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We demonstrate one-dimensional Doppler cooling of a beam of buffer-gas cooled Barium monofluoride (BaF) molecules. The dependences of the cooling efficiency with the laser detuning, the bias filed and the laser intensity are carefully…

Atomic Physics · Physics 2022-03-23 Yuhe Zhang , Zixuan Zeng , Qian Liang , Wenhao Bu , Bo Yan

We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…

A novel method of electron beam cooling is considered which can be used for linear colliders. The electron beam is cooled during collision with focused powerful laser pulse. With reasonable laser parameters (laser flash energy about 10 J)…

High Energy Physics - Experiment · Physics 2013-10-25 Valery Telnov

We use two-dimensional transverse laser cooling to produce an ultracold beam of YbF molecules. Through experiments and numerical simulations, we study how the cooling is influenced by the polarization configuration, laser intensity, laser…

We demonstrate buffer-gas cooling, high-resolution spectroscopy and cycling fluorescence of cold barium monofluoride (BaF) molecules. Our source produces an intense and internally cold molecular beam containing the different BaF…

Atomic Physics · Physics 2020-01-13 Ralf Albrecht , Michael Scharwaechter , Tobias Sixt , Lucas Hofer , Tim Langen

Precision measurements of the electron's electric dipole moment (eEDM) are critical for testing fundamental symmetries in particle physics, and heavy polar molecules-such as barium monofluoride (BaF)-have emerged as promising candidates for…

Atomic Physics · Physics 2026-01-01 Shuhua Deng , Shoukang Yang , Zixuan Zeng , Bo Yan

Achieving high-quality electron beams from laser-plasma accelerators critically relies on density tailoring to control electron dynamics during injection, acceleration, and extraction. We report on the experimental observation of electron…

We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation…

Atomic Physics · Physics 2017-03-22 Wenhao Bu , Tao Chen , Guitao Lv , Bo Yan

Currently, there is great interest in laser cooling of barium monofluoride (BaF) molecules for precision tests of fundamental symmetries. We use high-resolution absorption spectroscopy to characterize several as yet imprecisely known…

Atomic Physics · Physics 2024-12-16 Marian Rockenhäuser , Felix Kogel , Einius Pultinevicius , Tim Langen

We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…

Atomic Physics · Physics 2022-08-24 S. F. Vázquez-Carson , Q. Sun , J. Dai , D. Mitra , T. Zelevinsky

We report an experimental investigation on the Doppler-free saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride (BaF) molecules in a 4~K cryogenic cell. The obtained spectra with a resolution of 19~MHz, much smaller…

Atomic Physics · Physics 2023-02-14 Wenhao Bu , Yuhe Zhang , Qian Liang , Tao Chen , Bo Yan

A thermal atomic beam of dysprosium (Dy) atoms is cooled using the $4f^{10}6s^2 (J=8) \to 4f^{10}6s6p (J=9)$ transition at 421 nm. The cooling is done via a standing light wave orthogonal to the atomic beam. Efficient transverse cooling to…

Atomic Physics · Physics 2013-05-29 N. Leefer , A. Cingöz , B. Gerber-Siff , Arijit Sharma , J. R. Torgerson , D. Budker

A full density-matrix simulation is performed for optical deflection of a barium monofluoride ($^{138}$Ba$^{19}$F) beam using the bichromatic force, which employs pairs of counter-propagating laser beams that are offset in frequency. We…

Atomic Physics · Physics 2023-07-26 A. Marsman , M. Horbatsch , E. A. Hessels

There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…

Atomic Physics · Physics 2013-05-30 J. F. Barry , E. S. Shuman , E. B. Norrgard , D. DeMille

We demonstrate laser cooling of barium monofluoride (138BaF) molecules. We use serrodynes to synthesize time-sequenced optical spectra that can be precisely tailored to the hyperfine structure of this heaviest non-radioactive alkaline earth…

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

Atomic Physics · Physics 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

We present a cold atomic beam source based on a two-dimensional (2D)+ magneto-optical trap (MOT), capable of generating a continuous cold beam of 87Rb atoms with a flux up to 4.3*10^9 atoms/s, a mean velocity of 10.96(2.20) m/s, and a…

Atomic Physics · Physics 2023-12-20 Shengzhe Wang , Zhixin Meng , and Peiqiang Yan , Yuanxing Liu , Yanying Feng

In work is considered average transverse dynamics of an electron beam in the autoresonant laser. It is shown, that in approach of the given external electromagnetic wave (small gain free electron laser) transverse emittance of a beam of the…

Accelerator Physics · Physics 2009-11-07 R. V. Tumanian

Direct laser cooling of molecules has made significant progress in recent years. However, the selective cooling and manipulation of molecules based on their isotopic composition, which is ubiquitous in atomic laser cooling, has not yet been…

A cryogenic neon solid doped with barium monofluoride (BaF) is created on a cryogenic substrate using a stream of Ne gas and a high-intensity beam of BaF molecules produced in a cryogenic helium-buffer-gas laser-ablation source. The…

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