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The pyrochlore spin ice compounds Dy2Ti2O7 and Ho2Ti2O7 are well described by classical Ising models down to very low temperatures. Given the empirical success of this description, the question of the importance of quantum effects in these…

Strongly Correlated Electrons · Physics 2015-10-28 Jeffrey G. Rau , Michel J. P. Gingras

We have studied spin relaxation in the spin ice compound Dy2Ti2O7 through measurements of the a.c. magnetic susceptibility. While the characteristic spin relaxation time is thermally activated at high temperatures, it becomes almost…

Materials Science · Physics 2009-11-10 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , Ari Mizel , P. Schiffer

We report the low temperature magnetic properties of Nd$^{3+}$ pyrochlore $\rm Nd_2ScNbO_7$. Susceptibility and magnetization show an easy-axis moment, and heat capacity reveals a phase transition to long range order at $T_N=371(2)$ mK with…

Strongly Correlated Electrons · Physics 2022-08-11 A. Scheie , M. Sanders , Yiming Qiu , T. R. Prisk , R. J. Cava , C. Broholm

The quantum antiferromagnet on the pyrochlore lattice offers an archetypal frustrated system, which potentially realizes a quantum spin liquid characterized by the absence of standard spontaneous symmetry breaking even at zero temperature,…

Strongly Correlated Electrons · Physics 2023-11-21 Rico Pohle , Youhei Yamaji , Masatoshi Imada

Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2Ti2O7 and Dy2Ti2O7 exemplify this phenomenon, displaying a classical spin liquid state, with…

Strongly Correlated Electrons · Physics 2017-12-11 Mathieu Taillefumier , Owen Benton , Han Yan , L. D. C. Jaubert , Nic Shannon

We report magnetization and ac susceptibility of single crystals of the spin ice compound Dy2Ti2O7. Saturated moments at 1.8 K along the charasteristic axes [100] and [110] agree with the expected values for an effective ferromagnetic…

Strongly Correlated Electrons · Physics 2016-08-31 H. Fukazawa , R. G. Melko , R. Higashinaka , Y. Maeno , M. J. P. Gingras

The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low…

We report magnetization data for several titanium pyrochlore systems measured down to 0.5 K. The measurements, performed on single crystal samples in fields of up to 7 T, have captured the essential elements of the previously reported phase…

Strongly Correlated Electrons · Physics 2014-08-18 O. A. Petrenko , M. R. Lees , G. Balakrishnan

Motivated by recent experimental and theoretical progress on the Er2Ti2O7 pyrochlore XY antiferromagnet, we study the problem of quantum order-by-disorder in pyrochlore XY systems. We consider the most general nearest-neighbor pseudo…

Strongly Correlated Electrons · Physics 2013-11-15 Anson W. C. Wong , Zhihao Hao , Michel J. P. Gingras

We present magnetization and Hall effect measurements on the pyrochlore iridate Nd2Ir2O7. Previous muon spin rotation measurements have shown that the system undergoes an unusual transition at T$_M$ = 110 K into a magnetic phase lacking…

Strongly Correlated Electrons · Physics 2015-06-12 S. M. Disseler , S. R. Giblin , Chetan Dhital , K. C. Lukas , Stephen D. Wilson , M. J. Graf

In this study, I have investigated the magnetic and critical properties of manganese pyrochlore fluoride NaSrMn$_{2}$F$_{7}$, which exhibits a glass transition at T$_\text{f}$$=$2.5 (K) due to charge disorder. A DFT+$U$+SOC framework is…

Strongly Correlated Electrons · Physics 2023-05-09 Mohammad Amirabbasi

We present an experimental study of the pyrochlore coumpound Nd2Zr2O7 by means of neutron scattering and magnetization measurements down to 90 mK. The Nd$^{3+}$ magnetic moments exhibit a strong local $\langle$111$\rangle$ Ising anisotropy…

Strongly Correlated Electrons · Physics 2016-01-05 E. Lhotel , S. Petit , S. Guitteny , O. Florea , M. Ciomaga Hatnean , C. Colin , E. Ressouche , M. R. Lees , G. Balakrishnan

The search for two dimensional quantum spin liquids, exotic magnetic states with an entangled ground state remaining disordered down to zero temperature, has been a great challenge in frustrated magnetism during the last decades. Recently,…

Strongly Correlated Electrons · Physics 2018-10-15 E. Lhotel , S. Petit , M. Ciomaga Hatnean , J. Ollivier , H. Mutka , E. Ressouche , M. R. Lees , G. Balakrishnan

Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…

Strongly Correlated Electrons · Physics 2015-05-30 Sylvain Petit , Pierre Bonville , Isabelle Mirebeau , Hannu Mutka , Julien Robert

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order…

Strongly Correlated Electrons · Physics 2025-02-28 Ludovic D. C. Jaubert , Yasir Iqbal , Harald O. Jeschke

In their recent communication (Phys. Rev. B 64, 060406(R) (2001)) Cornelius and Gardner have reported the results of magnetization and susceptibility studies on single crystals of the pyrochlore Ho2Ti2O7. The observed field dependence of…

Strongly Correlated Electrons · Physics 2009-11-07 O. A. Petrenko , M. R. Lees , G. Balakrishnan

We consider possible exotic ground states of quantum spin ice as realized in rare earth pyrochlores. Prior work in Phys. Rev. Lett. 108, 037202 introduced a gauge mean field theory (gMFT) to treat spin or pseudospin Hamiltonians for such…

Strongly Correlated Electrons · Physics 2015-06-04 SungBin Lee , Shigeki Onoda , Leon Balents

The consequences of nonmagnetic-ion dilution for the pyrochlore family Y$_{2}$($M_{1-x}N_{x}$)$_{2}$O$_{7}$ ($M$ = magnetic ion, $N$ = nonmagnetic ion) have been investigated. As a first step, we experimentally examine the magnetic…

Strongly Correlated Electrons · Physics 2017-10-04 L. Shen , C. Greaves , R. Riyat , T. C. Hansen , E. Blackburn

We report low temperature specific heat and muon spin relaxation/rotation ($\mu$SR) measurements on both polycrystalline and single crystal samples of the pyrochlore magnet Yb$_2$Ti$_2$O$_7$. This system is believed to possess a spin…

Collective behaviour of electrons, frustration induced quantum fluctuations and entanglement in quantum materials underlie some of the emergent quantum phenomena with exotic quasi-particle excitations that are highly relevant for…