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Highly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of…

We present a study of the Rydberg spectrum in \ts{166}Er for series connected to the $4f^{12} (^3H_6) 6s$, $J_c=13/2 $ and $J_c=11/2 $ ionic core states using an all-optical detection based on electromagnetically induced transparency in an…

Quantum information processing with neutral atoms relies on Rydberg excitation for entanglement generation. While the use of heavy divalent or open-shell elements, such as strontium or ytterbium, has benefits due to their optically active…

New measurements of high-lying even parity $6sns\, {}^1 \! S_0$ and $6snd\,{}^{3,1}\!D_2$ levels of neutral $^{174}$Yb are presented in this paper. Spectroscopy is performed by a two-step laser excitation from the ground state $4f^{14}6s^2…

Atomic Physics · Physics 2018-12-12 H. Lehec , A. Zuliani , W. Maineult , E. Luc-Koenig , P. Pillet , P. Cheinet , F. Niyaz , T. F. Gallagher

Rydberg atoms provide a powerful platform for exploring strongly interacting quantum systems, both in free space and in structured electromagnetic environments, with growing applications in quantum technology. Accurately modeling their…

Using the reactance matrix approach, we systematically develop new multichannel quantum defect theory models for the singlet and triplet S, P, D and F states of strontium based on improved energy level measurements. The new models reveal…

Atomic Physics · Physics 2014-07-17 C L Vaillant , M P A Jones , R M Potvliege

Neutral alkaline earth(-like) atoms have recently been employed in atomic arrays with individual readout, control, and high-fidelity Rydberg-mediated entanglement. This emerging platform offers a wide range of new quantum science…

Atomic Physics · Physics 2022-05-26 Neville Chen , Lintao Li , William Huie , Mingkun Zhao , Ian Vetter , Chris H. Greene , Jacob P. Covey

Rydberg electromagnetically induced transparency (EIT) enables realization of atom-based SI-traceable microwave (MW) sensing, imaging and communication devices by exploiting the strong microwave electric dipole coupling of highly excited…

Atomic Physics · Physics 2021-08-09 Aurélien Chopinaud , Jonathan D. Pritchard

The interactions between Rydberg atoms and microwave fields provide a valuable framework for studying the complex dynamics out of equilibrium, exotic phases, and critical phenomena in many-body physics. This unique interplay allows us to…

Neutral atoms in optical tweezer arrays possess broad applicability for quantum information science, in computing, simulation, and metrology. Among atomic species, Ytterbium-171 is unique as it hosts multiple qubits, each of which is…

Divalent atoms have emerged as powerful alternatives to alkalis in ultracold atom platforms, offering unique advantages arising from their two-electron structure. Among these species, ytterbium (Yb) is especially promising, yet its anionic…

Rydberg excited states of molecules pose a challenge for electronic structure calculations because of their highly diffuse electron distribution. Even large and elaborate atomic basis sets tend to underrepresent the long-range tail, overly…

Applicability of Rydberg atoms to quantum computers is examined from experimental point of view. In many theoretical proposals appeared recently, excitation of atoms into highly excited Rydberg states was considered as a way to achieve…

Quantum Physics · Physics 2007-05-23 Igor I. Ryabtsev , Denis B. Tretyakov , Ilya I. Beterov

We report an investigation of the low-lying excited states of the YbF molecule--a candidate molecule for experimental measurements of the electron electric dipole moment--with 2-component based multi-reference configuration interaction…

Chemical Physics · Physics 2023-09-18 Johann V. Pototschnig , Kenneth G. Dyall , Lucas Visscher , André S. P. Gomes

The Rydberg excitation blockade has been at the heart of an impressive array of recent achievements; however, state-mixing interactions can compromise its efficiency. When ultracold atoms are excited to Rydberg states near F\"orster…

Atomic Physics · Physics 2022-09-05 Milo Eder , Andrew Lesak , Abigail Plone , Tomohisa Yoda , Michael Highman , Aaron Reinhard

Atoms in highly excited (Rydberg) states have a number of unique properties which make them attractive for applications in quantum information. These are large dipole moments, lifetimes and polarizabilities, as well as strong long-range…

Quantum Physics · Physics 2016-05-25 I. I. Ryabtsev , I. I. Beterov , D. B. Tretyakov , V. M. Entin , E. A. Yakshina

We present an experimental system for Rydberg tweezer arrays with ytterbium (Yb) atoms featuring internal state manipulation between the ground ${}^1$S$_0$ and the metastable ${}^3$P$_2$ states, and single-photon excitation from the…

We report on a significant discrepancy between recently published highly accurate variational calculations and precise measurements of the spectrum of Rydberg states in $^{87}$Rb on the energy scale of fine splitting. Introducing a modified…

Quantum Physics · Physics 2016-08-07 Ali Sanayei , Nils Schopohl , Jens Grimmel , Markus Mack , Florian Karlewski , József Fortágh

In order to study ultracold charge-transfer processes in hybrid atom-ion traps, we have mapped out the potential energy curves and molecular parameters for several low lying states of the Rb, Yb$^+$ system. We employ both a multi-reference…

Atomic Physics · Physics 2013-05-30 H. D. L. Lamb , J. F. McCann , B. M. McLaughlin , J. Goold , N. Wells , I. Lane

We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…

Atomic Physics · Physics 2020-09-02 Andrew L. Hunter , Matthew T. Eiles , Alex Eisfeld , Jan M. Rost
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