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Van der Waals heterostructures formed by stacking two-dimensional atomic crystals are a unique platform for exploring new phenomena and functionalities. Interlayer excitons, bound states of spatially separated electron-hole pairs in van der…

Materials Science · Physics 2018-02-14 Zefang Wang , Yi-Hsin Chiu , Kevin Honz , Kin Fai Mak , Jie Shan

Interlayer excitons in semiconducting bilayers separated by insulating hBN layers constitute a promising platform for investigation of strongly correlated bosonic phases. Here, we report an optical method for the generation and…

Mesoscale and Nanoscale Physics · Physics 2025-10-13 Alperen Tüğen , Anna M. Seiler , Arthur Christianen , Kenji Watanabe , Takashi Taniguchi , Martin Kroner , Ataç İmamoğlu

Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission…

Mesoscale and Nanoscale Physics · Physics 2021-10-18 Alberto Ciarrocchi , Dmitrii Unuchek , Ahmet Avsar , Kenji Watanabe , Takashi Taniguchi , Andras Kis

We report robust room temperature interlayer excitons in transition metal dichalcogenide heterostructures engineered via precise stacking orientation and twist-angle control. We integrate 2H-stacked…

Exciton binding energies of hundreds of meV and strong light absorption in the optical frequency range make transition metal dichalcogenides (TMDs) promising for novel optoelectronic nanodevices. In particular, atomically thin TMDs can be…

Mesoscale and Nanoscale Physics · Physics 2018-04-24 Simon Ovesen , Samuel Brem , Christopher Linderälv , Mikael Kuisma , Paul Erhart , Malte Selig , Ermin Malic

Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

Mesoscale and Nanoscale Physics · Physics 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

Bilayer van der Waals (vdW) heterostructures such as MoS2/WS2 and MoSe2/WSe2 have attracted much attention recently, particularly because of their type II band alignments and the formation of interlayer exciton as the lowest-energy…

Mesoscale and Nanoscale Physics · Physics 2017-12-14 Shiyuan Gao , Li Yang , Catalin D. Spataru

Twisted van der Waals heterostructures and the corresponding superlattices, moire superlattices, are remarkable new material platforms, in which electron interactions and excited-state properties can be engineered. Particularly, the band…

Mesoscale and Nanoscale Physics · Physics 2019-11-13 Xiaobo Lu , Xiaoqin Li , Li Yang

Controlling interlayer excitons in van der Waals heterostructures holds promise for exploring Bose-Einstein condensates and developing novel optoelectronic applications, such as excitonic integrated circuits. Despite intensive studies,…

Mesoscale and Nanoscale Physics · Physics 2024-04-09 Lifu Zhang , Ruihao Ni , Liuxin Gu , Ming Xie , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , You Zhou

Van der Waals materials and heterostructures manifesting strongly bound room temperature exciton states exhibit emergent physical phenomena and are of a great promise for optoelectronic applications. Here, we demonstrate that nanostructured…

Identifying two-dimensional heterostructures with exceptional electronic and optical properties remains an active area of research in advanced optoelectronics. Here, we present a comprehensive first-principles investigation of the…

Recent measurements have shown that a continuously tunable bandgap of up to 250 meV can be generated in biased bilayer graphene [Y. Zhang et al., Nature 459, 820 (2009)], opening up pathway for possible graphene-based nanoelectronic and…

Materials Science · Physics 2010-02-11 Cheol-Hwan Park , Steven G. Louie

Optical resonators are a powerful platform to control the spontaneous emission dynamics of excitons in solid-state nanostructures. Here, we study a MoSe$_2$-WSe$_2$ van-der-Waals heterostructure that is integrated in a widely tunable open…

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal…

We explore a new platform for realising excitonic insulators, namely van der Waals (vdW) bilayers comprising 2D Janus materials. In previous studies, Type-II heterobilayers have been brought to the excitonic insulating regime by tuning the…

Mesoscale and Nanoscale Physics · Physics 2023-08-10 Fredrik Nilsson , Mikael Kuisma , Sahar Pakdel , Kristian S. Thygesen

Interlayer excitons (IXs), composed of electron and hole states localized in different layers, excel in bilayers composed of atomically thin van der Waals materials such as semiconducting transition metal dichalcogenides (TMDs) due to…

Mesoscale and Nanoscale Physics · Physics 2024-07-16 Mauro Brotons-Gisbert , Brian D. Gerardot , Alexander W. Holleitner , Ursula Wurstbauer

Our ability to efficiently detect and generate far-infrared (i.e., terahertz) radiation is vital in areas spanning from biomedical imaging to interstellar spectroscopy. Despite decades of intense research, bridging the terahertz gap between…

Materials Science · Physics 2023-07-24 Zhao Tang , Greis J. Cruz , Fanhao Jia , Yabei Wu , Weiyi Xia , Peihong Zhang

We demonstrate the possibility of engineering the optical properties of transition metal dichalcogenide heterobilayers when one of the constitutive layers has a Janus structure. This has important consequences for the charge separation…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 Engin Torun , Fulvio Paleari , Milorad V. Milosevic , Ludger Wirtz , Cem Sevik

Excitons dominate the optics of atomically-thin transition metal dichalcogenides and 2D van der Waals heterostructures. Interlayer 2D excitons, with an electron and a hole residing in different layers, form rapidly in heterostructures…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 M. G. Burdanova , M. Liu , M. Staniforth , Y. Zheng , R. Xiang , S. Chiashi , A. Anisimov , E. I. Kauppinen , S. Maruyama , J. Lloyd-Hughes

The fundamental properties of an exciton are determined by the spin, valley, energy, and spatial wavefunctions of the Coulomb bound electron and hole. In van der Waals materials, these attributes can be widely engineered through layer…

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