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Black Phosphorus (BP) is unique among layered materials owing to its homonuclear lattice and strong structural anisotropy. While recent investigations on few layers BP have extensively explored the in-plane (a,c) anisotropy, much less…

The temperature dependence of the band gap is crucial to a semiconductor. Bulk black phosphorus (BP) is known to exhibit an anomalous behavior. Through optical spectroscopy, here we show that the temperature effect on BP band gap gradually…

Lattice-matched GaP layers without extended defects can be grown on Si(001) substrate via a two-step growth procedure, consisting of low-temperature nucleation followed by high-temperature overgrowth. A transient reflectivity experiment on…

Uncooled Terahertz (THz) photodetectors (PDs) showing fast (ps) response and high sensitivity (noise equivalent power (NEP) < $nWHz^{-1/2}$) over a broad (0.5THz-10THz) frequency range are needed for applications in high-resolution…

The interaction between light and matter in condensed matter excitations and electromagnetic resonators serves as a rich playground for fundamental research and lies at the core of photonic and quantum technologies. Herein, we present…

In this work we study phonon-phonon coupling in bismuth vanadate (BiVO4), known for its second-order transition involving a variety of coupling mechanisms. Using Raman spectroscopy as a probe, we identify two optical coupled phonon modes of…

Materials Science · Physics 2023-06-09 Christina Hill , Georgy Gordeev , Mael Guennou

The possibility of hybridizing collective electronic motion with mid-infrared (mid-IR) light to form surface polaritons has made van der Waals layered materials a versatile platform for extreme light confinement and tailored nanophotonics.…

Terahertz and far-infrared electric and magnetic responses of hexagonal piezomagnetic YMnO3 single crystals are investigated. Antiferromagnetic resonance is observed in the spectra of magnetic permeability mu_a [H(omega) oriented within the…

Materials Science · Physics 2012-02-13 C. Kadlec , V. Goian , K. Z. Rushchanskii , P. Kuzel , M. Lezaic , K. Kohn , R. V. Pisarev , S. Kamba

Phonon polaritons (PhPs), the collective phonon oscillations with hybridized electromagnetic fields, concentrate optical fields in the mid-infrared frequency range that matches the vibrational modes of molecules. The utilization of PhPs…

Optics · Physics 2020-06-24 Haomin Wang , Eli Janzen , Le Wang , James H. Edgar , Xiaoji G. Xu

The achievable instrument sensitivity is a critical parameter for the continued development of THz applications. Techniques such as Cavity-Enhanced Techniques and Cavity Ring Down Spectroscopy have not yet been employed at THz frequency due…

Carrier and phonon dynamics in a multilayer WSe2 film are captured by extreme ultraviolet (XUV) transient absorption (TA) spectroscopy at the W N6,7, W O2,3, and Se M4,5 edges (30-60 eV). After the broadband optical pump pulse, the XUV…

Materials Science · Physics 2023-03-06 Juwon Oh , Hung-Tzu Chang , Christopher T. Chen , Shaul Aloni , Adam Schwartzberg , Stephen R. Leone

We discuss terahertz pump-probe experiments in hBN from the perspective of Floquet optical materials and photonic time crystals. Anisotropic nature of this material results in a large separation of frequencies of in-plane and out-of-plane…

Recently developed terahertz (THz) two-dimensional coherent spectroscopy (2DCS) is a powerful technique to obtain materials information in a fashion qualitatively different from other spectroscopies. Here, we utilized THz 2DCS to…

Among its many outstanding properties, graphene supports terahertz surface plasma waves -- sub-wavelength charge density oscillations connected with electromagnetic fields that are tightly localized near the surface[1,2]. When these waves…

Atomic layers of Black Phosphorus (BP) present unique opto-electronic properties dominated by a direct tunable bandgap in a wide spectral range from visible to mid-infrared. In this work, we investigate the infrared photoluminescence of BP…

Mesoscale and Nanoscale Physics · Physics 2021-01-13 Etienne Carré , Lorenzo Sponza , Alain Lusson , Ingrid Stenger , Etienne Gaufrès , Annick Loiseau , Julien Barjon

Sub-wavelength graphene structures support localized plasmonic resonances in the terahertz and mid-infrared spectral regimes. The strong field confinement at the resonant frequency is predicted to significantly enhance the light-graphene…

To control structure-function relationships in solids with light, we must harness the shape of the potential energy surface, as expressed in anharmonic coupling coefficients. We use two-dimensional terahertz (THz) spectroscopy to identify…

Here we perform a series of time-resolved experiments where a 100 fs pump pulse is tuned between 528 nm and 555 nm, across the second indirect gap of intrinsic silicon at ~540 nm which involves electrons in a higher-lying conduction band…

Optics · Physics 2017-01-24 Fabio Novelli , Jeffrey A Davis

Ultrafast charge transport in strongly biased semiconductors is at the heart of highspeed electronics, electro-optics, and fundamental solid-state physics. Intense light pulses in the terahertz (THz) spectral range have opened fascinating…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 O. Schubert , M. Hohenleutner , F. Langer , B. Urbanek , C. Lange , U. Huttner , D. Golde , T. Meier , M. Kira , S. W. Koch , R. Huber

As a fundamental physical quantity of thermal phonons, temporal coherence participates in a broad range of thermal and phononic processes, while a clear methodology for the measurement of phonon coherence is still lacking. In this Lettter,…

Applied Physics · Physics 2023-05-03 Zhongwei Zhang , Yangyu Guo , Marc Bescond , Masahiro Nomura , Sebastian Volz , Jie Chen
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