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An implementation of the Hartree-Fock (HF) method capable of robust convergence for well-behaved arbitrary central potentials is presented. The Hartree-Fock equations are converted to a generalized eigenvalue problem by employing a B-spline…

Atomic Physics · Physics 2021-08-13 D. T. Waide , D. G. Green , G. F. Gribakin

Electron transfer processes are ubiquitous in chemistry and of great importance in many systems of biological and commercial interest. The ab-initio description of these processes remains a challenge in theoretical chemistry, partly due to…

Chemical Physics · Physics 2018-08-14 Kristopher T. Jensen , Raz L. Benson , Salvatore Cardamone , Alex J. W. Thom

An efficient excited state method, named xCDFCI, in the configuration interaction framework, is proposed. xCDFCI extends the unconstrained nonconvex optimization problem in coordinate descent full configuration interaction~(CDFCI) to a…

Chemical Physics · Physics 2023-08-23 Zhe Wang , Zhiyuan Zhang , Jianfeng Lu , Yingzhou Li

We calculate the ground state phase diagram of the homogeneous electron gas in two dimensions within the Hartree-Fock approximation. At high density, we find stable solutions, where the electronic charge and spin density form an…

Strongly Correlated Electrons · Physics 2014-03-04 B. Bernu , F. Delyon , M. Holzmann , L. Baguet

The (2+1)-dimensional generalized massless Thirring model with 4-component Fermi-fields is investigated by the Hartree-Fock method. The Lagrangian of this model is constructed from two different four-fermion structures. One of them takes…

High Energy Physics - Theory · Physics 2022-10-19 T. G. Khunjua , K. G. Klimenko , R. N. Zhokhov

Two of the most widely used electronic structure theory methods, namely Hartree-Fock and Kohn-Sham density functional theory, both requires the iterative solution of a set of Schr\"odinger-like equations. The speed of convergence of such…

Chemical Physics · Physics 2024-06-06 S. Hazra , U. Patil , S. Sanvito

We derive the photoionisation cross section in dipole approximation for many-electron atoms and ions for neutron star magnetic field strengths in the range of 10^7 to 10^9 T. Both bound and continuum states are treated in adiabatic…

Atomic Physics · Physics 2013-08-08 Thorsten Kersting , Damir Zajec , Peter Diemand , Günter Wunner

This paper deals with the solution of the spherically symmetric time-dependent Hartree-Fock approximation applied to nuclear giant monopole resonances in the small amplitude regime. The problem is spatially unbounded as the resonance state…

Nuclear Theory · Physics 2015-06-16 C. I. Pardi , P. D. Stevenson , K. Xu

We study the electromagnetic responses of $^4$He within the framework of the self-consistent continuum random phase approximation theory. In this approach the ground state properties are described by a Hartree-Fock calculation. The single…

Nuclear Theory · Physics 2015-05-30 V. De Donno , M. Anguiano , G. Co' , A. M. Lallena

We present and compare several many-body methods as applied to two-dimensional quantum dots with circular symmetry. We calculate the approximate ground state energy using a harmonic oscillator basis optimized by Hartree-Fock (HF) theory and…

We present a fully numerical framework for the optimization of molecule-specific quantum chemical basis functions within the quantics tensor train format using a finite-difference scheme. The optimization is driven by solving the…

Chemical Physics · Physics 2025-06-12 Paul Haubenwallner , Matthias Heller

While Hartree-Fock theory is well established as a fundamental approximation for interacting fermions, it has been unclear how to describe corrections to it due to many-body correlations. In this paper we start from the Hartree-Fock state…

Mathematical Physics · Physics 2020-04-13 Niels Benedikter , Phan Thành Nam , Marcello Porta , Benjamin Schlein , Robert Seiringer

The configuration interaction relativistic Hartree-Fock (CI-RHF) model is developed in this work. Compared to the conventional configuration interaction shell model (CISM), the CI-RHF model can be applied to study the structural properties…

Nuclear Theory · Physics 2025-04-14 Jia Liu , Yi Fei Niu , Wen Hui Long

The possible compatibility of density matrices for single-party subsystems is described by linear constraints on their respective spectra. Whenever some of those quantum marginal constraints are saturated, the total quantum state has a…

Quantum Physics · Physics 2017-11-09 Christian Schilling , Carlos L. Benavides-Riveros , Péter Vrana

The time-dependent Hartree and Hartree-Fock equations provide effective mean-field descriptions for the dynamics of large fermionic systems and play a fundamental role in many areas of physics. In this work, we rigorously derive the…

Mathematical Physics · Physics 2025-07-17 Duc Viet Hoang , David Mitrouskas , Peter Pickl

In the limit of infinite spatial dimensions a thermodynamically consistent theory, which is valid for arbitrary value of the Coulombic interaction ($U<\infty$), is built for the Hubbard model when the total auxiliary single-site problem…

Strongly Correlated Electrons · Physics 2014-02-17 A. M. Shvaika

The hybridization between light and matter is fundamental for achieving cavity-induced control over quantum materials, necessitating accurate ab initio methods for their analysis. Among these, the quantum electrodynamics Hartree-Fock…

Quantum Physics · Physics 2024-11-25 Ilia Mazin , Yu Zhang

Lattice field theory methods, usually associated with non-perturbative studies of quantum chromodynamics, are becoming increasingly common in the calculation of ground-state and thermal properties of strongly interacting non-relativistic…

Statistical Mechanics · Physics 2013-09-18 Joaquín E. Drut , Amy N. Nicholson

A microscopic mean-field description of heavy ions fusion is performed in the framework of the Time-Dependent Hartree-Fock (TDHF) theory using a Skyrme interaction with the SLy4d parametrization. A good agreement with experiments is…

Nuclear Theory · Physics 2008-03-11 Cédric Simenel , Benoît Avez

We show that the Hartree-Fock (HF) results cannot be reproduced within the framework of Kohn-Sham (KS) theory because the single-particle densities of finite systems obtained within the HF calculations are not $v$-representable, i.e., do…

Other Condensed Matter · Physics 2009-11-10 M. Ya. Amusia , A. Z. Msezane , V. R. Shaginyan , D. Sokolovski