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High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…
The spectra produced by high-harmonic generation (HHG) typically exhibit well-defined peaks at odd integers times the laser frequency. However, in recent investigations of HHG from correlated materials, spectra exhibit signals at noninteger…
High-order harmonic generation (HHG) from crystals offers a new source of coherent extreme ultraviolet (XUV) attosecond radiation.
High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…
Fourth-generation storage-ring light sources have achieved transverse emittances approaching the diffraction limit at x-ray wavelengths, while their longitudinal coherence remains limited. Existing laser-modulation schemes can induce strong…
High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…
We demonstrate a new high-order harmonic generation mechanism reaching the `water window' spectral region in experiments with multi-terawatt femtosecond lasers irradiating gas jets. A few hundred harmonic orders are resolved, giving uJ/sr…
Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…
Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber,…
Photon channel perspective on high harmonic generation (HHG) is proposed by quantizing both the driving laser and high harmonics. It is shown that the HHG yield can be expressed as a sum of the contribution of all the photon channels. From…
High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…
High-harmonic spectroscopy in solids gives insight into the inner workings of solids, such as reconstructing band structures or probing the topological phase of materials. High-harmonic generation (HHG) is a highly non-linear phenomena and…
The neutral hydrogen 21cm line is potentially a very powerful probe of the observable universe, and a number of on-going experiments are trying to detect it at cosmological distances. However, the presence of strong foreground radiations…
High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…
Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…
The selection rules of high harmonic generation (HHG) are investigated using three-dimensional time-dependent density functional theory (TDDFT). From the harmonic spectra obtained with various real molecules and different forms of laser…
Time-resolved soft-x-ray-diffraction experiments give access to microscopic processes in a broad range of solid-state materials by probing ultrafast dynamics of ordering phenomena. While laboratory-based high-harmonic generation (HHG) light…
High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…
The recent progress in the quantum optical formulation of the process of high harmonic generation has reached a point where the successful semi-classical model shows its limitations. So far the light source which drives the process was…
High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…