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More than fifty years ago, excitonic insulators, formed by the pairing of electrons and holes due to Coulomb interactions, were first predicted. Since then, excitonic insulators have been observed in various classes of materials, including…

By systematic theoretical calculations, we have revealed an excitonic insulator (EI) in the Ta2Pd3Te5 monolayer. The bulk Ta2Pd3Te5 is a van der Waals (vdW) layered compound, whereas the vdW layer can be obtained through exfoliation or…

First-principles calculations reveal an unusual electronic state (dubbed as half excitonic insulator) in monolayer 1T-MX2 (M = Co, Ni and X = Cl, Br). Its one spin channel has a many-body ground state due to excitonic instability, while the…

Materials Science · Physics 2019-06-19 Zeyu Jiang , Yuanchang Li , Wenhui Duan , Shengbai Zhang

The excitonic insulator (EI) is a Bose-Einstein condensation (BEC) of excitons bound by electron-hole interaction in a solid, which could support high-temperature BEC transition. The material realization of EI has been elusive, which is…

An excitonic insulator$^{1,2}$ (EI) is a correlated many-body state of electron-hole pairs, potentially leading to high-temperature condensate and superfluidity$^{3-7}$. Despite ever-growing experiments suggesting possible EI states in…

Materials Science · Physics 2025-03-17 Fang Zhang , Jiawei Ruan , Gurjyot Sethi , Chen Hu , Steven G. Louie

Quantum spin-hall insulator (QSHI) processes nontrivial topology. We notice that the electronic structures of some particular QSHIs are favorable for realization of excitonic insulators (EIs). Using first-principles many-body perturbation…

Materials Science · Physics 2023-04-04 Huaiyuan Yang , Jiaxi Zeng , Yuelin Shao , Yuanfeng Xu , Xi Dai , Xin-Zheng Li

First-principles density functional theory plus Bethe-Salpeter equation calculations are employed to investigate the electronic and excitonic properties of monolayer titanium trichalcogenide alloys TiS$_{3-x}$Se$_x$ ($x$=1 and 2). It is…

Materials Science · Physics 2020-12-02 Shan Dong , Yuanchang Li

Bose-Einstein condensation of electron-hole pairs, exciton condensation, has been effortfully investigated since predicted 60 years ago. Irrefutable evidence has still been lacking due to experimental difficulties in verifying the…

Strongly Correlated Electrons · Physics 2023-04-11 Akihiko Ikeda , Yasuhiro H. Matsuda , Keisuke Sato , Yuto Ishii , Hironobu Sawabe , Daisuke Nakamura , Shojiro Takeyama , Joji Nasu

We predict Bose-Einstein condensation and superfluidity of dipolar excitons, formed by electron-hole pairs in spatially separated gapped hexagonal $\alpha-T_{3}$ (GHAT3) layers. In the $\alpha-T_{3}$ model, the AB-honeycomb lattice…

Materials Science · Physics 2024-09-06 Oleg L. Berman , Godfrey Gumbs , Gabriel P. Martins , Paula Fekete

Analogous to the charged electron-electron pair condensation in superconductors, an excitonic insulator (EI) represents Fermi surface instability due to spontaneous formation and condensation of charge-neutral electron-hole pair (exciton).…

Strongly Correlated Electrons · Physics 2024-05-28 R. Okuma , K. Yamagami , Y. Fujisawa , C. H. Hsu , Y. Obata , N. Tomoda , M. Dronova , K. Kuroda , H. Ishikawa , K. Kawaguchi , K. Aido , K. Kindo , Y. H. Chan , H. Lin , Y. Ihara , T. Kondo , Y. Okada

Owing to their integer spin, exciton-polaritons in microcavities can be used for observation of non-equilibrium Bose-Einstein condensation in solid state. However, spin-related phenomena of such condensates are difficult to explore due to…

The electronic properties of excitonic insulators have been examined precisely in recent years. Pictures of exciton condensation may be applied to the spin-state transition observed in perovskite cobalt oxides. We examine the crystal-field…

Strongly Correlated Electrons · Physics 2022-10-12 Koya Kitagawa , Hiroaki Matsueda

The interplay between topology and correlations can generate a variety of quantum phases, many of which remain to be explored. Recent advances have identified monolayer WTe2 as a promising material for doing so in a highly tunable fashion.…

Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature, and exciton condensates can be realized at much higher temperature than condensates of atoms because of strong…

Excitonic insulators are usually considered to form via the condensation of a soft charge mode of bound electron-hole pairs. This, however, presumes that the soft exciton is of spin-singlet character. Early theoretical considerations have…

Strongly Correlated Electrons · Physics 2022-02-18 D. G. Mazzone , Y. Shen , H. Suwa , G. Fabbris , J. Yang , S-S. Zhang , H. Miao , J. Sears , Ke Jia , Y. G. Shi , M. H. Upton , D. M. Casa , X. Liu , J. Liu , C. D. Batista , M. P. M. Dean

Excitonic Bose-Einstein condensation (EBEC) has drawn increasing attention recently with the emergence of 2D materials. A general criterion for EBEC, as expected in an excitonic insulator (EI) state, is to have negative exciton formation…

Strongly Correlated Electrons · Physics 2023-05-05 Gurjyot Sethi , Martin Cuma , Feng Liu

We employ mean-field approximation to investigate the interplay between the nontrivial band topology and the formation of excitonic insulator (EI) in a one-dimensional chain of atomic $s-p$ orbitals in the presence of repulsive…

Strongly Correlated Electrons · Physics 2021-01-04 Zahra Khatibi , Roya Ahemeh , Mehdi Kargarian

We predict a phase transition in freestanding monolayer Xenes from the semiconducting phase to the excitonic insulating (EI) phase can be induced by reducing an external electric field below some critical value which is unique to each…

Mesoscale and Nanoscale Physics · Physics 2019-01-18 Matthew N. Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

Excitonic insulators (EI) arise from the formation of bound electron-hole pairs (excitons) in semiconductors and provide a solid-state platform for quantum many-boson physics. Strong exciton-exciton repulsion is expected to stabilize…

Excitons, the bosonic quasiparticle emerging from Coulomb interaction between electrons and holes, will undergo a Bose-Einstein condensation(BEC) and transition into a superfluid state with global phase coherence at low temperatures. An…

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