Related papers: Photoinduced Frustration Modulation in $\kappa$-ty…
The layered molecular conductors $\kappa$-(BEDT-TTF)$_2$X are a perfect experimental platform for studying the physics of the Mott transition and related exotic electronic states. In these materials, the subtle balance between various…
We review the interplay of frustration and strong electronic correlations in quasi-two-dimensional organic charge transfer salts, such as k-(BEDT-TTF)_2X and Et_nMe_{4-n}Pn[Pd(dmit)2]2. These two forces drive a range of exotic phases…
Geometric frustration is a key ingredient in the emergence of exotic states of matter, such as the quantum spin liquid in Mott insulators. While there has been intense interest in experimentally tuning frustration in candidate materials,…
Quantum spin liquids provide paradigmatic examples of highly entangled quantum states of matter. Frustration is the key mechanism to favor spin liquids over more conventional magnetically ordered states. Here we propose to engineer…
Frustration, or the competition between interacting components of a network, is often responsible for the complexity of many body systems, from social and neural networks to protein folding and magnetism. In quantum magnetic systems,…
Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…
Geometrically frustrated many-particle quantum systems are notoriously hard to study numerically but are of profound interest because of their unusual properties and emergent phenomena. In these systems energetic constraints cannot be…
I analyze the decoherence of a $\pi$-junction qubit encoded by two co-located Majorana modes. Although not topologically protected, the qubit leverages distinct spatial profiles to couple to two independent environmental baths, realizing…
Triangular Heisenberg antiferromagnets are prototypes of geometric frustration, even if for nearest-neighbor interactions quantum fluctuations are not usually strong enough to destroy magnetic ordering: stronger frustration is required to…
Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…
Geometrical frustration in strongly correlated systems can give rise to a plethora of novel ordered states and intriguing magnetic phases, such as quantum spin liquids. Promising candidate materials for such phases can be described by the…
Unlike conventional magnets where the magnetic moments are partially or completely static in the ground state, in a quantum spin liquid they remain in collective motion down to the lowest temperatures. The importance of this state is that…
The Mott-insulator \kappa-(BEDT-TTF)_2Cu_2(CN)_3 is the prime candidate of a quantum spin liquid with puzzling magnetic properties. Our THz and infrared investigations reveal that also the charge dynamics does not follow the expectations…
We systematically derive low-energy effective Hamiltonians for molecular solids $\beta^\prime$-$X$[Pd(dmit)$_{2}$]$_{2}$ ($X$ represents a cation) using ab initio density functional theory calculations and clarify how the cation controls…
Magnetism plays a key role in modern technology as essential building block of many devices used in daily life. Rich future prospects connected to spintronics, next generation storage devices or superconductivity make it a highly dynamical…
We map a geometrically frustrated Ising system with transversal field generated quantum dynamics to a strongly anisotropic lattice of non-crossing elastic strings. The combined effect of frustration, quantum and thermal spin fluctuations is…
Geometric frustration is a broad phenomenon that results from an intrinsic incompatibility between some fundamental interactions and the underlying lattice geometry1-7. Geometric frustration gives rise to new fundamental phenomena and is…
Geometrical frustration is a powerful route to realize exotic phases such as quantum spin liquids. Despite extensive efforts, systematic searches targeting specific frustration motifs and their potential to host unconventional magnetic…
Resonant inelastic x-ray scattering at the N K edge reveals clearly resolved harmonics of the anion plane vibrations in the kappa-(BEDT-TTF)2Cu2(CN)3 spin-liquid insulator. Tuning the incoming light energy at the K edge of two distinct N…
The concept of geometrical frustration has led to rich insights into condensed matter physics, especially as a mechansim to produce exotic low energy states of matter. Here we show that frustration provides a natural vehicle to generate…