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Related papers: Interaction between Rydberg Excitons in Cuprous Ox…

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We investigate the infrared optical transitions between excitons of the yellow, green and blue series in the cuprous oxide Cu$_{\mathrm{2}}$O. We show that in many cases the dipole approximation is inadequate and, in particular, that it…

Mesoscale and Nanoscale Physics · Physics 2019-08-05 Sjard Ole Krüger , Stefan Scheel

Rydberg states of excitons in Cu$_2$O are known to interact strongly with other carriers in their surrounding such as other excitons, free charge carriers and static charged impurities. In cw-experiments, discriminating the individual…

Mesoscale and Nanoscale Physics · Physics 2024-09-24 Binodbihari Panda , Julian Heckötter , Simon Siegeroth , Mariam Harati , Marc Aßmann

We report exciton-mediated coupling between microwave and optical fields in cuprous oxide (Cu$_2$O) at low temperatures. Rydberg excitonic states with principal quantum number up to $n=12$ were observed at 4~K using both one-photon…

We use two-color pump-probe spectroscopy to study Rydberg excitons in Cu$_2$O in the presence of free carriers injected by above-band-gap excitation. Already at plasma densities $\rho_\text{eh}$ below one hundredth electron-hole pair per…

Materials Science · Physics 2018-09-12 J. Heckötter , M. Freitag , D. Fröhlich , M. Aßmann , M. Bayer , P. Grünwald , F. Schöne , D. Semkat , H. Stolz , S. Scheel

In this study we analyze the transmission spectrum of a thin plate of Cuprous Oxide in the range of the absorption of the yellow exciton states with the coherent transfer matrix method. We demonstrate that, in contrast to the usual analysis…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Heinrich Stolz , Rico Schwartz , Julian Heckötter , Marc Aßmann , Dirk Semkat , Sjard O. Krüger , Manfred Bayer

The observation of giant Rydberg excitons in cuprous oxide $\left(\mathrm{Cu_{2}O}\right)$ up to a principal quantum number of $n=25$ by T.~Kazimierczuk \emph{et al.} [Nature \textbf{514}, 343, (2014)] inevitably raises the question whether…

Materials Science · Physics 2017-12-07 Frank Schweiner , Jan Ertl , Jörg Main , Günter Wunner , Christoph Uihlein

Excitons, i.e. the bound states of an electron and a positively charged hole are the solid state analogue of the hydrogen atom. As such they exhibit a Rydberg series, which in cuprous oxide has been observed up to high principal quantum…

Mesoscale and Nanoscale Physics · Physics 2025-11-18 Jan Ertl , Patric Rommel , Jörg Main

We analyze theoretically the Coulomb scattering processes of highly excited excitons in the direct bandgap semiconductor quantum wells. We find that contrary to the interaction of ground state excitons the electron and hole exchange…

Mesoscale and Nanoscale Physics · Physics 2016-06-15 V. Shahnazaryan , I. A. Shelykh , O. Kyriienko

The efficient optical second-harmonic generation (SHG) of two-dimensional (2D) crystals, coupled with their atomic thickness that circumvents the phase-match problem, has garnered considerable attention. While various 2D heterostructures…

Materials Science · Physics 2023-10-31 Wontaek Kim , Gyouil Jeong , Juseung Oh , Jihun Kim , Kenji Watanabe , Takashi Taniguchi , Sunmin Ryu

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

We study the absorption spectra of the yellow excitons in Cu$_2$O in high magnetic fields using polarization-resolved optical absorption measurements with a high frequency resolution. We show that the symmetry of the yellow exciton results…

We report on the experimental and theoretical investigation of magnetic-field-induced second harmonic generation (SHG) and two-photon absorption (TPA) of excited exciton states ($n \geq 3$) of the yellow series in Cu$_2$O. In this…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 A. Farenbruch , J. Mund , D. Fröhlich , D. R. Yakovlev , M. Bayer , M. A. Semina , M. M. Glazov

Recent high-resolution absorption spectroscopy on excited excitons in cuprous oxide [Nature (London) 514, 343 (2014)] has revealed significant deviations of their spectrum from that of the ideal hydrogen-like series. Here we show that the…

Excitons with a radius of a few lattice constants can be affected by strong central-cell corrections, leading to significant deviations of the optical spectrum from the hydrogen-like Rydberg series, and also to an enhancement of the exciton…

Materials Science · Physics 2018-01-30 Andreas Alvermann , Holger Fehske

We propose to implement a new kind of solid-state single-photon source based on the recently observed Rydberg blockade effect for excitons in cuprous oxide. The strong interaction between excitons in levels with high principal quantum…

Quantum Physics · Physics 2017-10-24 Mohammadsadegh Khazali , Khabat Heshami , Christoph Simon

We report on the observation of ultralong range interactions in a gas of cold Rubidium Rydberg atoms. The van-der-Waals interaction between a pair of Rydberg atoms separated as far as 100,000 Bohr radii features two important effects:…

For an ultra-dense exciton gas in cuprous oxide (Cu$_2$O), exciton-exciton interactions are the dominant cause of exciton decay. This study demonstrates that the accepted Auger recombination model overestimates the exciton decay rate…

Quantum Gases · Physics 2015-08-11 Laszlo Frazer , Richard D. Schaller , J. B. Ketterson

We use nonlinear pump-probe spectroscopy to study optical excitations in a charge-tunable MoSe$_2$\WS$_2$ moir\'e heterostructure. An intense red-detuned laser pulse creates a photonic dressing of the material by introducing a large virtual…

Strongly Correlated Electrons · Physics 2025-06-02 B. Evrard , H. S. Adlong , A. A. Ghita , T. Uto , L. Ciorciaro , K. Watanabe , T. Taniguchi , M. Kroner , A. İmamoğlu

Strongly bound excitons and many-body interactions between them determine light-matter interactions in van der Waals (vdW) heterostructures of 2D semiconductors. Unlike fundamental particles, quasiparticles in condensed matter, such as…

Mesoscale and Nanoscale Physics · Physics 2022-08-12 Weijie Li , Zach Hadjri , Jin Zhang , Luka M. Devenica , Song Liu , James Hone , Kenji Watanabe , Takashi Taniguchi , Angel Rubio , Ajit Srivastava

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…