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We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

Atomic Physics · Physics 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

Using dynamical Hartree-Fock mean-field theory, we study the high-harmonic generation (HHG) in the fullerene molecules C$_{60}$ and C$_{70}$ under strong pump wave driving. We consider a strong-field regime and show that the output harmonic…

Atomic Physics · Physics 2021-10-04 H. K. Avetissian , A. G. Ghazaryan , G. F. Mkrtchian

Several correlation and interference effects in strong-field physics are investigated. We show that the interference of continuum wave packets can be the dominant mechanism of high-harmonic generation (HHG) in the over-the-barrier regime.…

Dynamically rich nature of the high-order harmonic generation process lends itself to a variety of ways to increase photon yield and extend the harmonic cut-off frequency. We show here that high-harmonic generation from an atom confined…

Atomic Physics · Physics 2019-12-25 T. Topcu , E. A. Bleda , Z. Altun

High-harmonic generation (HHG) spectrum from a LiH molecule induced by an intense laser pulse is computed and analyzed with potential energy surfaces for electron motion (ePES) constructed from a model of localized electron wave packets…

Chemical Physics · Physics 2020-03-18 Koji Ando

An optical cavity enhances the interaction between atoms and light, and the rate of coherent atom-photon coupling can be made larger than all decoherence rates of the system. For single atoms, this strong coupling regime of cavity quantum…

Quantum Physics · Physics 2007-11-10 Yves Colombe , Tilo Steinmetz , Guilhem Dubois , Felix Linke , David Hunger , Jakob Reichel

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

Recent experiments have revealed the tantalizing possibility of fabricating lattice electronic systems strongly coupled to quantum fluctuations of electromagnetic fields, e.g., by means of geometry confinement from a cavity or artificial…

Strongly Correlated Electrons · Physics 2022-05-03 Jiajun Li , Lukas Schamriß , Martin Eckstein

The polarization state of light plays a central role in strong-field light--matter interactions and is widely used to probe electronic structure in solids via high-order harmonic generation (HHG). In particular, helicity-resolved HHG has…

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

Atomic Physics · Physics 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

Strongly driven systems of emitters offer an attractive source of light over broad spectral ranges up to the X-ray region. A key limitation of these systems is that the light they emit is for the most part classical. We challenge this…

Quantum Physics · Physics 2023-06-06 Andrea Pizzi , Alexey Gorlach , Nicholas Rivera , Andreas Nunnenkamp , Ido Kaminer

We show that strong electron-electron interactions in cavity-coupled quantum materials can enable collectively enhanced light-matter interactions with ultrastrong effective coupling strengths. As a paradigmatic example we consider a…

Strongly Correlated Electrons · Physics 2019-09-04 Martin Kiffner , Jonathan Coulthard , Frank Schlawin , Arzhang Ardavan , Dieter Jaksch

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

Materials Science · Physics 2020-12-23 G. P. Zhang , Y. H. Bai

High-harmonic generation (HHG), a typical nonlinear optical effect, has been actively studied in electron systems such as semiconductors and superconductors. As a natural extension, we theoretically study HHG from electric polarization,…

Strongly Correlated Electrons · Physics 2020-03-10 Tatsuhiko N. Ikeda , Masahiro Sato

A reduced-density-matrix (RDM)-based approach to {\em ab initio} cavity quantum electrodynamics (QED) is developed. The expectation value of the Pauli-Fierz Hamiltonian is expressed in terms of one- and two-body electronic and photonic…

Chemical Physics · Physics 2022-11-23 Joel D. Mallory , A. Eugene DePrince

A system of one electron in a Coulomb potential in an optical cavity is solved using a tensor-product light-matter basis. The problem was treated at the level of the Pauli-Fierz Hamiltonian describing both light and matter quantum…

Chemical Physics · Physics 2024-07-12 Yetmgeta Aklilu , Kálmán Varga

Superradiance, the enhanced collective emission of light from a coherent ensemble of quantum systems, has been typically studied in atomic ensembles. In this work we study the enhanced emission of energy from coherent ensembles of harmonic…

Quantum Physics · Physics 2011-07-27 Michael Delanty , Stojan Rebic , Jason Twamley

High harmonic generation (HHG) is an extremely nonlinear effect, where a medium is driven by a strong laser field, generating coherent broadband radiation with photon energies ranging up to the X-ray and pulse durations reaching attosecond…

Optics · Physics 2020-10-20 Alexey Gorlach , Ofer Neufeld , Nicholas Rivera , Oren Cohen , Ido Kaminer

In this report, a novel methodology based on the static coherent states approach is introduced with the capability of calculating various strong-field laser-induced nonlinearities in full dimensional single-electron molecular systems; an…

Quantum Physics · Physics 2019-10-10 Mohammadreza Eidi , Mohsen Vafaee , Hamed Koochaki Kelardeh , Alexandra Landsman