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A family of unusually stable boron cages was identified and examined using first-principles local density functional method. The structure of the fullerenes is similar to that of the B12 icosahedron and consists of six crossing…

Materials Science · Physics 2021-09-21 Nevill Gonzalez Szwacki

Two-dimensional boron monolayer (borophene) stands out from the two-dimensional atomic layered materials due to its structural flexibility, tunable electronic and mechanical properties from a large number of allotropic materials. The…

Materials Science · Physics 2022-05-31 Yuchong Kang , Xiaoyun Ma , Jing Fu , Kun Yang , Zongguo Wang , Haibo Li , Wei Ma , Jin Zhang

The recent discovery of borophene, a two-dimensional allotrope of boron, raises many questions about its structure and its chemical and physical properties. Boron has a high chemical affinity to oxygen but little is known about the…

Materials Science · Physics 2020-02-28 Florian M. Arnold , Gotthard Seifert , Jens Kunstmann

Rhombohedral B$_{12}$ unit is viewed as a host matrix embedding linear tri-atomic arrangements of elements (E) resulting in a relatively large family of boron-rich compounds with B$_{12}${E-E-E} generic formulation. The present work focuses…

Materials Science · Physics 2021-01-13 Samir F. Matar , Vladimir L. Solozhenko

We present novel structural motifs for boron-carbon nano-cages of the stochiometries B12C48 and B12C50, based on first principle calculations. These configurations are distinct from those proposed so far by the fact that the boron atoms are…

Two-dimensional (2D) boron-based materials have gained increasing interest due to their exceptional physicochemical properties and potential technological applications. In this way, borospherenes, a 2D Boron-based fullerene-like lattice…

Two-dimensional boron sheets (borophenes) have been successfully synthesized in experiments and are expected to exhibit intriguing transport properties such as the emergence of superconductivity and Dirac Fermions. However, quantitative…

Computational Physics · Physics 2020-07-28 Jin Zhang , Jia Zhang , Cai Cheng , Jian Liu , Johannes Lischner , Feliciano Giustino , Sheng Meng

Boron is the fifth element in the periodic table and possesses rich chemistry second only to carbon. A striking feature of boron is that B12 icosahedral cages occur as the building blocks in bulk boron and many boron compounds. This is in…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 Baojie Feng , Jin Zhang , Qing Zhong , Wenbin Li , Shuai Li , Hui Li , Peng Cheng , Sheng Meng , Lan Chen , Kehui Wu

We have built an ab-initio LDA energy database with over 60 hypothetical extended structures of pure Boron, in each of which the coordination environment of each atom is equivalent. Focusing on eleven 6-coordinated structures, which are…

Materials Science · Physics 2007-05-23 Wei-Jing Zhu , Christopher L. Henley

A set of general constructing schemes is unveiled to predict a large family of stable boron monoelemental, hollow fullerenes with magic numbers 32+8k (k>=0). The remarkable stabilities of these new boron fullerenes are then studied by…

Materials Science · Physics 2009-11-13 Qing-Bo Yan , Xian-Lei Sheng , Qing-Rong Zheng , Li-Zhi Zhang , Gang Su

By means of ab initio calculations within the density functional theory, we have found that B80 fullerenes can condense to form stable face-centered-cubic fcc solids. It is shown that when forming a crystal, B80 cages are geometrically…

Materials Science · Physics 2009-11-13 Qing-Bo Yan , Qing-Rong Zheng , Gang Su

In this study, we employ density functional theory (DFT) to investigate the structural and electronic properties B$_8$Cu$_3^-$ clusters -- boron-based frameworks doped with three copper atoms. The results indicate that the lowest-energy…

Materials Science · Physics 2025-05-22 P. L. Rodríguez-Kessler

We investigate the stability of boron fullerene sets B76, B78 and B82. We evaluate the ground state energies, nucleus-independent chemical shift (NICS), the binding energies per atom and the band gap values by means of first-principles…

Materials Science · Physics 2017-09-13 Serkan Polad , Mete Ozay

The effect of external static charging on borophenes - 2D boron crystals - is investigated by using first principles calculations. The influence of the excess negative charge on the stability of the 2D structures is examined using a very…

Materials Science · Physics 2021-09-21 T. Tarkowski , J. A. Majewski , N. Gonzalez Szwacki

Molybdenum borides were studied theoretically using first-principles calculations, empirical total energy model and global optimization techniques to determine stable crystal structures. Our calculations reveal the structures of known Mo-B…

Materials Science · Physics 2020-03-10 Dmitry V. Rybkovskiy , Alexander G. Kvashnin , Yulia A. Kvashnina , Artem R. Oganov

We investigate the symmetry of the boron buckyball and a related boron nanotube. Using large-scale ab-initio calculations up to second-order M{\o}ller Plesset perturbation theory, we have determined unambiguously the equilibrium…

Materials Science · Physics 2015-05-14 N. Gonzalez Szwacki , C. J. Tymczak

We present results of computer simulations of amorphous Si3B3N7 ceramics. The computed pair correlation functions are in agreement with the experimental results. Regarding the structural properties of the B-N, Si-N and N-Si/B coordination…

Materials Science · Physics 2007-05-23 A. Hannemann , J. C. Schoen , C. Oligschleger , M. Jansen

Using the minima hopping global geometry optimization method on the density functional potential energy surface we study medium size and large boron clusters. Even though for isolated medium size clusters the ground state is a cage like…

Atomic and Molecular Clusters · Physics 2015-03-17 Sandip De , Alexander Willand , Maximilian Amsler , Pascal Pochet , Luigi Genovese , Stefan Goedecker

Based on crystal chemistry rationale and calculations within the density functional theory DFT, the U:B system is complemented with additional binary compounds UB3, U2B6, and UB6 possessing two-dimensional 2D and 3D boron substructures.…

Materials Science · Physics 2020-02-18 Samir F. Matar

Using density functional theory (DFT) and quantum Monte Carlo (QMC) calculations we show that the B12Hn and B12Fn (n = 0-4) quasi-planar structures are energetically more favorable than the corresponding icosahedral clusters. Moreover, we…

Mesoscale and Nanoscale Physics · Physics 2021-09-21 N. Gonzalez Szwacki , C. J. Tymczak
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