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The coherent spin dynamics of holes are investigated for CsPbBr$_3$ and CsPb(Cl,Br)$_3$ perovskite nanocrystals in a glass matrix using the time-resolved Faraday rotation/ellipticity techniques. In an external magnetic field, pronounced…

The lead halide perovskite nanocrystals embedded into a glass matrix exhibit strong interaction with light and demonstrate exceptional optical and spin related features along with long-term chemical and physical stability. We apply the spin…

Mesoscale and Nanoscale Physics · Physics 2025-02-25 V. O. Kozlov , I. A. Smirnov , M. S. Kuznetsova , E. V. Kolobkova , G. G. Kozlov , V. S. Zapasskii , D. S. Smirnov , I. I. Ryzhov

Optical orientation of electron and hole spins by circularly polarized light is investigated for MAPbI$_3$ single crystals. The Hanle and polarization recovery effects measured in transverse and longitudinal magnetic fields, respectively,…

Mesoscale and Nanoscale Physics · Physics 2026-02-10 Mladen Kotur , Nataliia E. Kopteva , Dmitri R. Yakovlev , Bekir Turedi , Maksym V. Kovalenko , Manfred Bayer

The spin physics of perovskite nanocrystals with confined electrons or holes is attracting increasing attention, both for fundamental studies and spintronic applications. Here, stable CsPb(Cl$_{0.5}$Br$_{0.5}$)$_3$ lead halide perovskite…

Methylammonium lead triiodine (MAPbI$_3$) is a material representative of the hybrid organic-inorganic lead halide perovskites which attract currently great attention due to their photovoltaic efficiency and bright optoelectronic…

Materials Science · Physics 2022-06-08 E. Kirstein , D. R. Yakovlev , E. A. Zhukov , J. Höcker , V. Dyakonov , M. Bayer

The Land\'e $g$-factor of charge carriers is a key parameter in spin physics controlling spin polarization and spin dynamics. In turn, it delivers information of the electronic band structure in vicinity of the band gap and its modification…

The coherent spin dynamics of electrons and holes in CsPbI3 perovskite nanocrystals in a glass matrix are studied by the time-resolved Faraday ellipticity technique in magnetic fields up to 430 mT across a temperature range from 6 K up to…

A theory of electron spin relaxation in semiconducting carbon nanotubes is developed based on the hyperfine interaction with disordered nuclei spins I=1/2 of $^{13}$C isotopes. It is shown that strong radial confinement of electrons…

Materials Science · Physics 2009-11-11 Y. G. Semenov , K. W. Kim , G. J. Iafrate

We have performed a systematic calculation for the non-Markovian dynamics of a localized electron spin interacting with an environment of nuclear spins via the Fermi contact hyperfine interaction. This work applies to an electron in the s…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 W. A. Coish , Daniel Loss

Carrier spins in semiconductor nanocrystals are promising candidates for quantum information processing. Using a combination of time-resolved Faraday rotation and photoluminescence spectroscopies, we demonstrate optical spin polarization…

Metal halide perovskites make up a promising class of materials for semiconductor spintronics. Here we report a systematic investigation of coherent spin precession, spin dephasing and spin relaxation of electrons and holes in two hybrid…

Materials Science · Physics 2024-08-20 Haochen Zhang , Zehua Zhai , Zhixuan Bi , Han Gao , Meng Ye , Yong Xu , Hairen Tan , Luyi Yang

Optical orientation of carrier spins by circularly polarized light is the basic concept and tool of spin physics in semiconductors. We study the optical orientation of electrons and holes in a crystal of the…

We present an advanced method to study spin fluctuations in superconductors quantitatively, and entirely from first principles. This method can be generally applied to materials where electron-phonon coupling and spin fluctuations coexist.…

Superconductivity · Physics 2018-01-16 Jonas Bekaert , Alex Aperis , Bart Partoens , Peter M. Oppeneer , Milorad V. Milošević

A possibility of controlled manipulation of electron spin states has been investigated for a cylindrical two-dimensional electron gas confined in a semiconductor nanotube/cylindrical nanowire with the Rashba spin-orbit interaction. We…

Mesoscale and Nanoscale Physics · Physics 2014-04-03 P. Wójcik , J. Adamowski , M. Wołoszyn , B. J. Spisak

The lead halide perovskites demonstrate huge potential for optoelectronic applications, high energy radiation detectors, light emitting devices and solar energy harvesting. Those materials exhibit strong spin-orbit coupling enabling…

Perovskite nanocrystals are a convenient model system for optical spin orientation and manipulation. However, its real potential might be underestimated due to the incomplete knowledge on spin relaxation times, which are obscured by the…

The tunability of the optical properties of lead halide perovskite nanocrystals makes them highly appealing for applications. Both, halide anion exchange and quantum confinement pave the way for tailoring their band gap energy. For…

The combined effect of electron-electron interactions and spin-orbit scattering in metal nanoparticles can be studied by measuring splitting of electron levels in magnetic field ($g$ factors) in tunneling spectroscopy experiments. Using…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Denis A. Gorokhov , Piet W. Brouwer

Long spin coherence times of carriers are essential for implementing quantum technologies using semiconductor devices for which, however, a possible obstacle is spin relaxation. For the spin dynamics, decisive features are the band…

Optical spin orientation measured by time-resolved photoluminescence provides a powerful tool to probe the spin dynamics of excitons and charge carriers in perovskite semiconductors. The impact of alloy fluctuations on the spin dynamics of…

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