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The crystal structure and phonon dynamics of pentacene is computed with the Quasi Harmonic Lattice Dynamics (QHLD) method, based on atom-atom potential. We show that two crystalline phases of pentacene exist, rather similar in thermodynamic…

We study the structural effects produced by the quantization of vibrational degrees of freedom in periodic crystals at zero temperature. To this end we introduce a methodology based on mapping a suitable subspace of the vibrational manifold…

Materials Science · Physics 2009-11-13 I. Scivetti , N. I. Gidopoulos , J. Kohanoff

We present a theory of finite-frequency noise in non-equilibrium conductors. It is shown that Non-Markovian correlations are essential to describe the physics of quantum noise. In particular, we show the importance of a correct treatment of…

Mesoscale and Nanoscale Physics · Physics 2011-04-01 D. Marcos , C. Emary , T. Brandes , R. Aguado

We generalize a proposal for detecting single phonon transitions in a single nanoelectromechanical system (NEMS) to include the intrinsic anharmonicity of each mechanical oscillator. In this scheme two NEMS oscillators are coupled via a…

Quantum Physics · Physics 2009-11-10 D. H. Santamore , Hsi-Sheng Goan , G. J. Milburn , M. L. Roukes

We study the effect of quantum vibronic coupling on the electronic properties of carbon allotropes, including molecules and solids, by combining path integral first principles molecular dynamics (FPMD) with a colored noise thermostat. In…

Materials Science · Physics 2021-08-04 Arpan Kundu , Marco Govoni , Han Yang , Michele Ceriotti , Francois Gygi , Giulia Galli

We study thermal transport in a chain of coupled atoms, which can vibrate in longitudinal as well as transverse directions. The particles interact through anharmonic potentials upto cubic order. The problem is treated quantum mechanically.…

Statistical Mechanics · Physics 2010-04-19 Santhosh G , Deepak Kumar

We present a quantum algorithm for calculating the vibronic spectrum of a molecule, a useful but classically hard problem in chemistry. We show several advantages over previous quantum approaches: vibrational anharmonicity is naturally…

Quantum Physics · Physics 2019-08-02 Nicolas P. D. Sawaya , Joonsuk Huh

We apply the classical field method to simulate the production of correlated atoms during the collision of two Bose-Einstein condensates. Our non-perturbative method includes the effect of quantum noise, and provides for the first time a…

Soft Condensed Matter · Physics 2009-11-10 A. A. Norrie , R. J. Ballagh , C. W. Gardiner

We apply modern techniques from quantum optics and quantum information science to Bose-Einstein Condensates (BECs) in order to study, for the first time, the quantum decoherence of phonons of isolated BECs. In the last few years, major…

Quantum Physics · Physics 2017-12-13 R. Howl , Carlos Sabín , Lucia Hackermüller , Ivette Fuentes

We compute the high-frequency emission and absorption noise in a fractional quantum Hall effect (FQHE) sample at arbitrary temperature. We model the edges of the FQHE as chiral Luttinger liquids (LL) and we use the non-equilibrium…

Strongly Correlated Electrons · Physics 2009-11-13 Cristina Bena , Ines Safi

Molecules like water have vibrational modes with a zero-point energy well above room temperature. As a consequence, classical molecular dynamics simulations of their liquids largely underestimate the energy of modes with a higher zero-point…

Statistical Mechanics · Physics 2013-05-08 Sriram Ganeshan , Rafael Ramírez , M. V. Fernández-Serra

We investigate the effects of a low frequency (acoustic) phonon bath on the dynamics of a quantum dot modelled as a cascade three-level system. We show that the phonon bath appears to the upper transition of the cascade system as a…

Quantum Physics · Physics 2014-08-27 Hui Huang , Gao-xiang Li , Wen-ju Gu , Zbigniew Ficek

The breakdown of the quasiparticle approximation (QPA) for phonons in strongly anharmonic materials necessitates advanced first-principles frameworks for accurate lattice dynamics and thermal transport predictions. We develop a…

Materials Science · Physics 2025-12-23 Yi Xia

We investigate the structural and thermodynamic properties of high-pressure ice by incorporating quantum anharmonicity at a non-perturbative level. Quantum fluctuations reduce the critical pressure of the phase transition between phase VIII…

Other Condensed Matter · Physics 2024-03-15 Marco Cherubini , Lorenzo Monacelli , Bingjia Yang , Roberto Car , Michele Casula , Francesco Mauri

External coherent fields can drive quantum materials into non-equilibrium states, revealing exotic properties that are unattainable under equilibrium conditions -- an approach known as ``Floquet engineering.'' While optical lasers have…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Christopher Yang , Will Hunt , Gil Refael , Iliya Esin

The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely…

A new formulation is presented to treat thermal and quantum fluctuations around the kaon condensate on the basis of chiral symmetry; separating the zero-mode from the beginning and using the path-integral method, we can formulate the…

Nuclear Theory · Physics 2009-10-31 Toshitaka Tatsumi , Masatomi Yasuhira

Previous studies in quantum information have recognized that specific types of noise can encode information in certain applications. However, the role of noise in Quantum Hypothesis Testing (QHT), traditionally assumed to undermine…

Quantum Physics · Physics 2024-08-06 Qing Li , Lingna Wang , Min Jiang , Ze Wu , Haidong Yuan , Xinhua Peng

We study the impact of phonon anharmonicity on the electronic dynamics of soft materials using a nonperturbative quantum-classical approach. The method is applied to a one-dimensional model of doped organic semiconductors with low-frequency…

Materials Science · Physics 2025-09-24 Jonathan H. Fetherolf , Petra Shih , Timothy C. Berkelbach

Based on thermodynamic principles, we derive expressions quantifying the non-harmonic vibrational behavior of materials, which are rigorous yet easily evaluated from experimentally available data for the thermal expansion coefficient and…

Materials Science · Physics 2016-07-29 Dipanshu Bansal , Amjad Aref , Gary Dargush , Olivier Delaire