Related papers: Arrested Ostwald Ripening in Non-Equilibrium Syste…
In active systems, whose constituents have non-equilibrium dynamics at local level, fluid-fluid phase separation is widely observed. Examples include the formation of membraneless organelles within cells; the clustering of self-propelled…
This paper considers an Ostwald ripening process in which new droplets are injected at a constant rate, with a fixed distribution of radii, and in which droplets are removed when they grow to a specified maximum radius. This process…
Understanding how multi-component liquid mixtures undergo phase separation is central to elucidating biophysical organization in the cell. Here, combining analytical and numerical results, we characterise the dynamics of mixtures with…
Living cells use phase separation and concentration gradients to organize chemical compartments in space. Here, we present a theoretical study of droplet dynamics in gradient systems. We derive the corresponding growth law of droplets and…
Chemically active droplets provide simple models for cell-like systems that can grow and divide. Such active droplet systems are driven away from thermodynamic equilibrium and turn over chemically, which corresponds to a simple metabolism.…
Additives of sparingly soluble components are known to slow down or completely inhibit Ostwald ripening in dispersed systems. In this paper, our earlier model of stabilization against Ostwald ripening is revisited and extended. In a…
Phase separation of biomolecular condensates promotes membrane-free compartmentalization in cells. The dynamics of these biocondensates is routinely regulated by energy-consuming processes. Here, we devise a theory pinpointing how active…
We present a systematic quasi-mean field model of the Ostwald ripening process in two dimensions. Our approach yields a set of dynamic equations for the temporal evolution of the minority phase droplets' radii. The equations contain only…
The ostwald ripening of bubbles is studied by molecular dynamics simulations involving up to 679 million Lennard-Jones particles. Many bubbles appear after depressurizing a system that is initially maintained in the pure-liquid phase, and…
Phase separation under non-equilibrium conditions is exploited by biological cells to organize their cytoplasm but remains poorly understood as a physical phenomenon. Here, we study a ternary fluid model in which phase-separating molecules…
Phase separation has recently emerged as an important organizational principle in the dense and heterogeneous environment within living cells. Here, we use a synthetic system to show that compressive stresses in a polymer network suppress…
Liquid-liquid phase separation is an important mechanism for compartmentalizing the cell's cytoplasm, allowing the dynamic organization of the components necessary for survival. However, it is not clear how phase separation is affected by…
Controlling the size of droplets, for example in biological cells, is challenging because large droplets typically outcompete smaller droplets due to surface tension. This coarsening is generally accelerated by hydrodynamic effects, but…
The phase separation mechanism of a binary liquid mixture off-critically quenched in its miscibility gap is nucleation and growth, its homogeneous phase reaching a metastable equilibrium state. The successive stages of growth of the…
Underground gas storage is central to both climate mitigation and energy transition strategies, supporting both long-term carbon sequestration and seasonal hydrogen storage. A key mechanism governing the fate of injected gases is Ostwald…
The Ostwald ripening phenomenon for gas bubbles in a liquid consists mainly in gas transfer from smaller bubbles to larger bubbles. An experiment was carried out in which the Ostwald ripening for air bubbles, in a liquid fluid with some…
We present a systematic extension of mean field models for Ostwald ripening in two dimensions. We derived, using a mean field type approximation, an analytic expression for pairwise interactions between the minority phase droplets. These…
We explore the evolution of the aggregate size distribution in systems where aggregates grow by diffusive accretion of mass. Supersaturation is controlled in such a way that the overall aggregate volume grows linearly in time. Classical…
Suspensions of spherical active particles often show microphase separation. At a continuum level, coupling their scalar density to fluid flow, there are two distinct explanations. Each involves an effective interfacial tension: the first…
In living cells, cycles of formation and dissolution of liquid droplets can mediate biological functions such as DNA repair. However, the minimal physicochemical prerequisite for such droplet oscillations remains elusive. Here, we present a…