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Using the Hubbard model we study how the process of high-order harmonic generation (HHG) is modified by beyond mean-field electron-electron correlation for both finite and bulk systems. A finite-size enhancement of the HHG signal is found…

Atomic Physics · Physics 2022-06-01 Thomas Hansen , Simon Vendelbo Bylling Jensen , Lars Bojer Madsen

Quantum-optical descriptions of strong-field processes have attracted significant attention in recent years. Typically, the theoretical modeling has been conducted in the Schr\"odinger picture, where results are only obtainable under…

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

Nonadiabatic corrections in molecules composed of a few atoms are considered. It is demonstrated that a systematic perturbative expansion around the adiabatic solution is possible, with the expansion parameter being the electron-nucleus…

Chemical Physics · Physics 2009-11-13 Krzysztof Pachucki , Jacek Komasa

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems…

We perform a Bohmian-trajectory analysis of high-order harmonic generation (HHG), focusing on the fact that typical HHG spectra are best reproduced by the Bohmian trajectory starting at the innermost part of the core [Phys. Rev. A…

Atomic Physics · Physics 2013-12-30 J. Wu , B. B. Augstein , C. Figueira de Morisson Faria

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

Atomic Physics · Physics 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…

Other Condensed Matter · Physics 2019-07-26 Francisco Navarrete , Marcelo F. Ciappina , Uwe Thumm

High-order harmonic generation (HHG) provides a broad spectral bandwidth for synthesizing attosecond pulses. However, in the current HHG schemes, only part of the harmonics can be phase-locked, which limits the ability to achieve shorter…

Optics · Physics 2024-06-18 ShiJun Wang , XuanYang Lai , XiaoJun Liu

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

One key parameter in the high-order harmonic generation (HHG) phenomenon is the exact frequency of the generated harmonic field. Its deviation from perfect harmonics of the laser frequency can be explained considering (i) the single-atom…

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

Recently it was shown [A. Gordon and F. X. Kaertner, Phys. Rev. Lett. 95, 223901 (2005)] that the strong field approximation (SFA) for high-order harmonic generation (HHG) is significantly improved when the SFA wave function is used with…

Optics · Physics 2007-05-23 Ariel Gordon , Franz X. Kaertner

We study the tunneling mechanism of nonlinear optical processes in solids induced by strong coherent laser fields. The theory is based on an extension of the Landau-Zener model with nonadiabatic geometric effects. In addition to the…

Mesoscale and Nanoscale Physics · Physics 2021-10-15 Shintaro Takayoshi , Jianda Wu , Takashi Oka

We extend the existing framework of macroscopic HHG to combine it with high-accuracy ab initio calculations for molecules as microscopic input. This approach is applied to HHG spectra exhibiting Mollow sidebands, for open shell molecules…

Chemical Physics · Physics 2025-08-13 T Joyce , A. Jaron

The comparison study of high pressure superconducting state of recently synthesized H$_3$S and PH$_3$ compounds are conducted within the framework of the strong-coupling theory. By generalization of the standard Eliashberg equations to…

Superconductivity · Physics 2017-07-05 Artur P. Durajski

We study above-threshold ionization (ATI) of atoms in strong elliptical laser fields numerically and analytically. Recent benchmark experiments for H showed that the attoclock offset angle related to each ATI ring increases remarkably with…

Atomic Physics · Physics 2026-01-12 Jia'nan Wu , Shiqi Shen , Jiayin Che , Shang Wang , Weiyan Li , Guoguo Xin , Yanjun Chen

High harmonic generation(HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gasses and semiconductors. It has attracted much attention because of its…

Optics · Physics 2023-09-08 Akira Kofuji , Robert Peters

We consider the interaction of gapped graphene in the two-band approximation using an explicit time-dependent approach. In addition to the full high-order harmonic generation (HHG) spectrum, we also obtain the perturbative harmonic response…

Materials Science · Physics 2017-02-01 Darko Dimitrovski , Lars Bojer Madsen , Thomas Garm Pedersen

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu