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This thesis studies light-matter interactions in strong and weak coupling regimes. In the first part, we study the formation and propagation of exciton-polariton condensates in different microcavities in the strong coupling regime.…

Mesoscale and Nanoscale Physics · Physics 2024-01-19 Dogyun Ko

Exciton polaritons based on atomically thin semiconductors are essential building blocks of quantum optoelectronic devices. Their properties are governed by an ultrafast and oscillatory energy transfer between their excitonic and photonic…

Hybridization of excitons with photons to form hybrid quasiparticles, exciton-polaritons (EPs), has been widely investigated in a range of semiconductor material systems coupled to photonic cavities. Self-hybridization occurs when the…

We theoretically demonstrate the coupling between excitons in 2D semiconductors and surface plasmons in a thin metal film by means of a surface acoustic wave (SAW), proving that the generated exciton-plasmon polaritons (or plexcitons) are…

Mesoscale and Nanoscale Physics · Physics 2021-07-30 Rajveer Fandan , Jorge Pedrós , Fernando Calle

We show that in the recent artificial light-harvesting experiment [Angewandte Chemie Intl. Ed. 55, 2759 (2016)] on organic nanocrystals self-assembled from difluoroboron chromophores, the spontaneous emission of an excited pigment should…

Applied Physics · Physics 2019-07-03 Yong-Cong Chen , Bo Song , Anthony J. Leggett , Ping Ao , Xiaomei Zhu

Sub-wavelength thick photonic crystal (PhC) slabs coupled to 2D excitonic materials, such as transition metal dichalcogenides (TMDs), are a promising platform for highly tunable, room-temperature, on-chip optoelectronic devices. Unlike…

Enabling coherent light-matter interactions is a critical step toward next-generation quantum technologies. However, achieving this under ambient temperature conditions remains challenging due to rapid dephasing in optically excited…

The strong coupling between photons and matter excitations such as excitons, phonons, and magnons is of central importance in the study of light-matter interactions. Bridging the flying and stationary quantum states, the strong light-matter…

We use path integral Monte Carlo to study the energetics of excitons in layered, hybrid organic-inorganic perovskites in order to elucidate the relative contributions of dielectric confinement and electron-phonon coupling. While the…

Materials Science · Physics 2025-03-26 Rohit Rana , David T. Limmer

The dynamics of a mobile quantum impurity in a degenerate Fermi system is a fundamental problem in many-body physics. The interest in this field has been renewed due to recent ground-breaking experiments with ultra-cold Fermi gases. Optical…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 Meinrad Sidler , Patrick Back , Ovidiu Cotlet , Ajit Srivastava , Thomas Fink , Martin Kroner , Eugene Demler , Atac Imamoglu

Strong coupling of two-dimensional semiconductor excitons with plasmonic resonators enables control of light-matter interaction at the subwavelength scale. Here we develop strong coupling in plasmonic nano-gap resonators that allow…

Exciton-polaritons (EPs) arising from strong light-matter coupling offer new pathways for controlling optoelectronic properties. While typically requiring closed optical cavities for strong coupling, we demonstrate that 2D metal-organic…

Optics · Physics 2025-12-11 Bongjun Choi , Adam D. Alfieri , Wangleong Chen , Deep Jariwala

Van der Waals antiferromagnetic and topological insulator materials provide powerful platforms for modern optical, electronic, and spintronic devices applications. The interaction between an antiferromagnet (AFM) and a topological insulator…

Exceptional points with coalescence of eigenvalues and eigenvectors are spectral singularities in the parameter space, achieving which often needs fine-tuning of parameters in quantum systems. We predict a \textit{persistent} realization of…

Mesoscale and Nanoscale Physics · Physics 2024-10-28 Zhuolun Qiu , Xi-Han Zhou , Hanchen Wang , Guang Yang , Tao Yu

We investigate the dynamics of photon echo exhibited by exciton-plasmon systems under strong coupling conditions. Using a self-consistent model based on coupled Maxwell-Bloch equations we investigate femtosecond time dynamics of ensembles…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 Adam Blake , Maxim Sukharev

Ultrastrong light-matter coupling has traditionally been studied in optical cavities, where it occurs when the light-matter coupling strength reaches a significant fraction of the transition frequency. This regime fundamentally alters the…

Optics · Physics 2025-05-13 Niclas S. Mueller , Eduardo B. Barros , Stephanie Reich

In recent years, organic materials have emerged as promising candidates for a variety of light-harvesting applications ranging from the infrared to the visible regions of the electromagnetic spectrum. Their enhanced excitonic binding…

Mesoscale and Nanoscale Physics · Physics 2025-06-19 V. G. M. Duarte , A. J. Chaves , N. M. R. Peres

Exciton-polaritons in organic materials are hybrid states that result from the strong interaction of photons and the bound excitons that these materials host. Organic polaritons hold great interest for optoelectronic applications, however…

Room temperature strong coupling of WS_2 monolayer exciton transitions to metallic Fabry-Perot and plasmonic optical cavities is demonstrated. A Rabi splitting of 101 meV is observed for the Fabry-Perot cavity, more than double those…

Materials Science · Physics 2016-08-24 S. Wang , S. Li , T. Chervy , A. Shalabney , S. Azzini , E. Orgiu , J. A. Hutchison , C. Genet , P. Samori , T. W. Ebbesen

The functionality of phonon-based quantum devices largely depends on the efficiency of interaction of phonons with other excitations. For phonon frequencies above 20 GHz, generation and detection of the phonon quanta can be monitored…