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We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

We report extensive measurements on a new compound (Yb0.24Sn0.76)Ru that crystallizes in the cubic CsCl structure. Valence band photoemission and L3 x-ray absorption show no divalent component in the 4f configuration of Yb. Inelastic…

We use inelastic neutron scattering to study the crystalline electric field (CEF) excitations of Ce$^{3+}$ in CeFeAsO$_{1-x}$F$_{x}$($x=0,0.16$). For nonsuperconducting CeFeAsO, the Ce CEF levels have three magnetic doublets in the…

Frustrated quasidoublets without time-reversal symmetry can host highly unconventional magnetic structures with continuously distributed order parameters even in a single-phase crystal. Here, we report the comprehensive thermodynamic and…

The R3MBi5 rare-earth intermetallics (R = rare earth, M = Ti, Zr, Sc) provide a versatile platform to explore how Kondo hybridization, RKKY exchange, magnetic frustration, and broken inversion symmetry may cooperate to generate unusual…

We present the low-temperature magnetic properties of two Yb$^{3+}$-based triangular lattice compounds NaSrYb(BO$_3$)$_2$ and K$_3$YbSi$_2$O$_7$ via thermodynamic measurements followed by crystal electric field (CEF) calculations.…

Materials Science · Physics 2025-01-27 S. Guchhait , R. Kolay , A. Magar , R. Nath

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

Materials Science · Physics 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

We have measured crystalline electric field (CEF) excitations of Nd3+ ions in the two-channel Kondo lattice candidates NdT2Zn20 (T = Co, Rh, and Ir) by means of inelastic neutron scattering (INS). In the INS measurements at 5 K,…

Strongly Correlated Electrons · Physics 2023-02-15 Rikako Yamamoto , Manh Duc Le , Devashibhai T. Adroja , Yasuyuki Shimura , Toshiro Takabatake , Takahiro Onimaru

In this work, we explore experimentally and theoretically the spectrum of magnetic excitations of the Fe$^{3+}$ and Yb$^{3+}$ ions in ytterbium iron garnet (Yb$_3$Fe$_5$O$_{12}$). We present a complete description of the crystal-field…

Magnetic order in most materials occurs when magnetic ions with finite moments in a crystalline lattice arrange in a particular pattern below the ordering temperature determined by exchange interactions between the ions. However, when the…

We investigate the magnetic and crystal electric field (CEF) states of the Kondo lattice system CeCuGa3 by muon spin relaxation (muSR), neutron diffraction, and inelastic neutron scattering (INS) measurements. A noncentrosymmetric…

Time-of-flight neutron spectroscopy has been used to determine the crystalline electric field (CEF) Hamiltonian, eigenvalues and eigenvectors appropriate to the $J$ = 7/2 Yb$^{3+}$ ion in the candidate quantum spin ice pyrochlore magnet…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , D. D. Maharaj , G. Sala , E. Kermarrec , K. A. Ross , H. A. Dabkowska , A. I. Kolesnikov , G. E. Granroth , B. D. Gaulin

Inelastic neutron scattering measurement is performed on a breathing pyrochlore antiferromagnet Ba3Yb2Zn5O11. The observed dispersionless excitations are explained by a crystalline electric field (CEF) Hamiltonian of Kramers ion Yb3+ of…

Materials Science · Physics 2016-03-03 T. Haku , M. Soda , M. Sera , K. Kimura , S. Itoh , T. Yokoo , T. Masuda

Neutron scattering experiments have been performed on the ternary rare-earth diborocarbide Ce$^{11}$B$_2$C$_2$. The powder diffraction experiment confirms formation of a long-range magnetic order at $T_{\rm N} = 7.3$ K, where a sinusoidally…

Strongly Correlated Electrons · Physics 2009-11-13 Isao Nakanowatari , Rei Morinaga , Takahiro Onimaru , Taku J. Sato

We report studies of the Yb$^{3+}$ site distribution in Er$^{3+}$ co-doped upconverting alkaline earth fluoride nanoparticles using high-resolution absorption measurements. Similar to bulk crystals, Yb$^{3+}$ single ion cubic (O$_h$), and…

Materials Science · Physics 2020-04-30 Sangeetha Balabhadra , Michael F. Reid , Vladimir Golovko , Jon-Paul R. Wells

Here we present a neutron scattering-based study of magnetic excitations and magnetic order in NaYbO$_2$ under the application of an external magnetic field. The crystal electric field-split $J = 7/2$ multiplet structure is determined,…

Frustration, spin correlations and interplay between competing degrees of freedom are some of the key ingredients that underlie exotic states with fractional excitations in quantum materials. Rare-earth based two dimensional magnetic…

Strongly Correlated Electrons · Physics 2022-09-13 J. Khatua , M. Pregelj , A. Elghandour , Z. Jaglicic , R. Klingeler , A. Zorko , P. Khuntia

The Kondo lattice antiferromagnet YbNiSi3 was investigated by neutron scattering. The magnetic structure of YbNiSi3 was determined by neutron diffraction on a single-crystalline sample. Inelastic scattering experiments were also performed…

Thermodynamic and muon spin-relaxation measurements have recently highlighted BiYbGeO$_5$ as a new example of a rare-earth-based quantum dimer magnet with isolated Yb$^{3+}$ spin-$\frac{1}{2}$ dimers. However, direct spectroscopic evidence…

Strongly Correlated Electrons · Physics 2025-12-10 Rachit Kapoor , J. Ramirez Diaz , D. Yahne , V. O. Garlea , G. Hester

A spin-1/2 triangular-lattice antiferromagnet is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between geometric spin frustration and quantum fluctuations. It can…

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