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First-principles calculations combining density functional theory and many-body perturbation theory can provide microscopic insight into the dynamics of electrons and phonons in materials. We review this theoretical and computational…

Materials Science · Physics 2016-11-23 Marco Bernardi

Indium iodides, which adopt layered or molecular-crystal-like arrangements depending on composition, are expected to exhibit low lattice thermal conductivity because of their heavy constituent atoms and weak In-I bonding. In this work, we…

Materials Science · Physics 2026-01-06 Takuma Shiga , Yoshikazu Mizuguchi , Hiroshi Fujihisa

We present a framework for quantifying the uncertainty that results from the choice of exchange-correlation (XC) functional in predictions of phonon properties and thermal conductivity that use density functional theory (DFT) to calculate…

It is well known that conventional harmonic lattice dynamics cannot be applied to energetically unstable crystals at 0 K, such as high temperature body centered cubic (BCC) phase of crystalline Zr. Predicting phonon spectra at finite…

Materials Science · Physics 2019-01-02 Xin Qian , Ronggui Yang

We experimentally determine the lattice dynamics of black phosphorus layered crystals through a combination of x-ray diffuse scattering and inelastic x-ray scattering, and we rationalize our experimental findings using $\textit{ab initio}$…

This paper addresses the first principles description of coherent phonons in systems subjected to optical excitations and/or doping. We reformulate the first-principles Ehrenfest equation (fpEE) [Phys. Rev. X {\bf 13}, 031026 (2023)] in…

Materials Science · Physics 2025-04-24 Gianluca Stefanucci , Enrico Perfetto

High-order bases provide major advantages over linear ones in terms of efficiency, as they provide (for the same physical model) higher accuracy for the same running time, and reliability, as they are less affected by locking artifacts and…

Graphics · Computer Science 2023-05-30 Zachary Ferguson , Pranav Jain , Denis Zorin , Teseo Schneider , Daniele Panozzo

We present a comprehensive investigation of lattice dynamics in the double-helix antiferromagnet FeP by means of high-resolution time-of-flight neutron spectroscopy and ab-initio calculations. Phonons can hybridize with the magnetic…

We apply the compressive sensing lattice dynamics (CSLD) method to calculate phonon dispersion for crystalline solids. While existing methods such as frozen phonon, small displacement, and linear response are routinely applied for phonon…

Materials Science · Physics 2019-11-25 Fei Zhou , Babak Sadigh , Daniel Aberg , Yi Xia , Vidvuds Ozolins

The phonon thermal conductivity of semiconducting periodic solids can be obtained using the lattice dynamics calculations along with the Boltzmann transport equation and with input from density functional theory calculations. These…

Mesoscale and Nanoscale Physics · Physics 2025-05-30 Ankit Jain , Yagyank Srivastava , Amey G. Gokhale , Nidheesh Virakante , Hardik L. Kagdada

A method is presented to calculate from first principles the higher-order elastic constants of a solid material. The method relies on finite strain deformations, a density functional theory approach to calculate the Cauchy stress tensor,…

Materials Science · Physics 2025-10-08 Ruvini Attanayake , Umesh C. Roy , Abhiyan Pandit , Angelo Bongiorno

Topologically-engineered mechanical frames are important model constructs for architecture, machine mechanisms, and metamaterials. Despite significant advances in macroscopically fashioned frames, realization and phonon imaging of…

Materials Science · Physics 2024-03-26 Chang Qian , Ethan Stanifer , Zhan Ma , Binbin Luo , Chang Liu , Lehan Yao , Wenxiao Pan , Xiaoming Mao , Qian Chen

We have examined the commonly used Tersoff and Brenner empirical interatomic potentials in the context of the phonon dispersions in graphene. We have found a parameter set for each empirical potential that provides improved fits to some…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 L. Lindsay , D. A. Broido

With the growing maturity of additive manufacturing, the fabrication of architected or lattice-based metamaterials has become a reality for industrial applications. These materials combine lightweight design with tailored mechanical…

Numerical Analysis · Mathematics 2026-03-12 Clément Guillet , Thibaut Hirschler , Pierre Jolivet , Pablo Antolin , Robin Bouclier

The package "fhi96md" is an efficient code to perform density-functional theory total-energy calculations for materials ranging from insulators to transition metals. The package employs first-principles pseudopotentials, and a plane-wave…

Condensed Matter · Physics 2009-10-30 Michel Bockstedte , Alexander Kley , Joerg Neugebauer , Matthias Scheffler

Perturbative treatments of the lattice dynamics are widely successful for many crystalline materials, their applicability is, however, limited for strongly anharmonic systems, metastable crystal structures and liquids. The full dynamics of…

Materials Science · Physics 2023-10-10 Erik Fransson , Mattias Slabanja , Paul Erhart , Göran Wahnström

Intrinsic Frequency (IF) has recently been introduced as an ample signal processing method for analyzing carotid and aortic pulse pressure tracings. The IF method has also been introduced as an effective approach for the analysis of…

Numerical Analysis · Mathematics 2017-08-03 Peyman Tavallali , Hana Koorehdavoudi , Joanna Krupa

We present the derivation and code implementation of a first-principles methodology to calculate the lattice-mediated contributions to the bulk flexoelectric tensor. The approach is based on our recent analytical long-wavelength extension…

Materials Science · Physics 2022-02-16 Miquel Royo , Massimiliano Stengel

The study of polycrystalline materials requires theoretical and computational techniques enabling multiscale investigations. The amplitude expansion of the phase field crystal model (APFC) allows for describing crystal lattice properties on…

Computational Physics · Physics 2019-04-25 Simon Praetorius , Marco Salvalaglio , Axel Voigt

We present an \textit{ab initio} framework to calculate anharmonic phonon frequency and phonon lifetime that is applicable to severely anharmonic systems. We employ self-consistent phonon (SCPH) theory with microscopic anharmonic force…

Materials Science · Physics 2015-08-20 Terumasa Tadano , Shinji Tsuneyuki
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