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We present a novel method to measure transient photovoltage at nanointerfaces using ultrafast electron diffraction. In particular, we report our results on the photoinduced electronic excitations and their ensuing relaxations in a…

Materials Science · Physics 2009-11-13 Ryan A. Murdick , Ramani K. Raman , Yoshie Murooka , Chong-Yu Ruan

Proposals to determine biomolecular structures from diffraction experiments using femtosecond X-ray free-electron laser (XFEL) pulses involve a conflict between the incident brightness required to achieve diffraction-limited atomic…

Optics · Physics 2015-05-19 Harry M. Quiney , Keith A. Nugent

Knowledge of the molecular structure is key to understanding the function of participating molecules in photo-induced chemical reactions. Visualizing the nuclear dynamics of a photochemical reaction requires an ultrafast measurement…

Chemical Physics · Physics 2021-12-21 Kasra Amini

To date, high-resolution electron microscopy has largely relied on using the phase of the exit wave function at the exit surface to form a high-resolution electron microscopic image. We have for the first time used chromatic aberration…

Materials Science · Physics 2014-09-02 Jianguo Wen , Dean J. Miller , Nestor J. Zaluzec , Russell E. Cook , Ho Nyung Lee , Xifan Wu

Using a combination of high-level ab initio electronic structure methods with efficient on-the-fly semiclassical evaluation of nuclear dynamics, we performed a massive scan of small polyatomic molecules searching for a long lasting…

Chemical Physics · Physics 2024-09-26 Alan Scheidegger , Jiří Vaníček , Nikolay V. Golubev

The ability to resolve the dynamics of matter on its native temporal and spatial scales constitutes a key challenge and convergent theme across chemistry, biology, and materials science. The last couple of decades have witnessed ultrafast…

Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent…

Atomic resolution imaging in transmission electron microscopy (TEM) and scanning TEM (STEM) of light elements in electron-transparent materials has long been a challenge. Biomolecular materials, for example, are rapidly altered when…

Instrumentation and Detectors · Physics 2018-12-05 Fehmi S. Yasin , Tyler R. Harvey , Jordan J. Chess , Jordan S. Pierce , Colin Ophus , Peter Ercius , Benjamin J. McMorran

Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron…

Strongly Correlated Electrons · Physics 2023-03-13 V. Valmispild , E. Gorelov , M. Eckstein , A. Lichtenstein , H. Aoki , M. Katsnelson , M. Ivanov , O. Smirnova

The global observable distributions of nucleus-nucleus collisions at high energy are studied. It is shown that these distributions are sensitive to interaction dynamics and can be used to investigate the evolution of dense nuclear matter.…

High Energy Physics - Phenomenology · Physics 2009-12-15 M. V. Savina , S. V. Shmatov , N. V. Slavin , P. I. Zarubin

We study the proton-hydrogen collision in the energy range from 0 to 5 K where the hyperfine structure of the hydrogen atom is important. The proper multichannel treatment of the hyperfine structure is found to be crucial at cold…

Atomic Physics · Physics 2014-10-08 Ming Li , Bo Gao

Understanding of the precise mechanisms of high-temperature superconductivity is elusive. In particular, in order to solve the puzzle of the pairing mechanism, it is important to understand the detailed nature of the excitations at energies…

Superconductivity · Physics 2020-03-05 Fabio Novelli , Jonathan O. Tollerud , Dharmalingam Prabhakaran , Jeffrey A. Davis

Improving our understanding of electron dynamics is essential for advancing energy transfer, optoelectronics, light harvesting systems and quantum computing. Recent developments in attosecond x-ray sources provide the fundamental…

Computational Physics · Physics 2025-11-26 Maksim Radionov , Daria Popova-Gorelova

Holography relies on the interference between a known reference and a signal of interest to reconstruct both the amplitude and phase of that signal. Commonly performed with photons and electrons, it finds numerous applications in imaging,…

Transparent conducting oxides are highly doped semiconductors that exhibit favourable characteristics when compared to metals, including reduced material losses, tuneable electronic and optical properties, and enhanced damage thresholds.…

Recent advances in scanning transmission electron and scanning probe microscopies have opened exciting opportunities in probing the materials structural parameters and various functional properties in real space with angstrom-level…

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

In this paper we do three things. First, we outline the conditions under which the interaction rate of inelastic processes that change the internal state of a system of $N$ targets scales as $N^2$. This is an effect distinct from coherent…

High Energy Physics - Phenomenology · Physics 2024-11-06 Asimina Arvanitaki , Savas Dimopoulos , Marios Galanis

Using a quantum-mechanical close-coupling method, we calculate cross sections for fine structure excitation and relaxation of Si and S atoms in collisions with atomic hydrogen. Rate coefficients are calculated over a range of temperatures…

Atomic Physics · Physics 2024-12-10 Pei-Gen Yan , James F. Babb

Monte-Carlo simulation calculation have been performed for 855 MeV electrons channeling in (110) planes of a diamond single crystal. The continuum potential picture has been utilized. Both, the transverse potential and the angular…

Computational Physics · Physics 2022-09-14 H. Backe