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We study theoretically and experimentally High Harmonic Generation (HHG) using two non collinear driving fields focused in gases. We show that these two fields form a non stationary blazed active grating in the generation medium. The…

Optics · Physics 2019-03-13 C. Chappuis , D. Bresteau , T. Auguste , O. Gobert , T. Ruchon

We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…

Optics · Physics 2025-07-15 Boyan Obreshkov , Tzveta Apostolova

High harmonic generation (HHG) in gaseous media provides a robust method for producing coherent extreme-ultraviolet (EUV) radiation and attosecond pulses. However, the spectral and temporal properties of these pulses -- such as bandwidth…

Quantum-mechanical investigation is presented to study single attosecond pulse generation by gating high-order harmonic emission from H$_2^+$ molecule in intense laser pulses with time-dependent ellipticity. The high-order harmonic…

Atomic Physics · Physics 2018-01-17 Nehzat Safaei

We study theoretically the effect of the giant resonance in Xe on the phase difference between the consecutive high order resonantly-enhanced harmonics and calculate the duration of the attosecond pulses produced by these harmonics. For…

Atomic Physics · Physics 2016-12-28 V. V. Strelkov

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

Attosecond pulses created by high-order harmonic generation in gases often exhibit strong chromatic aberrations, arising from the broad bandwidth and wavelength-dependent nonlinear light-matter interaction. When the driving laser intensity…

We report theoretical calculations of high-order harmonic generation (HHG) of Xe with the inclusion of multi-electron effects and macroscopic propagation of the fundamental and harmonic fields in an ionizing medium. By using the…

Atomic Physics · Physics 2011-10-11 Cheng Jin , Anh-Thu Le , Carlos A. Trallero-Herrero , C. D. Lin

A new regime in the interaction of a two-colour ($\omega$,$2\omega$) laser with a nanometre-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses - even in the case of multi-cycle lasers. For…

Plasma Physics · Physics 2020-04-22 Y. X. Zhang , S. Rykovanov , Mingyuan Shi , C. L. Zhong , X. T. He , B. Qiao , M. Zepf

Generating ever-shorter and brighter light pulses has long been a central pursuit in ultrafast science, as it benchmarks our ability to create and manipulate the coherence on the intrinsic timescale of sub-atomic electron motion. The…

High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…

Optics · Physics 2023-04-26 Liang Li , Pengfei Lan , Xiaosong Zhu , Peixiang Lu

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time)…

Atomic Physics · Physics 2019-09-04 Jan Troß , Georgios Kolliopoulos , Carlos A. Trallero-Herrero

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons…

Optics · Physics 2019-05-15 Martin Kozák , Norbert Schönenberger , Peter Hommelhoff

The interaction between relativistic electron beams and intense laser fields has been extensively studied for generating high-energy radiation. However, achieving coherent radiation from such interactions needs to precisely control the…

Plasma Physics · Physics 2025-09-01 H. Peng , T. W. Huang , C. N. Wu , K. Jiang , R. Li , C. Riconda , S. Weber , C. T. Zhou

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…

Chemical Physics · Physics 2022-11-07 Lorenzo Restaino , Deependra Jadoun , Markus Kowalewski
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