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Mirror symmetry is among the most fundamental concepts of physics and its spontaneous breaking at the molecular level allows chiral molecules to exist in two enantiomers that are mirror images of each other. The majority of chiro-optical…

Optics · Physics 2021-09-29 Alessandro Ciattoni

Chirality or handedness in condensed matter induces anomalous optical responses such as natural optical activity, rotation of the plane of light polarization, as a result of breaking of spatial-inversion symmetry. In this study, optical…

Mesoscale and Nanoscale Physics · Physics 2018-05-11 Hideo Kawaguchi , Gen Tatara

The chirality of an object can be studied by measuring the circular dichroism, that is, the difference in absorption of light with different helicity. The chiral optical response of an object, however, can have two different origins. On the…

Chiral functionalities exhibited by systems lacking any mirror symmetry encompass natural optical activity, magnetochiral effect, diagonal current-induced magnetization, chirality-selective spin-polarized current of charged electrons or…

Materials Science · Physics 2024-10-01 Sang-Wook Cheongand Fei-Ting Huang

Despite spin (SAM) and orbital (OAM) angular momentum dynamics are well-studied in demagnetization processes, their components receive less focus. Here, we utilize the non-collinear spin version of real-time time-dependent density…

Mesoscale and Nanoscale Physics · Physics 2024-02-28 Junjie He , Shuo Li , Thomas Fruenheim

Optical vortex beams are a type of topological light characterized by their inherent orbital angular momentum, leading to the propagation of a spiral-shaped wavefront. In this study, we focus on two-dimensional electrons with Rashba and…

Mesoscale and Nanoscale Physics · Physics 2025-12-04 Shunki Yamamoto , Masahiro Sato , Satoshi Fujimoto , Takeshi Mizushima

We theoretically analyze stimulated parametric down conversion as a means to produce dichroism based on the orbital angular momentum (OAM) of an incident signal field. The nonlinear interaction is shown to provide differential gain between…

Optics · Physics 2014-11-19 Joseph Lowney , Thomas Roger , Daniele Faccio , Ewan M. Wright

Optical beams carrying orbital angular momentum (OAM) have gained significant interest due to their unique properties, enhancing various communication systems and enabling applications such as the characterization of material or molecular…

Optics · Physics 2024-12-18 Ju-Young Kim , Minhaeng Cho

The interaction between light's angular momentum (AM) and material systems has unlocked new avenues in structured photonics, including in magneto-optical (MO) materials. While spin angular momentum (SAM) effects in MO systems are…

Optics · Physics 2025-07-04 Seth Nelson , Cong Yu , Daniel Watson , Shahrzad Ramtinfard , Miguel Levy

The inherent spin-orbit interaction of electrons inevitably couples spin to the orbital angular momentum (OAM), posing a fundamental challenge to spin-free orbital transport. Here, we propose a novel strategy to achieve spin-decoupled OAM…

Materials Science · Physics 2026-05-21 Dongjin Oh , Sungsoo Hahn , Chiara Pacella , Junseo Yoo , Angel Rubio , Domenico Di Sante , Changyoung Kim

Drawing inspiration from a remarkable chiral force found in nature, we show that a static electric field combined with an optical lin$\perp$lin polarization standing wave can exert a chiral optical force on a small chiral molecule that is…

Optics · Physics 2023-08-16 Robert P. Cameron , Duncan McArthur , Alison M. Yao

Optical spin and chirality play key roles in engineering photonic emission and light-matter interactions. Here we show that 3D evanescent coupling of guided modes by strongly confined waveguides can extrinsically produce optical spin and…

Optics · Physics 2024-11-26 Liang Fang , Jian Wang

The orbital angular momentum (OAM) of light is potentially interesting for astronomical study of rotating objects such as black holes, but the effect of reduced spatial coherence of astronomical light sources such as stars is largely…

Optics · Physics 2014-12-03 D. Hetharia , M. P. van Exter , W. Löffler

We report extremely strong optical activity and circular dichroism exhibited by subwavelength arrays of four-start-screw holes fabricated with one-pass focused ion beam milling of freely suspended silver films. Having the fourth order…

Optics · Physics 2015-06-19 M. V. Gorkunov , A. A. Ezhov , V. V. Artemov , O. Y. Rogov , S. G. Yudin

Locking of the spin of a quasi-particle to its momentum in split bands of on the surfaces of metals and topological insulators (TIs) is understood in terms of Rashba effect where a free electron in the surface states feels an effective…

Optical activity, the power of a medium to rotate the polarization of a light beam, has contributed significantly to molecular structure assessments in stereochemistry, biomolecular science and crystallography. Thus far, it is commonly…

In exploring the light-induced dynamics within the linear response regime, this study investigates the induced orbital angular momentum on a wide variety of electronic structures. We derive a general expression for the torque induced by…

Mesoscale and Nanoscale Physics · Physics 2023-11-28 Philippe Scheid , Stéphane Mangin , Sébastien Lebègue

We show, both theoretically and experimentally, that high-numerical-aperture (NA) optical microscopy is accompanied by strong spin-orbit interaction of light, which translates fine infomation about the specimen to the polarization degrees…

Metasurfaces, the two-dimensional analogues of metamaterials, are ideal platforms for sensing molecular chirality at the nanoscale, e.g. of inclusions of natural optically active molecules, as they offer large accessible areas (they are…

Applied Physics · Physics 2020-08-19 Sotiris Droulias

In this work we present an alternative way to look at electron diffraction in a transmission electron microscope. In stead of writing the scattering amplitude in Fourier space as a set of plane waves, we use the cylindrical Fourier…

Instrumentation and Detectors · Physics 2015-11-13 Roeland Juchtmans , Jo Verbeeck