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We investigate the properties of a system of semi-diluted polymers in the presence of charged groups and counter-ions, by means of self-consistent field theory. We study a system of polyelectrolyte chains grafted to a similarly, as well as…

Soft Condensed Matter · Physics 2015-05-19 Gabriele Migliorini

Self-diffusion of a polymer chain in a melt is studied by Monte Carlo simulations of the bond fluctuation model, where only the excluded volume interaction is taken into account. Polymer chains, each of which consists of $N$ segments, are…

Soft Condensed Matter · Physics 2009-11-10 Katsumi Hagita , Hiroshi Takano

The equilibrium phase behaviour of hard spheres with size polydispersity is studied theoretically. We solve numerically the exact phase equilibrium equations that result from accurate free energy expressions for the fluid and solid phases,…

Soft Condensed Matter · Physics 2007-05-23 M. Fasolo , P. Sollich

We study the equilibrium behaviour of a mixture of monodisperse hard sphere colloids and polydisperse non-adsorbing polymers at their $\theta$-point, using the Asakura-Oosawa model treated within the free-volume approximation. Our focus is…

Soft Condensed Matter · Physics 2007-05-23 Moreno Fasolo , Peter Sollich

The folding transition of single, long semiflexible polymers was studied with special emphasis on the chain length effect using Monte Carlo simulations. While a relatively short chain (10-25 Kuhn segments) undergoes a large discrete…

Soft Condensed Matter · Physics 2008-05-06 Yuji Higuchi , Takahiro Sakaue , Kenichi Yoshikawa

We present Monte Carlo simulations of semidilute solutions of long self-attracting chain polymers near their Ising type critical point. The polymers are modeled as monodisperse self-avoiding walks on the simple cubic lattice with attraction…

Soft Condensed Matter · Physics 2009-10-30 H. Frauenkron , P. Grassberger , HLRZ Juelich , Germany

Synthetic polymers have a distribution of chain lengths which can be characterized by dispersity, D. Macroscopic properties of polymers are influenced by chain mobility in the melt and manipulating D can significantly impact these…

Chemical Physics · Physics 2024-09-30 Taofeek Tejuosho , Sohil Kollipara , Sumant Patankar , Janani Sampath

Diffusion properties of a self-avoiding polymer embedded in regularly distributed obstacles with spacing a=20 and confined in two dimensions is studied numerically using the extended bond fluctuation method which we have developed recently.…

Soft Condensed Matter · Physics 2009-10-31 Ryuzo Azuma , Hajime Takayama

We study irreversible polymer adsorption from dilute solutions theoretically. Universal features of the resultant non-equilibrium layers are predicted. Two cases are considered, distinguished by the value of the local monomer-surface…

Soft Condensed Matter · Physics 2009-11-10 Ben O'Shaughnessy , Dimitrios Vavylonis

A self consistent field theory for compressible polymer mixtures is developed by introducing elements of classical density functional theory into the framework of the Helfand theory. It is then applied to study free surfaces of binary (A,B)…

Condensed Matter · Physics 2009-10-28 F. Schmid

Using molecular dynamics simulation of a standard bead-spring model we investigate the density crossover scaling of strictly two-dimensional self-avoiding polymer chains focusing on properties related to the contact exponent set by the…

Soft Condensed Matter · Physics 2015-06-03 N. Schulmann , H. Meyer , J. P. Wittmer , A. Johner , J. Baschnagel

We present results of Monte Carlo study of the monomer-monomer correlation functions, static structure factor and asphericity characteristics of a single homopolymer in the coil and globular states for three distinct architectures of the…

Soft Condensed Matter · Physics 2009-11-07 Edward G. Timoshenko , Yuri A. Kuznetsov , Ronan Connolly

We investigate interfacial properties between two highly incompatible polymers of different stiffness. The extensive Monte Carlo simulations of the binary polymer melt yield detailed interfacial profiles and the interfacial tension via an…

Statistical Mechanics · Physics 2009-10-30 Marcus Mueller , Andreas Werner

The conformational properties of a semi-flexible polymer chain, anchored at one end in a uniform force field, are studied in a simple two-dimensional model. Recursion relations are derived for the partition function and then iterated…

Soft Condensed Matter · Physics 2009-11-07 A. Lamura , T. W. Burkhardt , G. Gompper

We use an off-lattice microscopic model for solutions of equilibrium polymers (EP) in a lamellar shear flow generated by means of a self-consistent external field between parallel hard walls. The individual conformations of the chains are…

Soft Condensed Matter · Physics 2009-10-31 A. Milchev , J. P. Wittmer , D. P. Landau

The conditions of multi-phase equilibrium are solved for generic polydisperse systems. The case of multiple polydispersity is treated, where several properties (e.g. size, charge, shape) simultaneously vary from one particle to another. By…

Statistical Mechanics · Physics 2009-10-31 R. M. L. Evans

We simulate structural phase behavior of polymer-grafted colloidal particles by molecular Monte Carlo technique. Interparticle potential, which has a finite repulsive square-step outside a rigid core of the colloid, was previously confirmed…

Soft Condensed Matter · Physics 2015-03-19 Yuki Norizoe , Toshihiro Kawakatsu

We generalize a recently investigated lattice model of semiflexible polymers formed under equilibrium polymerization in a solution and conduct a comprehensive investigation of its melting properties. The model is characterized by six…

Condensed Matter · Physics 2007-05-23 Sagar S. Rane , P. D. Gujrati

Periodic configurations of electrodes, in particular of microelectrodes, have been of interest since the advent of microfabrication. In this report, theory which is common to any periodic cell (or any cell that can be extended periodically)…

Chemical Physics · Physics 2018-02-13 Cristian F. Guajardo Yévenes , Werasak Surareungchai

The ground-state properties of two-component repulsive Fermi gases in two dimensions are investigated by means of fixed-node diffusion Monte Carlo simulations. The energy per particle is determined as a function of the intercomponent…

Quantum Gases · Physics 2021-06-23 S. Pilati , G. Orso , G. Bertaina