Related papers: Charge-Transfer Complex $\kappa$-(BEST)$_2$Cu$_2$(…
The spin-liquid candidate $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(ethylenedithio)tetrathiafulvalene] does not exhibit magnetic ordering down to a very low temperature, but shows a mysterious anomaly at 6 K. The origin of the so-called 6 K…
The organic conductor $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_{3}$ seems to form a quantum spin liquid, although at low temperatures unusual properties are seen in the charge, spin and lattice degrees of freedom. Here we report results of X-band…
We investigated the local magnetism of the organic conductor, $\kappa$-(ET)$_{2}$Hg(SCN)$_{2}$Cl, with a quasi-triangular lattice of weakly dimerized molecules through $^{13}$C NMR spectroscopy. The NMR spectra and nuclear relaxation show…
It has been more than 40 years since superconductivity was discovered in organic conductors, and the way scientists view organic superconductors has changed over time. At first, the fact that organic conductors exhibit superconductivity was…
We report an impurity effect in the organic superconductor $\kappa$-(ET)$_2$Cu(NCS)$_2$ by substitution of the ET molecule with an analogue, bis(methyleneditio)tetrathiafulvalene (MT). The superconducting transition temperature decreases…
We have developed a novel BEDT-TTF-based organic conductor, $\kappa$-(BEDT-TTF)$_2 m$-HOOCC$_6$H$_4$SO$_3$ ($\kappa$-$m$-SBA), and propose it as a candidate for altermagnet. Tight-binding band calculations of $\kappa$-$m$-SBA provide a…
We report ab-initio calculations for the electronic structure of organic charge transfer salts $\kappa$-(ET)$_2$Cu[N(CN)$_2$]Br, $\kappa$-(ET)$_2$Cu[N(CN)$_2$]I, $\kappa^{\prime \prime}$-(ET)$_2$Cu[N(CN)$_2$]Cl and…
Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…
A few organic conductors show a diversity of exciting properties like Mott insulating behaviour, spin liquid, antiferromagnetism, bad metal or unconventional superconductivity controlled by small changes in temperature, pressure or chemical…
The electrodynamic response of the organic spin-liquid candidate $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been measured in an extremely wide energy range ($10^{-13}$ to 2 eV) as a function of temperature (5 to 300 K). Below the Mott gap,…
EtMe$_3$Sb[Pd(dmit)$_2$]$_2$, an organic Mott insulator with nearly isotropic triangular lattice, is a candidate material for a quantum spin liquid, in which the zero-point fluctuations do not allow the spins to order. The itinerant gapless…
The magnetic susceptibility of the organic superconductors $\kappa$-(h8 or d8-ET)$_{2}$$X$, $X =$ Cu(NCS)$_{2}$ and Cu[N(CN)$_{2}$]Br has been studied. A metallic phase below $T^{*} =$ 37 $\sim$ 38 K for $X =$ Cu[N(CN)$_{2}$]Br and 46…
We report a combined theoretical and experimental investigation of the superconducting state in the quasi-two-dimensional organic superconductor $\kappa$-(ET)$_2$Cu[N(CN)$_2$]Br. Applying spin-fluctuation theory to a low-energy…
We present high-resolution measurements of the relative length change as a function of temperature of the organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl. We identify anomalous features at $T_g \approx\,63$ K which can be…
We present a detailed structural investigation of the organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br at temperatures $T$ from 9 to 300 K. Anomalies in the $T$ dependence of the lattice parameters are associated with a…
We demonstrated X-ray structural analysis of the pressure-induced superconductor, $\beta'$-ET$_2$ICl$_2$ under extremely high-pressure conditions, where ET denotes bis(ethylenedithio)tetrathiafulvalene. This material has been known as the…
We performed angular and temperature-dependent electron-spin-resonance measurements in the quasi-two-dimensional organic conductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]I. The interlayer spin-diffusion is much weaker compared to the Cl- and…
The realization of BCS-BEC crossover in superconductors, which smoothly connects Bardeen-Cooper-Schrieffer (BCS) theory with Bose-Einstein Condensation (BEC) in fermion systems, is an intriguing recent topic in strongly correlated electron…
Utilizing infrared vibrational spectroscopy we have investigated dimerized two-dimensional organic salts in order to search for possible charge redistribution that might cause electronic dipoles and ferroelectricity: the quantum spin liquid…
The thermal conductivity $\kappa$ of the quasi-2D organic spin-liquid candidate EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ (dmit-131) was measured at low temperatures, down to 0.07 K. We observe a vanishingly small residual linear term $\kappa_0/T$, in…