Related papers: Confocal Raman microscopy inside sessile multicomp…
The internal flow within an evaporating sessile droplet is one of the driving mechanisms that lead to the variety of particle deposition patterns seen in applications such as inkjet printing, surface patterning, and blood stain analysis.…
Raman transitions have a wide range of applications in atomic physics and have recently been proposed as a means for improving high-precision high-voltage measurements. Here, we present a theoretical analysis and a first experimental…
Droplets abound in nature and technology. In general, they are multicomponent, and, when out of equilibrium, with gradients in concentration, implying flow and mass transport. Moreover, phase transitions can occur, with either evaporation,…
Here we design, construct, and characterize a compact Raman-spectroscopy-based sensor that measures the concentration of a water-methanol mixture. The sensor measures the concentration with an accuracy of 0.5% and a precision of 0.2% with a…
In the field of microdroplet manipulation, optical tweezers have been used to form and grow droplets, to transport them, or to measure forces between droplet pairs. However, the exploration of out-of-equilibrium phenomena in optically…
Confocal Raman microscopy offers a particular pathway for monitoring chemical "fingerprints" of intracellular components like the cell membrane, organelles, and nucleus. Nevertheless, conventional Raman acquisitions of fixed or randomly…
Due to the potential application of regulating droplet shape by external fields in microfluidic technology and micro devices, it becomes increasingly important to understand the shape formation of a droplet in the presence of an electric…
The occurrence of concentration and temperature gradients in saline microdroplets evaporating directly in air makes them unsuitable for nucleation studies where homogeneous composition is required. This can be addressed by immersing the…
Raman spectroscopy is an integral part of graphene research. It is used to determine the number and orientation of layers, the quality and types of edge, and the effects of perturbations, such as electric and magnetic fields, strain,…
Raman spectroscopy is a powerful experimental technique for characterizing molecules and materials that is used in many laboratories. First-principles theoretical calculations of Raman spectra are important because they elucidate the…
We have employed the method of spectral moments to study the density of vibrational states and the Raman coupling coefficient of large 2- and 3- dimensional percolators at threshold and at higher concentration. We first discuss the over-and…
In microfluidic systems, droplets undergo intricate deformations as they traverse flow-focusing junctions, posing a challenging task for accurate measurement, especially during short transit times. This study investigates the physical…
Evaporating suspensions of colloidal particles lead to the formation of a variety of patterns, ranging from a left-over ring of a dried coffee drop to uniformly distributed solid pigments left behind wet paint. To characterize the…
Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…
Droplet-droplet interactions is ubiquitous in various applications ranging from medical diagnostics to enhancing and optimizing liquid jet propulsion. We employ an experimental technique where the laser pulse interacts with a micron-sized…
Molecular adsorption on surfaces plays a central role in catalysis, corrosion, desalination, and many other processes of relevance to industry and the natural world. Few adsorption systems are more ubiquitous or of more widespread…
In a retroreflective scheme atomic Raman diffraction adopts some of the properties of Bragg diffraction due to additional couplings to off-resonant momenta. As a consequence, double Raman diffraction has to be performed in a Bragg-type…
It is demonstrated that measurements of positions of atoms scattered from a quasi-condensate in a Raman process provide information on the temperature of the parent cloud. In particular, the widths of the density and second order…
A theoretical framework is presented that permits investigations of the relation between inelastic backscattering from microparticles and bulk samples of Raman-active materials. It is based on the Lorentz reciprocity theorem and no…
Vaporization of low-boiling point droplets has numerous applications in combustion, process engineering and in recent years, in clinical medicine. However, the physical mechanisms governing the phase conversion are only partly explained.…