Related papers: Giant Magneto-Optical Effects in Two-Dimensional F…
The recent discovery of long-range magnetic order in atomically thin films has triggered particular interest in two-dimensional (2D) van der Waals (vdW) magnetic materials. In this paper, we perform a systematic theoretical study of the…
The interplay of polarization and magnetism in materials with light can create rich nonlinear magneto-optical (NLMO) effects, and the recent discovery of two-dimensional (2D) van der Waals magnets provides remarkable control over NLMO…
Magneto-optical effect has been widely used in light modulation, optical sensing and information storage. Recently discovered two-dimensional (2D) van der Waals layered magnets are considered as promising platforms for investigating novel…
2D magnetic semiconductors, which intrinsically couple a rich landscape of magnetic orders with tightly bound electron-hole pairs (excitons), present an exciting platform to investigate the interplay between optical and magnetic phenomena…
Metallic nanostructures exhibit strong nonlinear-optical response at surface plasmon resonances, where the light-matter coupling efficiency is enhanced. An active modulation of this response can be realized by means of an external magnetic…
We calculate the Raman spectrum of the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet by exact diagonalization and quantum Monte Carlo techniques on clusters of up to 144 sites and, on a 16-site cluster, by considering the…
We calculate magnetic Raman spectra of Heisenberg antiferromagnets on the two-dimensional Penrose lattice. We follow the Shastry-Shraiman formulation of Raman scattering in a strongly correlated Hubbard system and obtain the second- and…
Nonreciprocal devices that allow the light propagation in only one direction are indispensable in photonic circuits and emerging quantum technologies. Contemporary optical isolators and circulators, however, require large size or strong…
The second-order magneto-optical effects, represented by Voigt and Sch\"{a}fer-Hubert effects, are effective methods to detect the spin textures in antiferromagnets, whereas the previous studies are usually limited to collinear…
We have observed a quadratic x-ray magneto-optical effect in near-normal incidence reflection at the M-edges of iron. The effect appears as the magnetically induced rotation of ca. 0.1$ degrees of the polarization plane of linearly…
We study the dynamical response function relevant for two-dimensional coherent nonlinear optical spectroscopy of the antiferromagnetic frustrated $J_{1}$-$J_{3}$ Heisenberg model on the square lattice within its long-range ordered,…
When two-dimensional electron gases (2DEGs) are exposed to magnetic field, they resonantly absorb electromagnetic radiation via electronic transitions between Landau levels (LLs). In 2DEGs with a Dirac spectrum, such as graphene, theory…
We report the optical and magneto-optical properties of K2V3O8, an S=1/2 quasi-two-dimensional Heisenberg antiferromagnet. Local spin density approximation electronic structure calculations are used to assign the observed excitations and…
A prominent character of two-dimensional magnetic systems is the enhanced spin fluctuations, which however reduce the ordering temperature. Here we report that a magnetic field of only one-thousandth of the Heisenberg superexchange…
Our experimental (neutron diffraction, M\"ossbauer spectroscopy, magnetic susceptibility, specific heat) and numerical studies on the evolution of short- and long-range magnetic order in $\gamma_{\rm II}$-Li\(_2\)FeSiO\(_4\) suggest a…
We employ first principles density-functional theory (DFT) and the Bethe-Salpeter equation (BSE) in the framework of tight-binding based maximally localized Wannier functions (MLWF-TB) model to investigate the electronic and optical…
We have uncovered a giant gyrotropic magneto-optical response for doped ferromagnetic manganite La2/3Ca1/3MnO3 around the near room-temperature paramagnetic-to-ferromagnetic transition. At odds with current wisdom, where this response is…
Quantum magnets in two dimensions display strong quantum interaction effects even when magnetically ordered. Using the metal-organic framework material CuF$_2$(D$_2$O)$_2$(pyz), we investigate the field-dependent spin dynamics of the $S =…
We present a theoretical study on the Landau levels (LLs) and magneto-optical absorption of a two-dimensional semi-Dirac electron system under a perpendicular magnetic field. Based on an effective k.p Hamiltonian, we find that the LLs are…
Motivated by recent experiments on quantum magnet NiCl$_{2}$-4SC(NH$_{2}$)$_{2}$ (DTN) and its Br-doped counterpart DTNX we propose a theoretical description of optical magnon branch in the antiferromagnet with large single-ion anisotropy…