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The optical nonlinearity of WS2, MoS2 monolayer and few-layer films was investigated using the Z-scan technique with femtosecond pulses from the visible to the near infrared. The dependence of nonlinear absorption of the WS2 and MoS2 films…

Strong two-photon absorption (TPA) in monolayer MoS2 is demonstrated in contrast to saturable absorption (SA) in multilayer MoS2 under the excitation of femtosecond laser pulses in the near infrared region. MoS2 in the forms of monolayer…

As a rapidly expanding family of two dimensional (2D) materials, MXenes have recently gained considerable attention due to their appealing properties. Here, by developing a solution based coating method that enables transfer free and layer…

Optics · Physics 2024-06-18 David J. Moss

Femtosecond pump-probe measurements find pronounced dimensionality dependence of the optical nonlinearity in cuprates. Although the coherent two-photon absorption (TPA) and linear absorption bands nearly overlap in both quasi-one and…

Strongly Correlated Electrons · Physics 2009-11-07 M. Ashida , Y. Taguchi , Y. Tokura , R. T. Clay , S. Mazumdar , Yu. P. Svirko , M. Kuwata-Gonokami

Advanced photonic materials showing two-photon absorption (2PA) have been widely explored to develop three-dimensional imaging, micro and nanofabrication, all-optical switching, lithography on a nanoscale and many other enabling…

Two dimensional materials such as graphene and transition metal dichalcogenides (TMDs) are promising for optical modulation, detection, and light emission since their material properties can be tuned on-demand via electrostatic doping. The…

Ultrafast, femtosecond laser pulse interaction with dielectric materials has shown them to have significantly higher laser fluence threshold requirements, as compared to metals and semiconductors, for laser material modification, such as…

Materials Science · Physics 2020-03-11 Saurabh Awasthi , Douglas J. Little , A. Fuerbach , D. M. Kane

In integrated photonics, specific wavelengths are preferred such as 1550 nm due to low-loss transmission and the availability of optical gain in this spectral region. For chip-based photodetectors, layered two-dimensional (2D) materials…

Non-degenerate two-photon absorption (TPA) is investigated in a nanophotonic silicon waveguide in a configuration such that the dispersion of the nonlinear absorption and refraction cannot be neglected. It is shown that a signal wave can…

Two-dimensional (2D) materials, due to their remarkable physical and chemical properties, hold significant potential for future optical and electrical applications. In this study, the synthesis of 2D phlogopite (magnesium-rich mica) via…

Nonlinear optical (NLO) phenomena such as harmonic generation, Kerr, and Pockels effects are of great technological importance for lasers, frequency converters, modulators, switches, etc. Recently, two-dimensional (2D) materials have drawn…

The optical response of traditional semiconductors depends on the laser excitation power used in experiments. For two-dimensional (2D) semiconductors, laser excitation effects are anticipated to be vastly different due to complexity added…

Two-dimensional (2D) compounds provide unique building blocks for novel layered devices and hybrid photonic structures. However, large surface-to-volume ratio in thin films enhances the significance of surface interactions and charging…

We present a detailed calculation of the linear and nonlinear optical response of four types of monolayer Two-Dimensional (2D) Transition-Metal Dichalcogenides (TMDCs), having the formula $\textrm{MX}_2$ with M=Mo,W and X=S,Se. The…

Mesoscale and Nanoscale Physics · Physics 2018-08-28 Sina Khorasani

Despite being only a few atoms thick, single-layer two-dimensional (2D) materials display strong electron-photon interactions that could be utilized in efficient light modulators on extreme subwavelength scales. In various applications…

Mesoscale and Nanoscale Physics · Physics 2018-09-21 Sunny Gupta , Sharmila N. Shirodkar , Alex Kutana , Boris I. Yakobson

We report a large third order nonlinear optical response of palladium diselenide (PdSe2) films, a two dimensional (2D) noble metal dichalcogenide material. Both open aperture (OA) and closed aperture (CA) Z scan measurements are performed…

Optics · Physics 2020-05-05 Linnan Jia , Jiayang Wu , Tieshan Yang , Baohua Jia , David J. Moss

We present a comprehensive optical study of thin films of tungsten disulfide (WS$_2$) with layer thicknesses ranging from mono- to octalayer and in the bulk limit. It is shown that the optical band-gap absorption of monolayer WS$_2$ is…

Mesoscale and Nanoscale Physics · Physics 2017-09-19 Maciej R. Molas , Karol Nogajewski , Artur O. Slobodeniuk , Johannes Binder , Miroslav Bartos , Marek Potemski

Photodetector based on two-dimensional (2D) materials is an ongoing quest in optoelectronics. These 2D photodetectors are generally efficient at low illuminating power but suffer severe recombination processes at high power, which results…

The nonlinear absorption of two-dimensional molybdenum disulfide was analyzed using the Z-scan technique. Sample size corresponding to a number of layer determines the band gap in the materials which play the key role for nonlinearity.…

Optics · Physics 2019-11-28 Tikaram Neupane , Dulitha Jayakodige , Sheng Yu

Monolayers of transition-metal dichalcogenides such as WSe2 have become increasingly attractive due to their potential in electrical and optical applications. Because the properties of these 2D systems are known to be affected by their…

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