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Achieving high energy resolution in spin systems is important for fundamental physics research and precision measurements, with alkali-noble-gas comagnetometers being among the best available sensors. We found a new relaxation mechanism in…

Atomic Physics · Physics 2023-02-22 Kai Wei , Tian Zhao , Xiujie Fang , Zitong Xu , Chang Liu , Qian Cao , Arne Wickenbrock , Yanhui Hu , Wei Ji , Dmitry Budker

We present a general method to realize resonant coupling between spins even though their energies are of different scales. Applying the method to the electron and nuclear spin systems such as a nitrogen-vacancy (NV) center with its nearby…

Quantum Physics · Physics 2023-11-20 Sichen Xu , Chanying Xie , Zhen-Yu Wang

Nuclear magnetic resonance imaging (MRI) at the atomic scale offers exciting prospects for determining the structure and function of individual molecules and proteins. Quantum defects in diamond have recently emerged as a promising platform…

Quantum Physics · Physics 2022-04-06 K. S. Cujia , K. Herb , J. Zopes , J. M. Abendroth , C. L. Degen

Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a…

Quantum Physics · Physics 2013-09-11 J. H. Shim , B. Nowak , I. Niemeyer , J. Zhang , F. D. Brandao , D. Suter

We investigate in detail, using both analytical and numerical tools, the decoherence of electron spins in quantum dots (QDs) coupled to a bath of nuclear spins in magnetic fields or with various initial bath polarizations, focusing on the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Wenxian Zhang , V. V. Dobrovitski , K. A. Al-Hassanieh , E. Dagotto , B. N. Harmon

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

We consider an electronic spin, such as a nitrogen-vacancy (NV) center in diamond, weakly coupled to a large number (bath) of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase (multiple rotary echo). We…

Mesoscale and Nanoscale Physics · Physics 2015-03-25 V. V. Mkhitaryan , F. Jelezko , V. V. Dobrovitski

The Weakly Interacting Massive Particles (WIMPs) are among the main candidates for the relic dark matter (DM). The idea of the direct DM detection relies on elastic in-dependent (SD) and spin-independent (SI) interaction of WIMPs with…

High Energy Physics - Phenomenology · Physics 2007-05-23 V. A. Bednyakov , F. Simkovic , I. V. Titkova

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

We show that nuclear spin subsystems can be completely controlled via microwave irradiation of resolved anisotropic hyperfine interactions with a nearby electron spin. Such indirect addressing of the nuclear spins via coupling to an…

Quantum Physics · Physics 2009-11-13 Jonathan S. Hodges , Jamie C. Yang , Chandrasekhar Ramanathan , David G. Cory

Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Jinkyung Kim , Kyungju Noh , Yi Chen , Fabio Donati , Andreas J. Heinrich , Christoph Wolf , Yujeong Bae

We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

Quantum Physics · Physics 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

Nuclear spins of dopant atoms in semiconductors are promising candidates as quantum bits, due to the long lifetime of their quantum states. Conventionally, coherent control of nuclear spins is done using ac magnetic fields. Using the…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 Péter Boross , Gábor Széchenyi , András Pályi

The study of hyperfine interactions in optically excited fullerenes has recently acquired importance within the context of nuclear spin entanglement for quantum information technology. We here report a first-principles pseudopotential study…

Quantum Physics · Physics 2015-06-03 Vasileia Filidou , Davide Ceresoli , John J. L. Morton , Feliciano Giustino

Quantum systems inside high-Q cavities offer an excellent testbed for the control of emergent symmetries induced by light and their interplay with quantum matter. Recently several developments in cavity experiments with neutral atoms and…

Quantum Physics · Physics 2026-03-24 Santiago F. Caballero-Benitez

Recent demonstrations of ultracoherent nanomechanical resonators introduce the prospect of new protocols for solid state sensing applications. Here, we propose to use two coupled ultracoherent resonator modes on a Si$_3$N$_4$ membrane for…

Applied Physics · Physics 2020-07-22 J. Košata , O. Zilberberg , Christian L. Degen , R. Chitra , A. Eichler

Nanoscale nuclear magnetic resonance (NMR) signals can be measured through hyperfine interaction to paramagnetic electron sensor spins. A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral…

Nuclear spins interact weakly with their environment. In particular, they are generally insensitive to mechanical vibrations. Here, we successfully demonstrate the coherent coupling of mechanics to a single nuclear spin. This coupling is…

The aim of this review is twofold. First, a general approach is presented allowing for a unified description of dynamics in radiating systems of different nature. Both atomic systems as well as spin assemblies can be treated in the frame of…

Atomic Physics · Physics 2015-06-22 V. I. Yukalov

Steady-state superradiance and superradiant lasing attract significant attentions in the field of optical lattice clocks, but have not been achieved so far due to the technical challenges and atom loss problem. In this article, we propose…

Quantum Physics · Physics 2022-12-06 Qilong Wu , Yuan Zhang , Hao Wu , Shi-Lei Su , Kai-Kai Liu , Mark Oxborrow , Chongxin Shan , Klaus Mølmer