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Magnetic adatom chains on surfaces constitute fascinating quantum spin systems. Superconducting substrates suppress interactions with bulk electronic excitations but couple the adatom spins to a chain of subgap Yu-Shiba-Rusinov (YSR)…

Magnetic adatoms coupled to an $s$-wave superconductor give rise to local bound states, so-called Yu-Shiba-Rusinov states. Focusing on the ultimate goal of tailoring chains of such adatoms into a topologically superconducting phase, we…

Superconductivity · Physics 2023-02-15 Philip Beck , Lucas Schneider , Roland Wiesendanger , Jens Wiebe

We study the effect of the coupling between the electronic ground state of high spin alkaline-earth fermionic atoms and their metastable optically excited state, when the system is confined in a one-dimensional chain, and show that the…

Quantum Gases · Physics 2015-06-16 Edina Szirmai

The coupling of a spin to an underlying substrate is the basis for a plethora of phenomena. In the case of a metallic substrate, Kondo screening of the adatom magnetic moment can occur. As the substrate turns superconducting, an intriguing…

Superconductivity · Physics 2020-11-18 Artem Odobesko , D. Di Sante , A. Kowalski , S. Wilfert , F. Friedrich , R. Thomale , G. Sangiovanni , M. Bode

Magnetic atoms on a superconductor give rise to Yu-Shiba-Rusinov (YSR) states within the superconducting energy gap. A spin chain of magnetic adatoms on an s-wave superconductor may lead to topological superconductivity accompanied by the…

Superconductivity · Physics 2018-08-15 Anand Kamlapure , Lasse Cornils , Jens Wiebe , Roland Wiesendanger

The hybridization of Yu-Shiba-Rusinov states in dimers of magnetic impurities leads to molecular-like bonding and antibonding modes. In many-impurity systems, the interaction gives rise to YSR bands and can even result in the formation of a…

Superconductivity · Physics 2023-02-03 Felix Friedrich , Robin Boshuis , Matthias Bode , Artem Odobesko

Magnetic atoms coupled to the Cooper pairs of a superconductor induce Yu-Shiba-Rusinov states (in short Shiba states). In the presence of sufficiently strong spin-orbit coupling, the bands formed by hybridization of the Shiba states in…

A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. Tiron , W. Wernsdorfer , D. Foguet-Albiol , N. Aliaga-Alcalde , G. Christou

Magnetic adatoms on a superconducting substrate undergo a quantum phase transition as their exchange coupling to the conduction electrons increases. For quantum spins, this transition is accompanied by screening of the adatom spin. Here, we…

Mesoscale and Nanoscale Physics · Physics 2022-06-22 Harald Schmid , Jacob F. Steiner , Katharina J. Franke , Felix von Oppen

Spin coupling between magnetic metal atoms and organic radicals plays a pivotal role in high-performance magnetic materials. The complex interaction involving multi-spin centers in bulk materials makes it challenging to study spin coupling…

Magnetic adatoms on superconductors induce Yu-Shiba-Rusinov (YSR) states, which are key to the design of low-dimensional correlated systems and topological superconductivity. Competing magnetic interactions and superconducting pairing lead…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 Lisa M. Rütten , Harald Schmid , Werner M. J. van Weerdenburg , Eva Liebhaber , Kai Rossnagel , Katharina J. Franke

The ground-state spin arrangement and the bipartite entanglement within Cu$^{2+}$-Cu$^{2+}$ dimers across the magnetization process of the 4f-3d heterometallic coordination polymer [{Dy(hfac)$_2$(CH$_3$OH)}$_2${Cu(dmg)(Hdmg)}$_2$]$_n$…

Statistical Mechanics · Physics 2022-07-28 Lucia Gálisová

Collective spin operators for symmetric multi-quDit (namely, identical $D$-level atom) systems generate a U$(D)$ symmetry. We explore generalizations to arbitrary $D$ of SU(2)-spin coherent states and their adaptation to parity…

Quantum Physics · Physics 2021-11-30 Manuel Calixto , Alberto Mayorgas , Julio Guerrero

We report the direct observation of two mid-gap core d-states of differing symmetry for a single Fe atom embedded in GaAs. These states are distinguished by the strength of their hybridization with the surrounding host electronic structure.…

Materials Science · Physics 2017-08-30 J. Bocquel , V. R. Kortan , R. P. Campion , B. L. Gallagher , M. E. Flatté , P. M. Koenraad

We present results for the electronic and magnetic structure of Mn and Fe clusters on Nb(110) surface, focusing on building blocks of atomic chains as possible realizations of topological superconductivity. The magnetic ground states of the…

Mesoscale and Nanoscale Physics · Physics 2021-09-29 András Lászlóffy , Krisztián Palotás , Levente Rózsa , László Szunyogh

Magnetic adsorbates on superconductors induce local bound states within the superconducting gap. These Yu-Shiba-Rusinov (\YSR) states decay slowly away from the impurity compared to atomic orbitals, even in 3d bulk crystals. Here, we use…

Mesoscale and Nanoscale Physics · Physics 2018-04-18 Michael Ruby , Benjamin W. Heinrich , Yang Peng , Felix von Oppen , Katharina J. Franke

The presence of long-range quantum spin correlations underlies a variety of physical phenomena in condensed matter systems, potentially including high-temperature superconductivity. However, many properties of exotic strongly correlated…

We study the magnetic and electronic phases of a 1D magnetic adatom chain on a 2D superconductor. In particular, we confirm the existence of a `self-organized' 1D topologically non-trivial superconducting phase within the set of subgap…

Superconductivity · Physics 2016-10-20 M. H. Christensen , M. Schecter , K. Flensberg , B. M. Andersen , J. Paaske

We discuss spin-$S$ antiferromagnetic Heisenberg chains with three-spin interactions, next-nearest-neighbor interactions, and bond alternation. First, we prove rigorously that there exist parameter regions of the exact dimerized ground…

Strongly Correlated Electrons · Physics 2014-01-30 Zheng-Yuan Wang , Shunsuke C. Furuya , Masaaki Nakamura , Ryo Komakura

Quantum phase transition in dimerized antiferromagnetic Heisenberg spin chain has been studied. A staircase structure in the variation of concurrence within strongly coupled pairs with that of external magnetic field has been observed…

Quantum Physics · Physics 2015-03-31 Aparajita Das , Sreeparna Bhadra , Sonali Saha
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