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Molecules intercalating two-dimensional (2D) materials form complex structures that have been mostly characterized by spatially averaged techniques. Here we use aberration-corrected scanning transmission electron microscopy and…

Recent intensive research on two-dimensional materials (2DMs) rekindle the interest in the intercalation of various atoms and molecules into layered compounds as a tool to manufacture 2DMs and tune their optoelectronic, magnetic and…

Mesoscale and Nanoscale Physics · Physics 2025-07-10 Arkady V. Krasheninnikov , Yung-Chang Lin , Kazu Suenaga

Ultrafast carrier dynamics of pristine bilayer graphene (BLG) and bilayer graphene intercalated with FeCl3 (FeCl3-G), were studied using time-resolved transient differential reflection (delta R/R). Compared to BLG, the FeCl3-G data showed…

Mesoscale and Nanoscale Physics · Physics 2010-10-12 Xingquan Zou , Da Zhan , Xiaofeng Fan , Dongwook Lee , Saritha K. Nair , Li Sun , Zhenhua Ni , Zhiqiang Luo , Lei Liu , Ting Yu , Zexiang Shen , Elbert E. M. Chia

Graphene is one of the most promising 2D materials for various applications due to its unique electronic properties and high thermal stability. In previous studies, it was shown that when graphene is deposited onto some transition metal…

Materials Science · Physics 2018-02-13 Tianbai Li , Jory A. Yarmoff

Modern nanoscience has focused on two-dimensional (2D) layer structure materials which have garnered tremendous attention due to their unique physical, chemical and electronic properties since the discovery of graphene in 2004. Recent…

Materials Science · Physics 2017-11-28 Srimanta Pakhira , Jose L. Mendoza-Cortes

Intercalation of two dimensional materials, particularly transition metal dichalcogenides, is a noninvasive way to modify electronic, optical and structural properties of these materials. However, research of these atomic-scale phenomena…

Crystallographic defects play a key role in determining the properties of crystalline materials. The new class of two-dimensional materials, foremost graphene, have enabled atomically resolved studies of defects, such as vacancies, grain…

Materials Science · Physics 2015-06-22 Ossi Lehtinen , Nilesh Vats , Gerardo Algara-Siller , Pia Knyrim , Ute Kaiser

The intercalation of metals beneath graphene offers a powerful route to stabilizing and protecting novel two-dimensional (2D) phases. The epitaxial growth of Pb monolayers on SiC(0001), combined with the relatively large spacing of the…

The interaction of metals with carbon materials, specifically with graphene, is of importance for various technological applications. In particular, intercalation of alkali metals is believed to provide a means for tuning the electronic…

Mesoscale and Nanoscale Physics · Physics 2023-01-26 Marianna Lorenzo , Conrad Escher , Tatiana Latychevskaia , Hans-Werner Fink

The AB-stacked bilayer graphene (BLG) is a pure semiconductor whose band gap and properties can be tuned by various methods such as doping or applying gate voltage. Here we show an alternative method to control the electronic properties of…

Materials Science · Physics 2017-02-06 Srimanta Pakhira , Kevin P. Lucht , Jose L. Mendoza-Cortes

Bilayer graphene (BLG) is semiconductor whose band gap and properties can be tuned by various methods such as doping or applying gate voltage. Here, we show how to tune electronic properties of BLG by intercalation of transition metal (TM)…

Materials Science · Physics 2018-03-14 Srimanta Pakhira , Kevin P. Lucht , Jose L. Mendoza-Cortes

The field of two-dimensional (2D) materials has expanded to multilayered systems where electronic, optical, and mechanical properties change-often dramatically-with stacking order, thickness, twist, and interlayer spacing [1-5]. For…

Materials Science · Physics 2019-06-27 Suk Hyun Sung , Noah Schnitzer , Lola Brown , Jiwoong Park , Robert Hovden

Intercalation of atomic species through epitaxial graphene layers began only a few years following its initial report in 2004. The impact of intercalation on the electronic properties of the graphene is well known; however, the intercalant…

We investigate the effects of lithium intercalation in twisted bilayers of graphene, using first-principles electronic structure calculations. To model this system we employ commensurate supercells that correspond to twist angles of…

Mesoscale and Nanoscale Physics · Physics 2020-02-11 Daniel T. Larson , Stephen Carr , Georgios A. Tritsaris , Efthimios Kaxiras

Intercalation of lithium atoms between layers of 2D materials can alter their atomic and electronic structure. We investigate effects of Li intercalation in twisted bilayers of the transition metal dichalcogenide MoS$_2$ through…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 Zheyu Lu , Stephen Carr , Daniel T. Larson , Efthimios Kaxiras

Properties of many layered materials, including copper- and iron-based superconductors, topological insulators, graphite and epitaxial graphene can be manipulated by inclusion of different atomic and molecular species between the layers via…

Graphene has attracted great attentions since its first discovery in 2004. Various approaches have been proposed to control its physical and electronic properties. Here, we report that graphene based intercalation compounds is an efficient…

Materials Science · Physics 2010-11-04 Da Zhan , Li Sun , Zhenhua Ni , Lei Liu , Xiaofeng Fan , Yingying Wang , Ting Yu , Yeng Ming Lam , Wei Huang , Zexiang Shen

Intercalation materials are promising candidates for reversible energy storage and are, for example, used as lithium-battery electrodes, hydrogen-storage compounds, and electrochromic materials. An important issue preventing the more…

Materials Science · Physics 2022-04-12 Ananya Renuka Balakrishna

Point defects give rise to sharp modifications in the structures and electronic properties of two-dimensional metals, offering an atomic-level platform for fundamental studies and potential applications. In this work, we investigate…

Mesoscale and Nanoscale Physics · Physics 2026-02-05 Van Dong Pham , Arpit Jain , Chengye Dong , Li-Syuan Lu , Joshua A. Robinson , Achim Trampert , Roman Engel-Herbert

In this work, we perform ab initio calculations, based on the density functional theory, of the effects on the graphene bilayer when we intercalate carbon atoms between the layers. We use the unit cell of the bilayer to construct larger…

Mesoscale and Nanoscale Physics · Physics 2020-01-31 A. K. M. Pinto , N. F. Frazão , D. L. Azevedo , F. Moraes
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