-02-12 Marta Gałyńska , Katharina Boguslawski

The quantum electrodynamics (QED) corrections are directly incorporated into the most accurate treatment of the correlation corrections for ions with complex electronic structure of interest to metrology and tests of fundamental physics. We…

Atomic Physics · Physics 2016-12-21 I. I. Tupitsyn , M. G. Kozlov , M. S. Safronova , V. M. Shabaev , V. A. Dzuba

Relativistic calculations of the electronic structure of the superheavy element of the eighth period $-$ eka-francium ($Z=119$) and its homologues, which form the group of alkali metals, are performed in the framework of the…

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