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We theoretically study high-harmonic generation (HHG) from transition metal elements Mn and Mn$^+$, using full-dimensional, all-electron, first-principles simulations. The HHG spectra calculated with the time-dependent complete-active-space…

Atomic Physics · Physics 2019-06-26 Imam S. Wahyutama , Takeshi Sato , Kenichi L. Ishikawa

High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…

Optics · Physics 2018-04-26 Dieter Bauer , Kenneth K. Hansen

High harmonic generation (HHG) is used to measure the spectral phase of the recombination dipole matrix element (RDM) in argon over a broad frequency range that includes the 3p Cooper minimum (CM). The measured RDM phase agrees well with…

Atomic Physics · Physics 2015-06-17 S. B. Schoun , R. Chirla , J. Wheeler , C. Roedig , P. Agostini , L. F. DiMauro , K. J. Schafer , M. B. Gaarde

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We investigate the feasibility of using high-harmonic generation (HHG) as a complementary probe of tunneling delay in strong-field ionization. By combining time--frequency analysis of HHG spectra obtained from full time-dependent…

Atomic Physics · Physics 2026-01-15 Amol R. Holkundkar

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

Optics · Physics 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

Atomic Physics · Physics 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. We perform the first temporal…

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian

We employ the R-matrix with time-dependence method to investigate extreme-ultraviolet-initiated high-harmonic generation (XIHHG) in Ar$^{+}$. Using a combination of extreme-ultraviolet (XUV, $92\textrm{ nm}$, $3\times…

Atomic Physics · Physics 2018-03-14 D. D. A. Clarke , H. W. van der Hart , A. C. Brown

High harmonic generation (HHG) is a striking phenomenon, which reflects the ultrafast dynamics of electrons. Recently, it has been demonstrated that HHG can be used to reconstruct not only the energy band structure but also the geometric…

Mesoscale and Nanoscale Physics · Physics 2024-09-10 Atsushi Ono , Shun Okumura , Shohei Imai , Yutaka Akagi

By employing the exact diagonalization method, we investigate the high-harmonic generation (HHG) of the correlated systems under the strong laser irradiation. For the extended Hubbard model on a periodic chain, HHG close to the quantum…

Strongly Correlated Electrons · Physics 2022-03-07 Can Shao , Hantao Lu , Xiao Zhang , Chao Yu , Takami Tohyama , Ruifeng Lu

A calculation of the high-harmonic generation (HHG) in $\alpha$-quartz using the time-dependent density functional theory is reported. The inter-band process is attributed to the dominant in HHG above the band gap. The photon energy is set…

Optics · Physics 2017-01-04 T. Otobe

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

We find that a donor-doped band-gap material can enhance the overall high-order harmonic generation (HHG) efficiency by several orders of magnitude, compared with undoped and acceptor-doped materials. This significant enhancement, predicted…

Optics · Physics 2019-01-30 Chuan Yu , Kenneth K. Hansen , Lars Bojer Madsen
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