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The hierarchical equations of motion (HEOM) for a generalized quantum dissipative system is rigorously constructed in the frameworks of two different stochastic dynamical descriptions, i.e., the non-Markovian quantum state diffusion…

Quantum Physics · Physics 2018-07-18 Wei Wu

The hierarchical equations of motion (HEOM) provide a numerically exact approach for simulating the dynamics of open quantum systems coupled to a harmonic bath. However, its applicability has traditionally been limited to specific spectral…

Quantum Physics · Physics 2023-08-07 Meng Xu , Joachim Ankerhold

We derive an extended version of the hierarchical equations of motion (HEOM) to compute output physical properties of a bosonic environment, which is allowed to be initially prepared at an earlier time in a non-Gaussian input state and then…

Quantum Physics · Physics 2025-08-15 Mauro Cirio , Pengfei Liang , Neill Lambert

We present a theoretical framework to investigate quantum thermodynamic processes under non-Markovian system-bath interactions on the basis of the hierarchical equations of motion (HEOM) approach, which is convenient to carry out…

Quantum Physics · Physics 2019-05-01 Akihito Kato , Yoshitaka Tanimura

The Hierarchical Equations of Motion (HEOM) method has become one of the cornerstones in the simulation of open quantum systems and their dynamics. It is commonly referred to as a non-perturbative method. Yet, there are certain instances,…

Quantum Physics · Physics 2024-08-13 Malte Krug , Jürgen Stockburger

The hierarchical equations of motion (HEOM) theory is one of the standard methods to rigorously describe open quantum dynamics coupled to harmonic environments. Such a model is used to capture non-Markovian and non-perturbative effects of…

Chemical Physics · Physics 2020-06-02 Tatsushi Ikeda , Gregory D. Scholes

A nonperturbative quantum impurity solver is proposed based on a formally exact hierarchical equations of motion (HEOM) formalism for open quantum systems. It leads to quantitatively accurate evaluation of physical properties of strongly…

Strongly Correlated Electrons · Physics 2014-08-04 Dong Hou , Rulin Wang , Xiao Zheng , NingHua Tong , JianHua Wei , YiJing Yan

An open quantum system refers to a system that is further coupled to a bath system consisting of surrounding radiation fields, atoms, molecules, or proteins. The bath system is typically modeled by an infinite number of harmonic…

Chemical Physics · Physics 2020-07-10 Yoshitaka Tanimura

The hierarchical equations of motion technique has found widespread success as a tool to generate the numerically exact dynamics of non-Markovian open quantum systems. However, its application to low temperature environments remains a…

Chemical Physics · Physics 2013-10-15 Jeremy M. Moix , Jianshu Cao

The study of open system quantum dynamics has been transformed by the hierarchical equations of motion (HEOM) method, which gives the exact dynamics for a system coupled to a harmonic bath at arbitrary temperature and system-bath coupling…

Chemical Physics · Physics 2022-08-17 Thomas P Fay

The hierarchical equations of motion (HEOM) provide a numerically exact approach for computing the reduced dynamics of a quantum system linearly coupled to a bath. We have found that HEOM contains temperature-dependent instabilities that…

Chemical Physics · Physics 2019-05-13 Ian S. Dunn , Roel Tempelaar , David R. Reichman

The hierarchical equations of motion (HEOM) approach is an accurate method to simulate open system quantum dynamics, which allows for systematic convergence to numerically exact results. To represent the effects of the bath, the reservoir…

Strongly Correlated Electrons · Physics 2023-05-31 Xiaohan Dan , Meng Xu , J. T. Stockburger , J. Ankerhold , Qiang Shi

The time evolution in open quantum systems, such as a molecular aggregate in contact with a thermal bath, still poses a complex and challenging problem. The influence of the thermal noise can be treated using a plethora of schemes, several…

Chemical Physics · Physics 2019-07-24 Hasan Rahman , Ulrich Kleinekathoefer

The hierarchical equations of motion (HEOM) method is a numerically exact open quantum system dynamics approach. The method is rooted in an exponential expansion of the bath correlation function, which in essence strategically reshapes a…

Chemical Physics · Physics 2023-06-14 Yaling Ke

The Hierarchical equations of motion (HEOM) method is an important non-perturbative technique, allowing numerically exact treatment of open quantum systems with strong coupling and non-Markovian memory. However, its encoding of bath memory…

Quantum Physics · Physics 2026-03-25 Po-Rong Lai , Jhen-Dong Lin , Yi-Te Huang , Po-Chen Kuo , Neill Lambert , Yueh-Nan Chen

For a system strongly coupled to a heat bath, the quantum coherence of the system and the heat bath plays an important role in the system dynamics. This is particularly true in the case of non-Markovian noise. We rigorously investigate the…

Statistical Mechanics · Physics 2015-02-16 Yoshitaka Tanimura

Studies of quantum thermal effects on molecular excitation dynamics have often relied on oversimplified models, such as energy eigenstates or low-dimensional potentials, which fail to capture the complexity of real chemical systems. In…

Chemical Physics · Physics 2025-12-30 Yankai Zhang , Yoshitaka Tanimura , So Hirata

Over the last two decades, the hierarchical equations of motion (HEOM) of Tanimura and Kubo have become the equation of motion-based tool for numerically exact calculations of system-bath problems. The HEOM is today generalized to many…

Quantum Physics · Physics 2023-05-15 Robert Fuchs , Marten Richter

We rigorously investigate the quantum non-Markovian dissipative dynamics of a system coupled to a harmonic oscillator bath by deriving hierarchical Schrodinger equations of motion (HSEOM) and studying their dynamics. The HSEOM are the…

Quantum Physics · Physics 2018-07-11 Kiyoto Nakamura , Yoshitaka Tanimura

The hierarchical equations of motion (HEOM), derived from the exact Feynman-Vernon path integral, is one of the most powerful numerical methods to simulate the dynamics of open quantum systems that are embedded in thermal environments.…

Quantum Physics · Physics 2025-10-07 Meng Xu , Yaming Yan , Qiang Shi , J. Ankerhold , J. T. Stockburger
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