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The development of many optical quantum technologies depends on the availability of solid-state single quantum emitters with near-perfect optical coherence. However, a standing issue that limits systematic improvement is the significant…

Photon emission correlation spectroscopy is an indispensable tool for the study of atoms, molecules, and, more recently, solid-state quantum defects. In solid-state systems, its most common use is as an indicator of single-photon emission,…

Quantum Physics · Physics 2023-11-28 Rebecca E. K. Fishman , Raj N. Patel , David A. Hopper , Tzu-Yung Huang , Lee C. Bassett

Solid-state single-photon emitters (SPE) are a basis for emerging technologies such as quantum communication and quantum sensing. SPE based on fluorescent point defects are ubiquitous in semiconductors and insulators, and new systems with…

Mesoscale and Nanoscale Physics · Physics 2023-11-28 Leah R. Narun , Rebecca E. K. Fishman , Henry J. Shulevitz , Raj N. Patel , Lee C. Bassett

Single photon emitters are core building blocks of quantum technologies, with established and emerging applications ranging from quantum computing and communication to metrology and sensing. Regardless of their nature, quantum emitters…

Quantum Physics · Physics 2023-08-28 G. Landry , C. Bradac

Fluorescence microscopy is of vital importance for understanding biological function. However most fluorescence experiments are only qualitative inasmuch as the absolute number of fluorescent particles can often not be determined.…

Lanthanide nanoparticles (LnNPs) feature sharp emission lines together with millisecond emission lifetimes which makes them promising luminescent probes for biosensing and bioimaging. Although LnNPs are gathering a large interest, their…

A detailed study of the photophysical properties of several novel color centers in chemical vapor deposition diamond is presented. These emitters show narrow luminescence lines in the near infra-red. Single photon emission was verified with…

Quantum Physics · Physics 2015-05-14 I. Aharonovich , S. Castelletto , D. A. Simpson , A. D. Greentree , S. Prawer

We show that the single emitter linewidth underlying a broadened ensemble emission spectrum can be extracted from correlations among the stochastic intensity fluctuations in the ensemble spectrum. Spectral correlations can be observed at…

Optics · Physics 2009-03-13 Xavier Brokmann , Lisa Marshall , Moungi Bawendi

The excited state population of single solid-state emitters is subjected to energy fluctuations around the equilibrium driven by the bath and relaxation through the emission of phonons or photons. Simultaneous measurement of the associated…

Quantum Physics · Physics 2021-05-12 Hendrik Utzat , Moungi G. Bawendi

We present a simple method to measure the radiative and non-radiative recombination rates of individual fluorescent emitters at room temperature. By placing a single molecule successively close and far from a dielectric interface and…

Other Condensed Matter · Physics 2009-03-14 X. Brokmann , L. Coolen , Maxime Dahan , J. P. Hermier

We present an unbiased and robust analysis method for power-law blinking statistics in the photoluminescence of single nano-emitters, allowing us to extract both the bright- and dark-state power-law exponents from the emitters' intensity…

Data Analysis, Statistics and Probability · Physics 2015-01-06 J. Houel , Q. T. Doan , T. Cajgfinger , G. Ledoux , D. Amans , A. Aubret , A. Dominjon , S. Ferriol , R. Barbier , M. Nasilowski , E. Lhuillier , B. Dubertret , C. Dujardin , F. Kulzer

As single-photon sources become more mature and are used more often in quantum information, communications and measurement applications, their characterization becomes more important. Single-photon-like light is often characterized by its…

A sequence of photoluminescence spectroscopy based methods are used to rigorously identify and study all the main spectral features (more than thirty emission lines) of site controlled InGaAs/AlGaAs quantum dots (QDs) grown along [111]B in…

Interfacing single emitters and photonic nanostructures enables modifying their emission properties, such as enhancing individual decay rates or controlling the emission direction. To achieve full control, the single emitter must be…

In the solid state, a large variety of single-photon emitters present high quality photophysical properties together with a potential for integration. However, in many cases, the host matrix induces fluctuations of the emission wavelength…

Optics · Physics 2026-02-05 Aymeric Delteil , Stéphanie Buil , Jean-Pierre Hermier

Defect-based quantum emitters in solid state materials offer a promising platform for quantum communication and sensing. Confocal fluorescence microscopy techniques have revealed quantum emitters in a multitude of host materials. In some…

In today's development of quantum technologies a hybrid integration of phononic excitations becomes increasingly attractive. As natural quasi-particle excitations in solid state systems, phonons couple to virtually any other excitation and…

Quantum Physics · Physics 2026-01-12 Daniel Groll , Fabian Paschen , Paweł Machnikowski , Ortwin Hess , Daniel Wigger , Tilmann Kuhn

Fundamental understanding of biological pathways requires minimally invasive nanoscopic optical resolution imaging. Many approaches to high-resolution imaging rely on localization of single emitters, such as fluorescent molecule or quantum…

Quantum Physics · Physics 2022-04-05 Shuo Li , Wenchao Li , Vladislav V. Yakovlev , Allison Kealy , Andrew D. Greentree

The light emission of self-assembled (In,Ga)As/GaAs quantum dots embedded in single GaAs-based micropillars has been studied by time-resolved photoluminescence spectroscopy. The altered spontaneous emission is found to be accompanied by a…

We report on a Python-toolbox for unbiased statistical analysis of fluorescence intermittency properties of single emitters. Intermittency, i.e., step-wise temporal variations in the instantaneous emission intensity and fluorescence decay…

Computational Physics · Physics 2021-05-06 Isabelle M. Palstra , A. Femius Koenderink
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