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Related papers: Enhanced second-harmonic generation from WS$_2$/Re…

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Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…

We study the effects of crystal anisotropy on optical phonon resonances in the second harmonic generation (SHG) from silicon carbide (SiC) in its Reststrahl region. By comparing experiments and simulations for isotropic 3C-SiC and…

Materials Science · Physics 2016-11-02 Alexander Paarmann , Ilya Razdolski , Sandy Gewinner , Wieland Schoellkopf , Martin Wolf

Second-harmonic generation (SHG) is a second-order nonlinear optical process that is not allowed in media with inversion sym-metry. However, due to the broken symmetry at the surface, surface SHG still occurs, but is generally small. We…

We have developed a numerical method for calculating the second harmonic generation (SHG) generated by an anisotropic material whose optical properties present an arbitrary modulation in one dimension. The method is based on the Berreman…

Optics · Physics 2023-05-31 J. Ortega , C. L. Folcia , J. Etxebarria

The in-plane anisotropic properties of two-dimensional (2D) group IV monochalcogenides provide an additional degree of freedom which can be used in future optoelectronic devices. Here, it is shown that the third harmonic generation (THG)…

Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…

Optics · Physics 2020-01-10 Xuexue Guo , Xingjie Ni

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

Imaging antiferromagnetic 180{\deg} domains with actively controlled visibility is vital for both fundamental science and sophisticated applications. While optical second-harmonic generation (SHG) is a well-known technique for…

Strongly Correlated Electrons · Physics 2024-09-02 Ziqian Wang , Meng Wang , Jannis Lehmann , Yuki Shiomi , Taka-hisa Arima , Naoto Nagaosa , Yoshinori Tokura , Naoki Ogawa

Two-dimensional (2D) tin(II) sulfide (SnS) crystals belong to a class of orthorhombic semiconducting materials that are lately attracting significant interest, given their remarkable properties, such as in-plane anisotropic optical and…

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

Understanding and controlling nonlinear processes is crucial for engineering light-matter interaction and generating non-classical light. A significant challenge in ultra-thin nonlinear materials is the marked diminution of the nonlinear…

Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…

Optics · Physics 2013-09-17 B. U. Felderhof , G. Marowsky

1T-TaS$_2$ is a layered charge density wave (CDW) crystal exhibiting sharp phase transitions and associated resistance changes. These resistance steps could be exploited for information storage, underscoring the importance of controlling…

While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $\sigma^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is…

The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…

Optical nonlinearity, especially the second harmonic generation (SHG), is generally weak in materials but has the potential to be applied in high-speed optical computers and energy-efficient artificial intelligence systems. In order to…

Strongly Correlated Electrons · Physics 2024-12-05 Junyi Shan

Twisting two dissimilar monolayer semiconductors induces structural chirality that remains largely elusive in linear optics but becomes remarkably pronounced in the nonlinear regime. Here we demonstrate that MoS2/WSe2 heterobilayers exhibit…

The transition metal monopnictide family of Weyl semimetals recently has been shown to exhibit anomalously strong second-order optical nonlinearity, which is theoretically attributed to a highly asymmetric polarization distribution induced…

Strongly Correlated Electrons · Physics 2022-07-21 Chen Li , Xiang Li , T. Deshpande , Xinwei Li , N. Nair , J. G. Analytis , D. M. Silevitch , T. F. Rosenbaum , D. Hsieh