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The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…

The image information acquisition ability of a conventional camera is usually much lower than the Shannon Limit since it does not make use of the correlation between pixels of image data. Applying a random phase modulator to code the…

Optics · Physics 2016-05-18 Zhentao Liu , Shiyu Tan , Jianrong Wu , Enrong Li , Xia Shen , Shensheng Han

Coherent anti-Stokes Raman scattering (CARS) microscopy is combined with second harmonic generation (SHG) technique in order to follow the early stage of stem cell differentiation within a 3D scaffold. CARS microscopy can detect lipid…

Biological Physics · Physics 2015-10-28 Leonardo Mortati , Carla Divieto , Maria Paola Sassi

Here we show how time-resolved broadband optical spectroscopy can be used to quantify, with femtometer resolution, the oscillation amplitudes of coherent phonons through a displacive model without free tuning parameters, except an overall…

Materials Science · Physics 2020-10-08 Davide Soranzio , Maria Peressi , Robert J. Cava , Fulvio Parmigiani , Federico Cilento

Accurate detection of cancer tissue regions (CTR) enables deeper analysis of the tumor microenvironment and offers crucial insights into treatment response. Traditional CTR detection methods, which typically rely on the rich cellular…

Computer Vision and Pattern Recognition · Computer Science 2026-03-09 Shuailin Xue , Jun Wan , Lihua Zhang , Wenwen Min

Thermometric techniques with high accuracy, fast response speed and ease of implementation are desirable for the study of dynamic combustion environments, transient reacting flows, and non-equilibrium plasmas. Herein, single-shot…

Charge-density waves (CDWs) are ordered quantum states of conduction electrons accompanied by periodic lattice distortions. Raman scattering (RS) spectroscopy is therefore well suited for probing CDW-induced structural modulations. We…

We present a femtosecond time-resolved optical spectroscopy (TRS) as an experimental tool to probe the changes in the low energy electronic density of states as a result of short and long range charge density wave order. In these…

Strongly Correlated Electrons · Physics 2007-05-23 J. Demsar , D. Mihailovic , V. V. Kabanov , K. Biljakovic

Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…

We demonstrate a compact, cost-effective snapshot spectral imaging system named Aperture Diffraction Imaging Spectrometer (ADIS), which consists only of an imaging lens with an ultra-thin orthogonal aperture mask and a mosaic filter sensor,…

Computer Vision and Pattern Recognition · Computer Science 2023-09-29 Tao Lv , Hao Ye , Quan Yuan , Zhan Shi , Yibo Wang , Shuming Wang , Xun Cao

We simulate a third-order nonlinear signal in a pump-probe spectroscopy from the interference between first- and second-order wavepackets (WPs), as well as from a state-to-state transition for Stokes and coherent anti-Stokes pathways in the…

Chemical Physics · Physics 2026-04-14 Subho Mitra , Arijit K. De

We investigate the arrival statistics of Stokes (S) and anti-Stokes (aS) Raman photons generated in diamond membranes. Strong quantum correlations between the S and aS signals are observed, which implies that the two processes share the…

Quantum Physics · Physics 2015-03-03 Mark Kasperczyk , Ado Jorio , Elke Neu , Patrick Maletinsky , Lukas Novotny

Spatiotemporal optical coherence (STOC) imaging is a new technique for suppressing coherent crosstalk noise in Fourier-domain full-field optical coherence tomography (FD-FF-OCT). In STOC imaging, the timevarying inhomogeneous phase masks…

The emergence of label-free microscopy techniques has significantly improved our ability to precisely characterize biochemical targets, enabling non-invasive visualization of cellular organelles and tissue organization. Each label-free…

Optics · Physics 2024-05-08 Lang Wang , Maxine Xii , Ali Pezeshki , Randy Bartels

Surface Enhanced Raman Spectroscopy (SERS) is a well-established technique for enhancing Raman signals. Recently photonic integrated circuits have been used, as an alternative to microscopy based excitation and collection, to probe SERS…

An accurate treatment of electronic spectra in large systems with a technique such as time dependent density functional theory (TDDFT) is computationally challenging. Due to the Nyquist sampling theorem, direct real time simulations must be…

Materials Science · Physics 2024-01-17 Matthias Kick , Ezra Alexander , Anton Beiersdorfer , Troy Van Voorhis

The non-equilibrium ro-vibrational distribution functions of molecules in a plasma can heavily influence the discharge operation and the plasma-chemistry. A convenient method for measuring the distribution function is by means of coherent…

Plasma Physics · Physics 2021-07-14 Jan Kuhfeld , Nikita Lepikhin , Dirk Luggenhölscher , Uwe Czarnetzki

We demonstrate a simple and robust high-resolution ghost spectroscopy approach for x-ray and extreme ultraviolet absorption spectroscopy at free-electron laser sources. Our approach requires an on-line spectrometer before the sample and a…

Bond-resolved STM (BRSTM) is a recent technique that combines the advantages of scanning tunneling microscopy (STM) with the outstanding intramolecular resolution provided by non-contact atomic force microscopy (ncAFM) using a…

With the advent of neuroimaging and microsurgery, there is a rising need for capturing images through an optical fiber. We present an approach of imaging through a single fiber without mechanical scanning by implementing spatial-spectral…