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We have recently demonstrated supervised deep learning methods for rapid generation of radiofrequency pulses in magnetic resonance imaging (https://doi.org/10.1002/mrm.27740, https://doi.org/10.1002/mrm.28667). Unlike the previous iterative…

Medical Physics · Physics 2021-11-01 Mads Sloth Vinding , David L. Goodwin , Ilya Kuprov , Torben Ellegaard Lund

Work within this thesis advances optimal control algorithms for application to magnetic resonance systems. Specifically, presenting a quadratically convergent version of the gradient ascent pulse engineering method. The work is formulated…

Quantum Physics · Physics 2018-08-30 David L. Goodwin

This article is aimed at extending the framework of optimal control techniques to the situation where the control field values are restricted to a finite set. We propose a generalization of the standard GRAPE algorithm suited to this…

Optimization and Control · Mathematics 2015-10-28 G. Dridi , M. Lapert , Julien Salomon , D Sugny , S. J. Glaser

In this paper, we propose a proximal gradient method and an accelerated proximal gradient method for solving composite optimization problems, where the objective function is the sum of a smooth and a convex, possibly nonsmooth, function. We…

Optimization and Control · Mathematics 2025-07-22 Raghu Bollapragada , Shagun Gupta

For many applications of pulsed radiation, the time-history of the radiation intensity must be optimized to induce a desired time-history of conditions. This optimization is normally performed using multi-physics simulations of the system.…

Computational Physics · Physics 2019-03-14 Damian C. Swift , George B. Zimmerman

Implementing a single qubit unitary is often hampered by imperfect control. Systematic amplitude errors $\epsilon$, caused by incorrect duration or strength of a pulse, are an especially common problem. But a sequence of imperfect pulses…

Quantum Physics · Physics 2014-10-02 Guang Hao Low , Theodore J. Yoder , Isaac L. Chuang

Accurate derivatives are important for efficiently locally traversing and converging in quantum optimization landscapes. By deriving analytically exact control derivatives (gradient and Hessian) for unitary control tasks, we show here that…

The proximal gradient algorithm has been popularly used for convex optimization. Recently, it has also been extended for nonconvex problems, and the current state-of-the-art is the nonmonotone accelerated proximal gradient algorithm.…

Optimization and Control · Mathematics 2017-05-24 Quanming Yao , James T. Kwok , Fei Gao , Wei Chen , Tie-Yan Liu

The past decade has demonstrated increasing interests in using optimal control based methods within coherent quantum controllable systems. The versatility of such methods has been demonstrated with particular elegance within nuclear…

Quantum Physics · Physics 2015-05-18 Ivan I. Maximov , Niels Chr. Nielsen , Julien Salomon , Gabriel Turinici

This paper investigates a category of constrained fractional optimization problems that emerge in various practical applications. The objective function for this category is characterized by the ratio of a numerator and denominator, both…

Optimization and Control · Mathematics 2026-05-28 Yizun Lin , Jian-Feng Cai , Zhao-Rong Lai , Cheng Li

Computation of derivatives (gradient and Hessian) of a fidelity function is one of the most crucial steps in many optimization algorithms. Having access to accurate methods to calculate these derivatives is even more desired where the…

Computational Physics · Physics 2020-03-05 Mohammadali Foroozandeh , Pranav Singh

Numerical optimal control (GRAPE) can in principle discover pulse shapes that suppress all coherent gate error to machine precision. But when does that capability actually matter? We present a systematic comparison of Gaussian, DRAG, and…

Quantum Physics · Physics 2026-02-16 Rylan Malarchick

Stochastic nonconvex optimization problems with nonlinear constraints have a broad range of applications in intelligent transportation, cyber-security, and smart grids. In this paper, first, we propose an inexact-proximal accelerated…

Optimization and Control · Mathematics 2021-07-08 Morteza Boroun , Afrooz Jalilzadeh

We propose new sequential simulation-optimization algorithms for general convex optimization via simulation problems with high-dimensional discrete decision space. The performance of each choice of discrete decision variables is evaluated…

Optimization and Control · Mathematics 2022-02-15 Haixiang Zhang , Zeyu Zheng , Javad Lavaei

We present a new family of min-max optimization algorithms that automatically exploit the geometry of the gradient data observed at earlier iterations to perform more informative extra-gradient steps in later ones. Thanks to this adaptation…

Optimization and Control · Mathematics 2020-11-20 Kimon Antonakopoulos , E. Veronica Belmega , Panayotis Mertikopoulos

We report analytical equations for the derivatives of spin dynamics simulations with respect to pulse sequence and spin system parameters. The methods described are significantly faster, more accurate and more reliable than the finite…

Chemical Physics · Physics 2015-05-14 Ilya Kuprov , Christopher T. Rodgers

We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

Numerically optimised microwave pulses are used to increase excitation efficiency and modulation depth in electron spin resonance experiments performed on a spectrometer equipped with an arbitrary waveform generator. The optimisation…

Chemical Physics · Physics 2018-10-19 David L. Goodwin , William K. Myers , Christiane R. Timmel , Ilya Kuprov

The gradients used to train neural networks are typically computed using backpropagation. While an efficient way to obtain exact gradients, backpropagation is computationally expensive, hinders parallelization, and is biologically…

Machine Learning · Computer Science 2026-01-14 Katharina Flügel , Daniel Coquelin , Marie Weiel , Charlotte Debus , Achim Streit , Markus Götz

This paper presents an algorithmic framework for solving unconstrained stochastic optimization problems using only stochastic function evaluations. We employ central finite-difference based gradient estimation methods to approximate the…

Optimization and Control · Mathematics 2025-01-14 Raghu Bollapragada , Cem Karamanli
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