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We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…
Exciton effects on conjugated polymers are investigated in soliton lattice states. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration-…
We investigate the imaging properties of copper-based superlens surrounded by copper oxide (Cu$_2$O). A subwavelength image resolution of the order $\lambda/9$ is demonstrated theoretically and verified in numerical simulations. It is shown…
Within a homologous series of cuprate superconductors, variations in the stacking of CuO$_2$ layers influence the collective charge dynamics through the long-range Coulomb interactions. We use O $K$-edge resonant inelastic x-ray scattering…
Rydberg excitons, the solid-state counterparts of Rydberg atoms, have sparked considerable interest in harnessing their quantum application potentials, whereas a major challenge is realizing their spatial confinement and manipulation.…
Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…
We investigate the two-pulse photon echo response of excitons in the mixed lead halide perovskite crystal \sample in dependence on the excitation intensity and polarization of the incident laser pulses. Using spectrally narrow picosecond…
Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and…
The realization of exciton-polaritons -- hybrid excitations of semiconductor quantum well excitons and cavity photons -- has been of great technological and scientific significance. In particular, the short-range collisional interaction…
We observe the direct excitation of pairs of Cs atoms from the ground state to molecular states correlating asymptotically to $ns\,n'f$ asymptotes. The molecular resonances are interpreted as originating from the dipole-quadrupole…
Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…
The Gamma Factory (GF) initiative aims at the construction of a unique experimental tool exploiting resonant interaction of light with ultra-relativistic partially stripped ions (PSI) stored in circular accelerators at CERN. Resonant…
Spin excitations in the overdoped high temperature superconductors Tl$_2$Ba$_2$CuO$_{6+\delta}$ and (Bi,Pb)$_2$(Sr,La)$_{2}$CuO$_{6+\delta}$ were investigated by resonant inelastic x-ray scattering (RIXS) as functions of doping and detuning…
Excitons are fundamental excitations that govern the optical properties of semiconductors. Interacting excitons can lead to various emergent phases of matter and large nonlinear optical responses. In most semiconductors, excitons interact…
Quantum electrodynamic calculations predict that truly incoherent light can be used to efficiently generate quantum-degenerate exciton population states. Resonant incoherent excitation directly converts photons into excitons with vanishing…
When ground state atoms are excited to a Rydberg state, van der Waals interactions among them can lead to a strong suppression of the excitation. Despite the strong interactions the evolution can still be reversed by a simple phase shift in…
Exciton-phonon interactions govern the energy level spectrum and thus the optical response in semiconductors. In this respect, lead-halide perovskite nanocrystals represent a unique system, for which the interaction with optical phonons is…
The basic theoretical foundation for the modelling of phonon assisted absorption spectra in direct bandgap semiconductors, introduced by Elliott 60 years ago using second order perturbation theory, results in a square root shaped dependency…
Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultra-violet (XUV)…
The Cu-$3d$ states in the high-$T_c$ cuprates are often described as a single band of $3d_{x^2-y^2}$ states, with the other four $3d$ states having about 2 to 3 eV higher energy due to the lower-than-octahedral crystal field at the copper…