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In the context of high-accuracy computational thermochemistry, the valence CCSD correlation component of molecular atomization energies present the most severe basis set convergence problem, followed by the (T) component. In the present…

Chemical Physics · Physics 2016-06-23 Nitai Sylvetsky , Kirk A. Peterson , Amir Karton , Jan M. L. Martin

We put forward a broader picture of the effective theory of a spinning particle within the EFT of spinning gravitating objects, through which we derive and establish the new precision frontier at the fifth PN (5PN) order. This frontier…

High Energy Physics - Theory · Physics 2023-04-20 Michèle Levi , Zhewei Yin

Electronic structure calculations on small systems such as H$_2$, H$_2$O, LiH, and BeH$_2$ with chemical accuracy are still a challenge for the current generation of the noisy intermediate-scale quantum (NISQ) devices. One of the reasons is…

Chemical Physics · Physics 2022-11-15 Hyuk-Yong Kwon , Gregory M. Curtin , Zachary Morrow , C. T. Kelley , Elena Jakubikova

Determinantal varieties -- the sets of bounded-rank matrices or tensors -- have attracted growing interest in low-rank optimization. The tangent cone to low-rank sets is widely studied and underpins a range of geometric methods. The…

Optimization and Control · Mathematics 2025-12-12 Yan Yang , Bin Gao , Ya-xiang Yuan

We construct a reference benchmark set for atomic and molecular random-phase-approximation (RPA) correlation energies in a density functional theory (DFT) framework at the complete basis set limit. This set is used to evaluate the accuracy…

Chemical Physics · Physics 2013-02-22 E. Fabiano , F. Della Sala

Ab initio no-core configuration interaction (NCCI) calculations for the nuclear many-body problem have traditionally relied upon an antisymmetrized product (Slater determinant) basis built from harmonic oscillator orbitals. The accuracy of…

Quantum variational algorithms (QVAs) are increasingly potent tools for simulating quantum many-body systems on noisy intermediate-scale quantum (NISQ) devices. This work examines the application of the Variational Quantum Eigensolver (VQE)…

Nuclear Theory · Physics 2026-01-28 Dhritimalya Roy , Somnath Nag

The semi-exponential basis set of radial functions (A.M. Frolov, Physics Letters A {\bf 374}, 2361 (2010)) is used for variational computations of bound states in three-electron atomic systems. It appears that semi-exponential basis set has…

High Energy Physics - Phenomenology · Physics 2011-03-21 Alexei M Frolov

A relativistic description of the structure of heavy alkali atoms and alkali-like ions using S-spinors and L-spinors has been developed. The core wavefunction is defined by a Dirac-Fock calculation using an S-spinors basis. The S-spinor…

Atomic Physics · Physics 2017-01-05 Jun Jiang , J. Mitroy , Yongjun Cheng , Michael W. J. Bromley

Relativistic self-consistent mean-field (SCMF) models naturally account for the coupling of the nucleon spin to its orbital motion, whereas non-relativistic SCMF methods necessitate a phenomenological ansatz for the effective spin-orbit…

Nuclear Theory · Physics 2016-08-24 J. -P. Ebran , A. Mutschler , E. Khan , D. Vretenar

Together with experimental data, theoretically predicted dipole moments represent a valuable tool for different branches in the chemical and physical sciences. With the diversity of levels of theory and basis sets available, a reliable…

Chemical Physics · Physics 2021-01-27 Juan Camilo Zapata , Laura K. McKemmish

Relativistic Mean Field Theory in the rotating frame is used to describe superdeformed nuclei. Nuclear currents and the resulting spatial components of the vector meson fields are fully taken into account. Identical bands in neighboring…

Nuclear Theory · Physics 2009-10-22 J. K"onig , P. Ring

Recent interest in point and line node semimetals has led to the proposal and discovery of these phenomena in numerous systems. Frequently, though, these nodal systems are described in terms of individual properties reliant on specific…

Mesoscale and Nanoscale Physics · Physics 2016-10-12 Benjamin J. Wieder , C. L. Kane

A review of methods for finding general expressions for matrix elements (non-diagonal with respect to configurations included) of any one- and two-particle operator for an arbitrary number of shells in an atomic configuration is given.…

Atomic Physics · Physics 2007-05-23 G. Gaigalas

We have optimized the parameters of extended relativistic mean-field model using a selected set of global observables which includes binding energies and charge radii for nuclei along several isotopic and isotonic chains and the iso-scalar…

Nuclear Theory · Physics 2015-06-04 B. K. Agrawal , A. Sulaksono , P. -G. Reinhard

A systematic study of nuclear level densities has been carried out within the relativistic Hartree-Bogoliubov plus combinatorial framework. Calculations were performed for even-even nuclei with available experimental data, based on the…

Nuclear Theory · Physics 2026-05-07 Pengxiang Du , Jian Li

Complete orthonormal sets of exponential-type orbitals with non-integer principal quantum numbers are discussed as basis functions in non-relativistic Hartree-Fock-Roothaan electronic structure calculations of atoms. A method is proposed to…

Quantum Physics · Physics 2025-07-08 Ali Bagci , Philip E. Hoggan

We present a general methodology to evaluate matrix elements of the effective core potentials (ECPs) within one-electron basis set of Slater-type orbitals (STOs). The scheme is based on translation of individual STO distributions in the…

Chemical Physics · Physics 2017-05-17 Michal Lesiuk , Aleksandra M. Tucholska , Robert Moszynski

We deal with the effects induced on the orbit of a test particle revolving around a central body by putative spatial variations of fundamental coupling constants $\zeta$. In particular, we assume a dipole gradient for $\zeta(\bds…

General Relativity and Quantum Cosmology · Physics 2011-10-24 Lorenzo Iorio

We formulate criteria for identification of the nuclear tetrahedral and octahedral symmetries and illustrate for the first time their possible realization in a Rare Earth nucleus 152Sm. We use realistic nuclear mean-field theory…

Nuclear Theory · Physics 2018-03-14 J. Dudek , D. Curien , I. Dedes , K. Mazurek , S. Tagami , Y. R. Shimizu , T. Bhattacharjee
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