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Electrochemical energy and substance conversion devices involve complex electrode processes, characterized by multiple charge transfer steps, competing pathways, and various intermediates. Such complexity makes it challenging to enhance…

The need to extract oil from wells where it is embedded on the surfaces of rocks has led to the development of new and improved enhanced oil recovery techniques. One of those is the injection of surfactants with water vapor, which promotes…

Soft Condensed Matter · Physics 2017-09-01 Ketzasmin A. Terrón-Mejía , Roberto López-Rendon , Armando Gama Goicochea

The conversion of CO2 into high-value chemicals through a photoreduction reaction in water is a promising route to reduce the dependence on fossil fuels. Ag nanoparticles can drive this reaction via localized surface plasmon resonance, but…

The desorption characteristics of molecules on interstellar dust grains are important for modelling the behaviour of molecules in icy mantles and, critically, in describing the solid-gas interface. In this study, a series of laboratory…

Solar and Stellar Astrophysics · Physics 2015-06-03 J. A. Noble , E. Congiu , F. Dulieu , H. J. Fraser

Dissociation of CO$_2$ on copper surfaces, a model system for understanding the elementary steps in catalytic conversion of CO$_2$ to methanol has been extensively studied in the past. It is thought to be reasonably well-understood from…

Chemical Physics · Physics 2024-01-30 Saurabh Kumar Singh , Pranav R. Shirhatti

The importance of co-adsorption for applications of porous materials in gas separation has motivated fundamental studies, which have initially focused on the comparison of the binding energies of different gas molecules in the pores (i.e.…

Materials Science · Physics 2015-04-08 Kui Tan , Sebastian Zuluaga , Qihan Gong , Yuzhi Gao , Nour Nijem , Jing Li , Timo Thonhauser , Yves J Chabal

CO oxidation on Ru(0001) is a long-standing example of a reaction that, being thermally forbidden in ultra-high vacuum, can be activated by femtosecond laser pulses. In spite of its relevance, the precise dynamics of the photo-induced…

Materials Science · Physics 2022-09-08 Auguste Tetenoire , Christopher Ehlert , J. I. Juaristi , Peter Saalfrank , M. Alducin

Adsorption of the molecule CO on metallic surfaces is an important unsolved problem in Kohn-Sham density functional theory (KS-DFT). We present a detailed study of carbon monoxide adsorption on fcc (111) surfaces of 3d, 4d and 5d metals…

Materials Science · Physics 2019-08-07 Abhirup Patra , Haowei Peng , Jianwei Sun , John P. Perdew

Ion hydrations are ubiquitous in natural and fundamental processes. A quantitative analysis of a novel CO2 sorbent driven by ion hydrations was presented by molecular dynamics (MD). We explored the humidity effect on the diffusion and…

Chemical Physics · Physics 2017-02-23 Xiaoyang Shi , Hang Xiao , Xi Chen , Tao Wang , Klaus. S. Lackner

A series of recyclable epoxy resin (REP) composites are successfully prepared in this study, aiming to improve flame retardancy while keep good recyclability and mechanical properties. The commercial…

Applied Physics · Physics 2021-05-06 Xiaolu Li , Jing Zhang , Lu Zhang , Alaitz Ruiz de Luzuriaga , Alaitz Rekondo , De-Yi Wang

Weakly bound, physisorbed hydrocarbons could in principle provide a similar water-repellency as obtained by chemisorption of strongly bound hydrophobic molecules at surfaces. Here we present experiments and computer simulations on the…

Understanding surface reactivity is crucial in many fields, going from heterogeneous catalysis to materials oxidation and corrosion. In order to decipher the surface reactions of ZrB2 exposed to the harsh environment of aerospace…

Materials Science · Physics 2021-08-18 Yanhui Zhang , Stefano Sanvito

Complete sticking at low incidence energies and broad angular scattering distributions at higher energies are often observed in molecular beam experiments on gas-surface systems which feature a deep chemisorption well and lack early…

Materials Science · Physics 2018-07-13 Ivor Lončarić , Gernot Füchsel , J. I. Juaristi , Peter Saalfrank

Using density functional theory and an exchange-correlationfunctional that includes the van der Waals interaction, we study the coadsorption of CO on Ru(0001) saturated with 0.5 ML of oxygen. Different coexisting CO coverages are considered…

Materials Science · Physics 2021-06-09 Auguste Tetenoire , J. Iñaki Juaristi , Maite Alducin

Underground carbon dioxide ($CO_2$) sequestration is considered to be one of the main methods to mitigate greenhouse gas (GHG) emissions. In this technology, pure $CO_2$ is injected into an underground geological formation and since it is…

Fluid Dynamics · Physics 2019-12-24 Federico Cao , Dmitry Eskin , Yuri Leonenko

Direct fired supercritical CO2 (sCO2) power cycles allow for the combustion of gaseous fuels under oxyfuel conditions with inherent carbon capture. As the CO2 is captured intrinsically, the efficiency penalty of capture on the overall plant…

Chemical Physics · Physics 2022-03-14 James M. Harman-Thomas , Kevin J. Hughes , Mohamed Pourkashanian

Mineralization of carbon dioxide is often seen as an attractive alternative to classical Carbon Capture and Storage (CCS) technologies, allowing the sequestration of \ce{CO2} as a solid mineral with no risk of aquifer contamination or…

Geophysics · Physics 2021-11-05 Florian Osselin , Michel Pichavant , Arnault Lassin

The discovery of high-performance electrocatalysts is crucial for advancing sustainable energy technologies. Compositionally complex solid solutions comprising multiple metals offer promising catalytic properties, yet their exploration is…

Materials Science · Physics 2025-02-27 F. Thelen , R. Zehl , R. Zerdoumi , J. L. Bürgel , L. Banko , W. Schuhmann , A. Ludwig

Environmental issues such as the wastewater have influenced each aspect of our lives. Coupling the existing remediation solutions with exploring new functional carbon nanomaterials (e.g. carbon nanotube, graphene oxide, graphene) by various…

Applied Physics · Physics 2019-05-21 Yanqing Wang , Can Panl , Adavan Kiliyankil Vipin , Ling Sun , Wei Chu

In a recent publication, we have highlighted the potential of phosphonic acid terminated PEG oligomers to functionalize strong UV absorption cerium oxide nanoparticles[1], which yield suspensions that are stable in aqueous or organic…

Materials Science · Physics 2013-05-07 L. Qi , J. Fresnais , P. Muller , O. Theodoly , J. -F. Berret , J. -P. Chapel
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