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Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

The direct measurement of Berry phases is still a great challenge in condensed matter systems. The bottleneck has been the ability to adiabatically drive an electron coherently across a large portion of the Brillouin zone in a solid where…

Using reflective cross-polarized 2D THz time-domain spectroscopy in the range of 1-12 THz, we follow the trajectory of the out-of-equilibrium electron population in the low-bandgap semiconductor InSb. The 2D THz spectra show a set of…

Strongly Correlated Electrons · Physics 2019-06-10 S. Houver , L. Huber , M. Savoini , E. Abreu , S. L. Johnson

Second-order nonlinear optical responses, including photogalvanic effect (PGE) and second harmonic generation (SHG), are important physical phenomena in nonlinear optics. The PGE (SHG) related to linearly and circularly polarized light are…

Mesoscale and Nanoscale Physics · Physics 2023-06-01 Yuan Liu , Zhen-Gang Zhu , Gang Su

Using a hydrodynamic approach we examine bulk- and surface-induced second and third harmonic generation from semiconductor nanowire gratings having a resonant nonlinearity in the absorption region. We demonstrate resonant, broadband and…

Spatio-temporal mode coupling in highly multimode physical systems permits new routes for exploring complex instabilities and forming coherent wave structures. We present here the first experimental demonstration of multiple geometric…

Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…

Optics · Physics 2013-09-17 B. U. Felderhof , G. Marowsky

Numerical simulations based on the quantum Langevin equations have been performed for a large number of two-level atoms in a beam interacting with a low-Q cavity with the atomic initial superposition states close to the north pole of the…

Quantum Physics · Physics 2024-08-20 Mingyu Jeon , Jinuk Kim , Kyungwon An

The magneto-optical longitudinal, transverse Hall and circularly-polarized response of silicene and other materials described by a Kane-Mele Hamiltonian are calculated. Particular attention is paid to the effects of an external electric…

Mesoscale and Nanoscale Physics · Physics 2013-08-29 Calvin J. Tabert , Elisabeth J. Nicol

Recent advances in electron microscopy trigger the question whether attosecond electron diffraction can resolve atomic-scale electron dynamics in crystalline materials in space and time. Here we explore the physics of the relevant…

Atomic Physics · Physics 2026-05-08 Yuya Morimoto , Peter Baum

We compute from first principles the infrared dispersion of the nonlinear susceptibility $\chi^{(2)}$ in zincblende semiconductors. At terahertz frequencies the nonlinear susceptibility depends not only on the purely electronic response…

Materials Science · Physics 2009-12-17 Eric Roman , Jonathan R. Yates , Marek Veithen , David Vanderbilt , Ivo Souza

We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We…

Mesoscale and Nanoscale Physics · Physics 2012-02-15 Pablo M. Jais , Catalina von Bilderling , Andrea V. Bragas

Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. Tailoring phase and amplitude of a nonlinearly generated wave with a high emission efficiency using…

Optics · Physics 2022-10-03 David Hähnel , Jens Förstner , Viktor Myroshnychenko

High-order sideband generation (HSG), as an analogue of the interband processes in high-harmonic generation (HHG) in solids, is a nonperturbative nonlinear optical phenomenon in semiconductors that are simultaneously driven by a relatively…

Optics · Physics 2023-05-31 Qile Wu , Mark S. Sherwin

Structural engineering techniques such as local strain engineering and folding provide functional control over critical optoelectronic properties of 2D materials. Accurate monitoring of local strain vector (both strain amplitude and…

Nonlinear frequency conversion provides essential tools for light generation, photon entanglement, and manipulation. Transition metal dichalcogenides (TMDs) possess huge nonlinear susceptibilities and 3R-stacked TMD crystals further combine…

We developed a novel technique for frequency measurement and synthesis, based on the operation of a femtosecond comb generator as transfer oscillator. The technique can be used to measure frequency ratios of any optical signals throughout…

Optics · Physics 2009-11-07 Jörn Stenger , Harald Schnatz , Christian Tamm , Harald R. Telle

Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium…

The nonlinear photoacoustic response of indium phosphide nanocrystals on silicon nanotip arrays is investigated using time-resolved optical pump-probe spectroscopy and synchrotron-based X-ray diffraction. Femtosecond laser excitation…

We show that nonlinear dynamics in diode lasers with optical injection leads to frequency tunable microwave sidebands which are suitable for atomic physics experiments. We demonstrate the applicability of the sidebands in an experiment…

Atomic Physics · Physics 2012-07-24 C. I. Laidler , S. Eriksson